182 research outputs found
Ultrafast all-optical switching by cross phase modulation induced wavelength conversion in silicon-on-insulator waveguides and ring resonators
We present new results on ultrafast alloptical wavelength conversion in Silicon-on-Insulator waveguides through cross phase modulation. We demonstrate sub-picosecond all-optical switching with 13dB on/off ratio by combining the nonlinear wavelength conversion in the port waveguide with passive filtering using an integrated SOI microring resonator.\u
Ultrafast all-optical wavelength conversion in silicon-insulator waveguides by means of cross phase modulation using 300 femtosecond pulses
In this paper we report the ultrafast all-optical wavelength conversion in Silicon-on-Insulator (SOI) waveguides. We used a pump-probe setup with 300 femtosecond pulses to demonstrate large temporal phase-shifts, caused by the Kerr effect and free carrier generation. Large wavelength shifts of a 1683nm probe signal have been observed. The wavelength conversion, ranging from 10nm redshifts to 15nm blueshifts, depending on the time delay between the pump and probe pulses, is caused by the pump induced Cross Phase Modulation. Furthermore, an all-optical switching scheme using SOI microring resonators is discussed. These results enable ultrafast all-optical switching using SOI microring resonators
Ultrafast all-optical wavelength conversion in silicon waveguides using femtosecond pump-probe pulses
Experimental results on ultrafast all-optical wavelength conversion in silicon-on-insulator waveguides are presented. Red and blue shifts of 10nm have been observed in femtosecond pump-probe experiments. Alloptical switching and the importance of waveguide dispersion are discussed
Coherent Modulation of the YBa2Cu3O6+x Atomic Structure by Displacive Stimulated Ionic Raman Scattering
We discuss the mechanism of coherent phonon generation by Stimulated Ionic
Raman Scattering, a process different from conventional excitation with near
visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling
between a directly excited infrared-active phonon mode and other Raman modes.
We experimentally study the response of YBa2Cu3O6+x to the resonant excitation
of apical oxygen motions at 20 THz by mid-infrared pulses, which has been shown
in the past to enhance the interlayer superconducting coupling. We find
coherent oscillations of four totally symmetric (Ag) Raman modes and make a
critical assessment of the role of these oscillatory motions in the enhancement
of superconductivity.Comment: 12 pages, 4 figure
Pump frequency resonances for light-induced incipient superconductivity in YBaCuO
Optical excitation in the cuprates has been shown to induce transient
superconducting correlations above the thermodynamic transition temperature,
, as evidenced by the terahertz frequency optical properties in the
non-equilibrium state. In YBaCuO this phenomenon has so far
been associated with the nonlinear excitation of certain lattice modes and the
creation of new crystal structures. In other compounds, like
LaBaCuO, similar effects were reported also for excitation at
near infrared frequencies, and were interpreted as a signature of the melting
of competing orders. However, to date it has not been possible to
systematically tune the pump frequency widely in any one compound, to
comprehensively compare the frequency dependent photo-susceptibility for this
phenomenon. Here, we make use of a newly developed optical parametric
amplifier, which generates widely tunable high intensity femtosecond pulses, to
excite YBaCuO throughout the entire optical spectrum (3 - 750
THz). In the far-infrared region (3 - 25 THz), signatures of non-equilibrium
superconductivity are induced only for excitation of the 16.4 THz and 19.2 THz
vibrational modes that drive -axis apical oxygen atomic positions. For
higher driving frequencies (25 - 750 THz), a second resonance is observed
around the charge transfer band edge at ~350 THz. These observations highlight
the importance of coupling to the electronic structure of the CuO planes,
either mediated by a phonon or by charge transfer.Comment: 47 pages, 21 figures, 2 table
Self Phase Modulation and Stimulated Raman Scattering due to High Power Femtosecond Pulse Propagation in Silicon-on-Insulator Waveguides.
Self Phase Modulation (SPM) and Stimulated Raman Scattering (SRS) in silicon waveguides have been observed and will be discussed theoretically using a modified Nonlinear Schrödinger Equation. The high optical peak powers needed for the experiments were obtained by coupling sub-picosecond (200fs) transform limited pulses with a spectral width of 12nm into a single mode silicon waveguide. Spectral broadening up to 50nm has been observed due to Self Phase Modulation. An intensity increase of the idler spectrum around 1650nm at the expense of the 1550nm pump signal has been observed as function of pump power, indicating the presence of Stimulated Raman Scattering
Nonlocal nonlinear phononics
Nonlinear phononics relies on the resonant optical excitation of infrared-active lattice vibrations to induce targeted structural deformations in solids. This form of dynamical crystal structure design has been applied to control the functional properties of many complex solids, including magnetic materials, superconductors and ferroelectrics. However, phononics has so far been restricted to protocols in which structural deformations occur within the optically excited volume, sometimes resulting in unwanted heating. Here, we extend nonlinear phononics to propagating polaritons, spatially separating the functional response from the optical drive. We use mid-infrared optical pulses to resonantly drive a phonon at the surface of ferroelectric LiNbO3. Time-resolved stimulated Raman scattering reveals that the ferroelectric polarization is reduced over the entire 50 µm depth of the sample, far beyond the micrometre depth of the evanescent phonon field. We attribute this effect to the anharmonic coupling between the driven mode and a polariton that propagates into the material. For high excitation amplitudes, we reach a regime in which the ferroelectric polarization is reversed, as revealed by a sign change in the Raman tensor coefficients of all the polar modes
Nonlinear electron-phonon coupling in doped manganites
We employ time-resolved resonant x-ray diffraction to study the melting of
charge order and the associated insulator-metal transition in the doped
manganite PrCaMnO after resonant excitation of a
high-frequency infrared-active lattice mode. We find that the charge order
reduces promptly and highly nonlinearly as function of excitation fluence.
Density functional theory calculations suggest that direct anharmonic coupling
between the excited lattice mode and the electronic structure drive these
dynamics, highlighting a new avenue of nonlinear phonon control
Comparison of charge modulations in LaBaCuO and YBaCuO
A charge modulation has recently been reported in (Y,Nd)BaCuO
[Ghiringhelli {\em et al.} Science 337, 821 (2013)]. Here we report Cu
edge soft x-ray scattering studies comparing the lattice modulation associated
with the charge modulation in YBaCuO with that associated with
the well known charge and spin stripe order in LaBaCuO.
We find that the correlation length in the CuO plane is isotropic in both
cases, and is \AA for LaBaCuO and \AA for YBaCuO. Assuming weak inter-planar correlations of
the charge ordering in both compounds, we conclude that the order parameters of
the lattice modulations in LaBaCuO and
YBaCuO are of the same order of magnitude.Comment: 3 pages, 2 figure
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