Variations in aerosol optical and microphysical properties during an Indian festival observed with space-borne and ground-based observations

This study analyzes changes in the response of meteorological parameters, aerosol, ozone, and water vapor properties over a tropical urban station in Pune, India, using ground-based and satellite data sets from February 23 to March 4, 2010 covering the Holi festival period. Continuous ground-based measurements of Microprocessor-based Total Ozone Portable Spectrometer (Microtops II) were made. The variations in aerosol optical depth (AOD) showed higher values on March 1, 2010 which coincide with the peak festival time. Using the least squares method, A °ngström exponent (α) is calculated in the spectral interval of 340-1020 nm, along with the coefficient a2 of the second-order polynomial fit to the plot of log AOD versus the log wavelength. The correlation between the coefficient a2 vs. AOD 500 nm is discussed. Results from ground-based Microtops and CIMEL sun-sky radiometer observations are also found to match well with satellite retrievals. The aerosol index (AI) derived from the Ozone Monitoring Instrument (OMI) along with AOD derived from the Moderate-Resolution Imaging Spectrometer (MODIS) indicate positive correlation. This suggests that satellite observations over the region confirm the presence of absorbing aerosols mainly due to bio-mass burning and colored powder spray activities during the festival

Atmospheric stability effects on aerosol structure and stratification

This paper essentially addresses the structure and stratification of the nocturnal boundary layer (NBL) derived from the vertical profile measurements of aerosol concentration made with a computer-controlled Argon ion lidar system at the Indian Institue of Tropical Meteorology (IITM), Pune, India. Companions are made between the lidar observations during clear night-sky conditions and concurrent aerometric observations carried out on some selected experimental days. The results show multiple stratified aerosol layer structures in the nocturnal lower atmosphere, which drift either upward or downward depending on atmospheric stability conditions prevailing at different altitudes. The normalized aerosol concentration gradient (NCG) profiles indicate the variations in the nocturnal mixing depth from 200 to 426 m and that in the stable layer height from 325 to 725 m during the period of observations. The importance of such observations in the context of monitoring and/or assesment of airborne particulate pollutants over the urban environments associated with non-uniform terrain is discussed

A study of lightning activity over land and oceanic regions of India

Monthly variations of lightning activity over typical land and oceanic regions of India were examined using satellite data (OTD) for a 5-year period (1995-1999). It is noted that the nature of variation between surface air maximum temperature (Tmax), thunderstorm days (Thn), and lightning flash count over ER and WR showed remarkable correspondence and sensitivity with each other on monthly time scale. As we move out of winter season and enter the monsoon season, via pre-monsoon season, the WR undergoes cooling relative to the ER in the range 0.1-1.2°C. As a result, WR experiences reduction of thunder days and lowering in flash count. This decrease in Tmax, Thn, and flash count over WR may also be associated with relatively small values of Tθw and CAPE in comparison with similar values over ER during the monsoon season. Our observation of associated reduction in Thn and lightning count per 1°C cooling in surface air maximum temperature suggests reduction of ~3.5 thunderstorms per station and 73 flashes. Comparison of lightning flashes between pairs of coastal, oceanic, arid-zone, hilly, and island stations reveals distinct relationship between climate regime and intensity of lightning activity. We may conclude the results of this study by saying that the overhead lightning activity is a clear reflection of the status of the underlying ground-earth properties. A close and continuous monitoring of lightning activity may be considered as a need of present day scientific studies

Winter aerosol and trace gas characteristics over a high-altitude station in the Western Ghats, India

This paper presents spectral distribution of aerosol optical depth (and derived size distribution), water vapor and ozone in total atmospheric column; in conjunction with particulate mass concentration in the size range from 0.3 to 20 μm and black carbon mass concentration at the surface-level during four different campaigns, conducted in months of December-January-2006-2007 (Campaign I), February-2007 (Campaign II), January-2008 (Campaign III) and November-2008 (Campaign IV) at a high-altitude station, Sinhgad (18°22'N, 73°45'E, 1450 m AMSL) in the Western Ghats of Indian Peninsula. Aerosol optical depth (AOD) measured within the spectral range 440-1020 nm is found lower as compared to that measured over a nearby urban station, Pune; but relatively higher than that over other remote high-altitude stations in India. The columnar Angstrom exponent derived within the 440-870 nm spectral range showed maximum values close to 1 indicating relatively higher contribution from fine-mode particles to aerosol size spectrum. Interestingly, this parameter shows lower values when the total aerosol mass concentration exhibits higher values during afternoon hours. Both columnar water vapor (CWV) and ozone (TCO) exhibit lower values in the morning hours and higher in the afternoon hours. The mass concentration of black carbon shows an association with AOD during the study period over the station. The measured surface aerosol particle number concentrations are used to reconstruct AOD spectra using the Optical Properties of Aerosols and Clouds (OPAC) software package and compared with simultaneously available columnar AOD spectra

