106 research outputs found
High-temperature superconductivity from fine-tuning of Fermi-surface singularities in iron oxypnictides
In the family of the iron-based superconductors, the FeAsO-type compounds
(with being a rare-earth metal) exhibit the highest bulk superconducting
transition temperatures () up to and thus hold
the key to the elusive pairing mechanism. Recently, it has been demonstrated
that the intrinsic electronic structure of SmFeCoAsO
() is highly nontrivial and consists of multiple
band-edge singularities in close proximity to the Fermi level. However, it
remains unclear whether these singularities are generic to the FeAsO-type
materials and if so, whether their exact topology is responsible for the
aforementioned record . In this work, we use angle-resolved
photoemission spectroscopy (ARPES) to investigate the inherent electronic
structure of the NdFeAsOF compound with a twice higher
. We find a similarly singular Fermi surface and
further demonstrate that the dramatic enhancement of superconductivity in this
compound correlates closely with the fine-tuning of one of the band-edge
singularities to within a fraction of the superconducting energy gap
below the Fermi level. Our results provide compelling evidence that the
band-structure singularities near the Fermi level in the iron-based
superconductors must be explicitly accounted for in any attempt to understand
the mechanism of superconducting pairing in these materials.Comment: Open access article available online at
http://www.nature.com/articles/srep1827
Anomalously enhanced photoemission from the Dirac point and symmetry of the self-energy variations for the surface states in Bi2Se3
Accurate analysis of the photoemission intensity from the surface states of
Bi2Se3 reveals two unusual features: spectral line asymmetry and anomalously
enhanced photoemission from the Dirac point. The former indicates a certain
symmetry of a scattering process, which results in strongly k\omega-dependent
contribution to the imaginary part of the self-energy that changes sign while
crossing both the dispersion curves and the energy of the Dirac point. The
latter is hard to describe by one particle spectral function while a final
state interference seems to be plausible explanation
Photoemission induced gating of topological insulator
The recently discovered topological insulators exhibit topologically
protected metallic surface states which are interesting from the fundamental
point of view and could be useful for various applications if an appropriate
electronic gating can be realized. Our photoemission study of Cu intercalated
Bi2Se3 shows that the surface states occupancy in this material can be tuned by
changing the photon energy and understood as a photoemission induced gating
effect. Our finding provides an effective tool to investigate the new physics
coming from the topological surface states and suggests the intercalation as a
recipe for synthesis of the material suitable for electronic applications.Comment: + resistivity data and some discussio
Resistivity and Hall effect of LiFeAs: Evidence for electron-electron scattering
LiFeAs is unique among the broad family of FeAs-based superconductors,
because it is superconducting with a rather large K under
ambient conditions although it is a stoichiometric compound. We studied the
electrical transport on a high-quality single crystal. The resistivity shows
quadratic temperature dependence at low temperature giving evidence for strong
electron-electron scattering and a tendency towards saturation around room
temperature. The Hall constant is negative and changes with temperature, what
most probably arises from a van Hove singularity close to the Fermi energy in
one of the hole-like bands. Using band structure calculations based on angular
resolved photoemission spectra we are able to reproduce all the basic features
of both the resistivity as well as the Hall effect data.Comment: 6 pages, 3 figures included; V2 has been considerably revised and
contain a more detailed analysis of the Hall effect dat
Non-monotonic pseudo-gap in high-Tc cuprates
The mechanism of high temperature superconductivity is not resolved for so
long because the normal state of cuprates is not yet understood. Here we show
that the normal state pseudo-gap exhibits an unexpected non-monotonic
temperature dependence, which rules out the possibility to describe it by a
single mechanism such as superconducting phase fluctuations. Moreover, this
behaviour, being remarkably similar to the behaviour of the charge ordering gap
in the transition-metal dichalcogenides, completes the correspondence between
these two classes of compounds: the cuprates in the PG state and the
dichalcogenides in the incommensurate charge ordering state reveal virtually
identical spectra of one-particle excitations as function of energy, momentum
and temperature. These results suggest that the normal state pseudo-gap, which
was considered to be very peculiar to cuprates, seems to be a general complex
phenomenon for 2D metals. This may not only help to clarify the normal state
electronic structure of 2D metals but also provide new insight into electronic
properties of 2D solids where the metal-insulator and metal-superconductor
transitions are considered on similar basis as instabilities of particle-hole
and particle-particle interaction, respectively
The superconducting gaps in LiFeAs: Joint study of specific heat and ARPES
We present specific heat, c_P, and ARPES data on single crystals of the
stoichiometric superconductor LiFeAs. A pronounced anomaly is found in c_P at
the superconducting transition. The electronic contribution can be described by
two s-type energy gaps with magnitudes of approximately Delta1 = 1.2 meV and
Delta2 = 2.6 meV and a normal-state gamma coefficient of 10 mJ/mol K^2. All
these values are in remarkable agreement with ARPES results.Comment: 4 pages, 3 figure
Pseudogap in the chain states of YBCO
As established by scanning tunneling microscopy (STM) cleaved surfaces of the
high temperature superconductor YBaCuO develop charge
density wave (CDW) modulations in the one-dimensional (1D) CuO chains. At the
same time, no signatures of the CDW have been reported in the spectral function
of the chain band previously studied by photoemission. We use soft X-ray angle
resolved photoemission (SX-ARPES) to detect a chain-derived surface band that
had not been detected in previous work. The for the new surface
band is found to be 0.55\,\AA, which matches the wave vector of the CDW
observed in direct space by STM. This reveals the relevance of the Fermi
surface nesting for the formation of CDWs in the CuO chains in
YBaCuO. In agreement with the short range nature of the
CDW order the newly detected surface band exhibits a pseudogap, whose energy
scale also corresponds to that observed by STM
A weak-coupling superconductivity in the electron doped NaFeCoAs is revealed by ARPES
We report a systematic study on the electronic structure and superconducting
(SC) gaps in electron doped NaFeCoAs superconductor using
angle-resolved photoemission spectroscopy. Hole-like Fermi sheets are at the
zone center and electron-like Fermi sheets are at the zone corner, and are
mainly contributed by and orbital characters. Our results reveal a
in the range of 1.8-2.1, suggesting a weak-coupling
superconductivity in these compounds. Gap closing above the transition
temperature () shows the absence of pseudogaps. Gap evolution with
temperature follow the BCS gap equation near the , , and high
symmetry points. Furthermore, an almost isotropic superconductivity along
direction in the momentum space is observed by varying the excitation energies.Comment: 6 pages, 5 figures, Accepted by Phy.Rev.
- …