Doping dependent optical properties of Bi2201

An experimental study of the in-plane optical conductivity of (Pb$_{x}$,Bi$_{2-x}$)(La$_{y}$Sr$_{2-y}$)CuO$_{6+\delta}$ (Bi2201) is presented for a broad doping and temperature range. The in-plane conductivity is analyzed within a strong coupling formalism. We address the interrelationship between the optical conductivity ($\sigma(\omega)$), the single particle self energy, and the electron-boson spectral function. We find that the frequency and temperature dependence can be well described within this formalism. We present a universal description of optical, ARPES and tunneling spectra. The full frequency and temperature dependence of the optical spectra and single particle self-energy is shown to result from an electron-boson spectral function, which shows a strong doping dependence and weak temperature dependence.Comment: 20 pages, 9 figures. To appear in special focus issue "Superconductors with Exotic Symmetries", New Journal of Physic

Infrared phonon activity in pristine graphite

We study experimentally and theoretically the Fano-shaped phonon peak at 1590 cm$^{-1}$ (0.2 eV) in the in-plane optical conductivity of pristine graphite. We show that the anomalously large spectral weight and the Fano asymmetry of the peak can be qualitatively accounted for by a charged-phonon theory. A crucial role in this context is played by the particle-hole asymmetry of the electronic $\pi$-bands.Comment: 5 pages, 4 figures, 1 tabl

Optical determination of the relation between the electron-boson coupling function and the critical temperature in high Tc_c cuprates

We take advantage of the connection between the free carrier optical conductivity and the glue function in the normal state, to reconstruct from the infrared optical conductivity the glue-spectrum of ten different high-Tc cuprates revealing a robust peak in the 50-60 meV range and a broad con- tinuum at higher energies for all measured charge carrier concentrations and temperatures up to 290 K. We observe that the strong coupling formalism accounts fully for the known strong temperature dependence of the optical spectra of the high Tc cuprates, except for strongly underdoped samples. We observe a correlation between the doping trend of the experimental glue spectra and the critical temperature. The data obtained on the overdoped side of the phase diagram conclusively excludes the electron-phonon coupling as the main source of superconducting pairing.Comment: Accepted for publication in Phys. Rev.

The cleavage surface of the BaFe_(2-x)Co_(x)As_(2) and Fe_(y)Se_(1-x)Te_(x) superconductors: from diversity to simplicity

We elucidate the termination surface of cleaved single crystals of the BaFe_(2-x)Co_(x)As_(2) and Fe_(y)Se_(1-x)Te_(x) families of the high temperature iron based superconductors. By combining scanning tunneling microscopic data with low energy electron diffraction we prove that the termination layer of the Ba122 systems is a remnant of the Ba layer, which exhibits a complex diversity of ordered and disordered structures. The observed surface topographies and their accompanying superstructure reflections in electron diffraction depend on the cleavage temperature. In stark contrast, Fe_(y)Se_(1-x)Te_(x) possesses only a single termination structure - that of the tetragonally ordered Se_(1-x)Te_(x) layer.Comment: 4 pages, 4 figure

Epitaxial growth and thermodynamic stability of SrIrO3/SrTiO3 heterostructures

Obtaining high-quality thin films of 5d transition metal oxides is essential to explore the exotic semimetallic and topological phases predicted to arise from the combination of strong electron correlations and spin-orbit coupling. Here, we show that the transport properties of SrIrO3 thin films, grown by pulsed laser deposition, can be optimized by considering the effect of laser-induced modification of the SrIrO3 target surface. We further demonstrate that bare SrIrO3 thin films are subject to degradation in air and are highly sensitive to lithographic processing. A crystalline SrTiO3 cap layer deposited in-situ is effective in preserving the film quality, allowing us to measure metallic transport behavior in films with thicknesses down to 4 unit cells. In addition, the SrTiO3 encapsulation enables the fabrication of devices such as Hall bars without altering the film properties, allowing precise (magneto)transport measurements on micro- and nanoscale devices.Comment: 5 pages, 3 figure

In-plane optical spectral weight transfer in optimally doped Bi2_{2}Sr2_{2}Ca2_{2}Cu3_{3}O10_{10}

We examine the redistribution of the in-plane optical spectral weight in the normal and superconducting state in tri-layer \bbb (Bi2223) near optimal doping ($T_c$ = 110 K) on a single crystal via infrared reflectivity and spectroscopic ellipsometry. We report the temperature dependence of the low-frequency integrated spectral weight $W(\Omega_c)$ for different values of the cutoff energy $\Omega_c$. Two different model-independent analyses consistently show that for $\Omega_c$ = 1 eV, which is below the charge transfer gap, $W(\Omega_c)$ increases below $T_c$, implying the lowering of the kinetic energy of the holes. This is opposite to the BCS scenario, but it follows the same trend observed in the bi-layer compound \bb (Bi2212). The size of this effect is larger in Bi2223 than in Bi2212, approximately scaling with the critical temperature. In the normal state, the temperature dependence of $W(\Omega_c)$ is close to $T^2$ up to 300 K

Optical Integral in the Cuprates and the Question of Sum Rule Violation

Much attention has been given to a possible violation of the optical sum rule in the cuprates, and the connection this might have to kinetic energy lowering. The optical integral is composed of a cut-off independent term (whose temperature dependence is a measure of the sum rule violation), plus a cut-off dependent term that accounts for the extension of the Drude peak beyond the upper bound of the integral. We find that the temperature dependence of the optical integral in the normal state of the cuprates can be accounted for solely by the latter term, implying that the dominant contribution to the observed sum rule `violation' in the normal state is due to the finite cut-off. This cut-off dependent term is well modeled by a theory of electrons interacting with a broad spectrum of bosons.Comment: some clarifications and minor additions are offered in the final (published) versio

From bad metal to Kondo insulator:Temperature evolution of the optical properties of SmB6

The recent rekindling of interest in the mixed valent Kondo insulator SmB$_{6}$ as candidate for a first correlated topological insulator has resulted in a wealth of new experimental observations. In particular, angle-resolved photoemission experiments have provided completely new insights into the formation of the low temperature Kondo insulating state starting from the high temperature correlated metal. Here, we report detailed temperature and energy dependent measurements of the optical constants of SmB$_6$ in order to provide a detailed study from the point of view of a bulk sensitive spectroscopic probe. We detect a previously unobserved infrared active optical phonon mode, involving the movement of the Sm ions against the boron cages. The changes taking place in the free carrier response with temperature and their connection to changes in optical transitions between different bands are discussed. We find that the free charge density starts to decrease rapidly below approximately 200 K. Below 60 K a small amount of spectral weight begins to accumulate in low lying interband transitions, indicating the formation of the Kondo insulating state; however, the total integrated spectral weight in our experimental window ($\sim 4.35$ eV) decreases. This indicates the involvement of a large Coulomb interaction ($>$ 5 eV) in the formation of the Kondo insulator.Comment: 10 pages, 7 figures (including supp.). Accepted for publication in New Journal of Physic