79 research outputs found
Spin- and angle-resolved photoemission on topological materials
A historical review of spin- and angle-resolved photoemission on topological
materials is presented, aimed at readers who are new to the field or who wish
to obtain an overview of the activities in the field. The main focus lies on
topological insulators, but also Weyl and other semimetals will be discussed.
Further it will be explained why the measured spin polarisation from a spin
polarised state should always add up to 100% and how spin interference effects
influence the measured spin texture.Comment: Invited review article for special issue "ARPES Studies of
Topological Materials" in Electronic Structur
Determination of the time scale of photoemission from the measurement of spin polarization
The Eisenbud-Wigner-Smith (EWS) time delay of photoemission depends on the
phase term of the matrix element describing the transition. Because of an
interference process between partial channels, the photoelectrons acquire a
spin polarization which is also related to the phase term. The analytical model
for estimating the time delay by measuring the spin polarization is reviewed in
this manuscript. In particular, the distinction between scattering EWS and
interfering EWS time delay will be introduced, providing an insight in the
chronoscopy of photoemission. The method is applied to the recent experimental
data for Cu(111) presented in M. Fanciulli et al., PRL 118, 067402 (2017),
allowing to give better upper and lower bounds and estimates for the EWS time
delays.Comment: 30 pages, 5 figure
Tuning of the Rashba effect in Pb quantum well states via a variable Schottky barrier
Spin-orbit interaction (SOI) in low-dimensional systems results in the
fascinating property of spin-momentum locking. In a Rashba system the inversion
symmetry normal to the plane of a two-dimensional (2D) electron gas is broken,
generating a Fermi surface spin texture reminiscent of spin vortices of
different radii. This can be exploited in a spin-based field-effect transistor
(spin- FET), where the Rashba system forms a 2D channel between ferromagnetic
(FM) source and drain electrodes. The electron spin precesses when propagating
through the Rashba channel and spin orientations (anti)parallel to the drain
give (low) high conductivity. Crucial is the possibility to tune the momentum
splitting, and consequently the precession angle, through an external
parameter. Here we show that this can be achieved in Pb quantum well states
through the doping dependence of the Schottky barrier, opening up the
possibility of a terahertz spin-FET.Comment: 8 pages, 7 figure
Controlling the effective mass of quantum well states in Pb/Si(111) by interface engineering
The in-plane effective mass of quantum well states in thin Pb films on a Bi
reconstructed Si(111) surface is studied by angle-resolved photoemission
spectroscopy. It is found that this effective mass is a factor of three lower
than the unusually high values reported for Pb films grown on a Pb
reconstructed Si(111) surface. Through a quantitative low-energy electron
diffraction analysis the change in effective mass as a function of coverage and
for the different interfaces is linked to a change of around 2% in the in-plane
lattice constant. To corroborate this correlation, density functional theory
calculations were performed on freestanding Pb slabs with different in-plane
lattice constants. These calculations show an anomalous dependence of the
effective mass on the lattice constant including a change of sign for values
close to the lattice constant of Si(111). This unexpected relation is due to a
combination of reduced orbital overlap of the 6p_z states and altered
hybridization between the 6p_z and 6p_xy derived quantum well states.
Furthermore it is shown by core level spectroscopy that the Pb films are
structurally and temporally stable at temperatures below 100 K.Comment: 7 pages, 6 figure
Single spin-polarised Fermi surface in SrTiO thin films
The 2D electron gas (2DEG) formed at the surface of SrTiO(001) has
attracted great interest because of its fascinating physical properties and
potential as a novel electronic platform, but up to now has eluded a
comprehensible way to tune its properties. Using angle-resolved photoemission
spectroscopy with and without spin detection we here show that the band filling
can be controlled by growing thin SrTiO films on Nb doped SrTiO(001)
substrates. This results in a single spin-polarised 2D Fermi surface, which
bears potential as platform for Majorana physics. Based on our results it can
furthermore be concluded that the 2DEG does not extend more than 2 unit cells
into the film and that its properties depend on the amount of SrO at the
surface and possibly the dielectric response of the system
Observation of Wannier-Stark localization at the surface of BaTiO films by photoemission
Observation of Bloch oscillations and Wannier-Stark localization of charge
carriers is typically impossible in single-crystals, because an electric field
higher than the breakdown voltage is required. In BaTiO however, high
intrinsic electric fields are present due to its ferroelectric properties. With
angle-resolved photoemission we directly probe the Wannier-Stark localized
surface states of the BaTiO film-vacuum interface and show that this effect
extends to thin SrTiO overlayers. The electrons are found to be localized
along the in-plane polarization direction of the BaTiO film
Concept of a multichannel spin-resolving electron analyzer based on Mott scattering
The concept of a multichannel electron spin detector based on optical imaging principles and Mott scattering (iMott) is presented. A multichannel electron image produced by a standard angle-resolving (photo) electron analyzer or microscope is re-imaged by an electrostatic lens at an accelerating voltage of 40 kV onto the Au target. Quasi-elastic electrons bearing spin asymmetry of the Mott scattering are imaged by magnetic lenses onto position-sensitive electron CCDs whose differential signals yield the multichannel spin asymmetry image. Fundamental advantages of this concept include acceptance of inherently divergent electron sources from the electron analyzer or microscope focal plane as well as small aberrations achieved by virtue of high accelerating voltages, as demonstrated by extensive ray-tracing analysis. The efficiency gain compared with the single-channel Mott detector can be a factor of more than 10 4 which opens new prospects of spin-resolved spectroscopies in application not only to standard bulk and surface systems (Rashba effect, topological insulators, etc.) but also to buried heterostructures. The simultaneous spin detection combined with fast CCD readout enables efficient use of the iMott detectors at X-ray free-electron laser facilities
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