Observation of superspin glass state in magnetically textured ferrofluid (gamma-Fe2O3)

Magnetic properties in a magnetically textured ferrofluid made out of interacting maghemite (gamma-Fe2O3) nanoparticles suspended in glycerin have been investigated. Despite the loss of uniform distribution of anisotropy axes, a superspin glass state exists at low temperature in a concentrated, textured ferrofluid as in the case of its non-textured counterpart. The onset of superspin glass state was verified from the sample's AC susceptibility. The influence of the anisotropy axis orientation on the aging behavior in the glassy states is also discussed

Nondestructive Testing Using Magnetic Field Visualization Technique

This paper describes a new technique to detect cracks or flaws in conducting or ferromagnetic materials using a magnetic field visualization system. In this system there are two sources for magnetic field generation, i.e. electrical current and magnetization. And the magnetic field generated by the source could give us useful information on cracks or flaws included in the material. Thus, visualization of magnetic field would enable us to identify the shape and size of cracks. We developed a preliminary system to verify the validity of the speculation and applied it to both ferromagnetic and conducting materials with flaws. The applicability of magnetic visualization has been confirmed to be an effective method in NDE and diagnosis of magnetic equipments in the present experiment. Furthermore, combination of this method with numerical prediction could demonstrate more potential capability in the field of NDE</p

Intrinsic Low Temperature Paramagnetism in B-DNA

We present experimental study of magnetization in $\lambda$-DNA in conjunction with structural measurements. The results show the surprising interplay between the molecular structures and their magnetic property. In the B-DNA state, $\lambda$-DNA exhibits paramagnetic behaviour below 20 K that is non-linear in applied magnetic field whereas in the A-DNA state, remains diamagnetic down to 2 K. We propose orbital paramagnetism as the origin of the observed phenomena and discuss its relation to the existence of long range coherent transport in B-DNA at low temperature.Comment: 5 pages, 4 figures, submitted to Physical Review Letters October 200

Noise Measurement of Interacting Ferromagnetic Particles with High Resolution Hall Microprobes

We present our first experimental determination of the magnetic noise of a superspinglass made of < 1 pico-liter frozen ferrofluid. The measurements were performed with a local magnetic field sensor based on Hall microprobes operated with the spinning current technique. The results obtained, though preliminary, qualitatively agree with the theoretical predictions of Fluctuation-Dissipation theorem (FDT) violation [1].Comment: 4pages, 2 figure

Growth of a dynamical correlation length in an aging superspin glass

We report on zero field cooled magnetization relaxation experiments on a concen- trated frozen ferrofluid exhibiting a low temperature superspin glass transition. With a method initially developed for spin glasses, we investigate the field dependence of the relaxations that take place after different aging times. We extract the typical number of correlated spins involved in the aging dynamics. This brings important insights into the dynamical correlation length and its time growth. Our results, consistent with expressions obtained for spin glasses, extend the generality of these behaviours to the class of superspin glasses. Since the typical flipping time is much larger for superspins than for atomic spins, our experiments probe a time regime much closer to that of numerical simulations

Superspin glass aging behavior in textured and nontextured frozen ferrofluid

The effect of magnetic anisotropy-axis alignment of individual nanoparticles on the collective aging behavior in the superspin glass state of a frozen ferrofluid has been investigated. The ferrofluid studied here consists of maghemite nanoparticles (\gamma-Fe2O3, mean diameter = 8.6 nm) dispersed in glycerin at a volume fraction of ~15%. The low temperature aging behavior has been explored through 'zero-field cooled magnetization' (ZFCM) relaxation measurements using SQUID magnetometry. The ZFCM response functions were found to scale with effective age of the system in both textured and non-textured superspin glass states, but with markedly different scaling exponents, \mu. The value of {\mu} was found to shift from ~0.9 in non-textured case to ~ 0.6 in the textured case, despite the identical cooling protocol used in both experiments

Non-generality of the Kadowaki-Woods ratio in correlated oxides

An explicit expression for the Kadowaki-Woods ratio in correlated metals is derived by invoking saturation of the (high-frequency) Fermi-liquid scattering rate at the Mott-Ioffe-Regel limit. Significant deviations observed in a number of oxides are quantitatively explained due to variations in carrier density, dimensionality, unit cell volume and the number of individual sheets in the Brillouin zone. A generic re-scaling of the original Kadowaki-Woods plot is also presented.Comment: 9 pages of text, 1 table, 2 figure

Anisotropy-axis orientation effect on the magnetization of {\gamma}-Fe2O3 frozen ferrofluid

The effect of magnetic anisotropy-axis alignment on the superparamagnetic (SPM) and superspin glass (SSG) states in a frozen ferrofluid has been investigated. The ferrofluid studied here consists of maghemite nanoparticles (\gamma-Fe2O3, mean diameter = 8.6 nm) dispersed in glycerine at a volume fraction of ~15%. In the high temperature SPM state, the magnetization of aligned ferrofluid increased by a factor varying between 2 and 4 with respect to that in the randomly oriented state. The negative interaction energy obtained from the Curie-Weiss fit to the high temperature susceptibility in the SPM states as well as the SSG phase onset temperature determined from the linear magnetization curves were found to be rather insensitive to the anisotropy axis alignment. The low temperature aging behaviour, explored via "zero-field cooled magnetization" (ZFCM) relaxation measurements, however, show distinct difference in the aging dynamics in the anisotropy-axis aligned and randomly oriented SSG states.Comment: to appear in Journal of Physics D: Applied Physic