Role of Symmetry in Raman Spectroscopy of Unconventional Superconductors

The role of symmetry of the inelastic light scattering amplitude, the superconducting energy gap, and the underlying Fermi surface manifold on the Raman spectra of unconventional superconductors is discussed in detail. Particular emphasis is placed on both single and bi-layer superconductors. It is found that the $B_{1g}$ channel may be the most sensitive to doping due to the role of the Van Hove singularity. Lastly the effects of both disorder and spin fluctuations are considered. The theory imposes strong constraints on both the magnitude and symmetry of the energy gap for the bi-layer cuprates, indicating that a nearly identical energy gap of $d_{x^{2}-y^{2}}$ symmetry provides a best fit to the data.Comment: 12 pages, 4 postscript files, 1 tabl

Symmetry dependence of phonon lineshapes in superconductors with anisotropic gaps

The temperature dependence below $T_{c}$ of the lineshape of optical phonons of different symmetry as seen in Raman scattering is investigated for superconductors with anisotropic energy gaps. It is shown that the symmetry of the electron-phonon vertex produces non-trivial couplings to an anisotropic energy gap which leads to unique changes in the phonon lineshape for phonons of different symmetry. The phonon lineshape is calculated in detail for $B_{1g}$ and $A_{1g}$ phonons in a superconductor with $d_{x^{2}-y^{2}}$ pairing symmetry. The role of satellite peaks generated by the electron-phonon coupling are also addressed. The theory accounts for the substantial phonon narrowing of the $B_{1g}$ phonon, while narrowing of the $A_{1g}$ phonon which is indistinguishable from the normal state is shown, in agreement with recent measurements on BSCCO.Comment: 15 pages (3 Figures available upon request), Revtex, 1

Electronic Raman response in anisotropic metals

Using a generalized response theory we derive the electronic Raman response function for metals with anisotropic relaxation rates. The calculations account for the long--range Coulomb interaction and treat the collision operator within a charge conserving relaxation time approximation. We extend earlier treatments to finite wavenumbers ($|{\bf q}|\ll k_{\rm F}$) and incorporate inelastic electron--electron scattering besides elastic impurity scattering. Moreover we generalize the Lindhard density response function to the Raman case. Numerical results for the quasiparticle scattering rate and the Raman response function for cuprate superconductors are presented.Comment: 5 pages, 4figures. accepted in PRB (Brief Report), in pres

Collective Spin Fluctuation Mode and Raman Scattering in Superconducting Cuprates

Although the low frequency electronic Raman response in the superconducting state of the cuprates can be largely understood in terms of a d-wave energy gap, a long standing problem has been an explanation for the spectra observed in the $A_{1g}$ polarization orientations. We present calculations which suggest that the peak position of the observed $A_{1g}$ spectra is due to a collective spin fluctuation mode.Comment: 4 pages, 5 eps figure

Raman Scattering in Cuprate Superconductors

A theory for electronic Raman scattering in the cuprate superconductors is presented with a specific emphasis on the polarization dependence of the spectra which can infer the symmetry of the energy gap. Signatures of the effects of disorder on the low frequency and low temperature behavior of the Raman spectra for different symmetry channels provide detailed information about the magnitude and the phase of the energy gap. Properties of the theory for finite T are discussed and compared to recent data concerning the doping dependence of the Raman spectra in cuprate superconductors, and remaining questions are addressed.Comment: 27 pages, 11 figures, style file include

Two Distinct Electronic Contributions in the Fully Symmetric Raman Response of High TcT_{c} Cuprates

We show by non resonant effect in HgBa$_2$CuO$_{4+\delta}$ (Hg-1201)and by Zn substitutions in YBa$_2$Cu$_3$O$_{7-\delta}$ (Y-123) compounds that the fully symmetric Raman spectrum has two distinct electronic contributions. The A$_{1g}$ response consists in the superconducting pair breaking peak at the 2$\Delta$ energy and a collective mode close to the magnetic resonance energy. These experimental results reconcile the \textit{d-wave} model to the A$_{1g}$ Raman response function in so far as a collective mode that is distinct from the pair breaking peak is present in the A$_{1g}$ channel.Comment: 4 pages, 2 figure