Recent trends in aerosol climatology and air pollution as inferred from multi-year lidar observations over a tropical urban station

Regular nighttime monitoring of aerosol and other atmospheric parameters was initiated in 1985 at the Indian Institute of Tropical Meteorology, Pune. This is a tropical urban station (18°32'N, 73°51'E, 559 m AMSL), situated approximately 100 km inland from the west coast of India. The multi-year aerosol vertical profile database, utilized in the present study, consisted of more than 1200 vertical aerosol concentration profiles. These data were collected with a computer-controlled, bistatic, argon-ion lidar system over a 12 year period from October 1986 to September 1998 and have been utilized to study the morphology of the nighttime atmospheric boundary layer and associated air quality. The recent climatological trend in the aerosol loading at the experimental station has also been studied. The study reveals higher pollution potential during late evenings in the winter and a total increase of about 3 in the aerosol loading over the 12 year observational period. This increase can be attributed partly due to the urban heat island effect and due to growing urbanization and industrialization, as well as to the land-usage patterns in proximity to the experimental station. Further, it has been found that the long-term trend in aerosol loading was not uniform, but it changed from year to year depending on meteorological parameters (precipitation, in particular) and local anthropogenic activities. The short-term variations in aerosol loading and their relationship with concurrent meteorological parameters over the observational site are discussed also

Aerosol optical depth, ozone and water vapor measurements over Gadanki, a tropical station in peninsular India

This paper reports the results of a study related to the optical and physical characteristics of columnar aerosols and variation in total column ozone (TCO) and precipitable water content (PWC) over Gadanki (13.45°N, 79.18°E), a tropical station in peninsular India, for the first time, using MICROTOPS-II (Microprocessor-based Total Ozone Portable Spectrometer), comprising of both sun photometer and ozonometer. Results show wavelength dependence of AOD, having mean value of �0.4 (± 0.09) at 500 nm optical channel. Daily mean aerosol size spectra shows, most of the time, power-law distribution. However, its diurnal variations show significant changes in aerosol size spectra modulated by a combination of both power-law and bi-modal distributions. To characterize AOD, the Angstrom parameters (i.e., a and β) were used. The day-to-day variations in TCO were found to be in fair agreement with that derived from TOMS satellite data for all the experimental days, having mean observed value of ~253 (± 8) DU over the station. Interestingly, an inverse relationship between TCO and AOD or PWC was observed over the station, on some times of the day, which could be attributed to the mixing of significant fraction of ozone with aerosol and water vapor-rich air mass. However, a significant positive correlation was observed between AOD and PWC

Relationship between lidar-based observations of aerosol content and monsoon precipitation over a tropical station, Pune, India

This paper reports the results of the aerosol lidar experiments that have been performed at the Indian Institute of Tropical Meteorology (IITM), Pune (18.54°N, 73.85°E, 559 m amsl), a tropical station in India. The lidar-observed cloud macro-physical parameters (cloud-base and cloud-ceiling heights, vertical thickness, etc.) and polarisation characteristics and their association with surface-generated aerosols at the experimental site are presented and discussed. The correspondence among the lidar-derived aerosol distributions, meteorological parameters and south-west (SW) monsoon (June-September) activity over Pune during 12 successive SW monsoon seasons (1987-98) including two pairs of contrasting seasons of 1987-8 and 1993-4 is also examined. The results indicate an association between variations in aerosol loading in the boundary layer during the pre-monsoon season (March-May) and precipitation intensity during the ensuing monsoon season. Moreover, the decrease in aerosol content from pre-monsoon to monsoon season is found to follow the SW monsoon season total precipitation. Thus the results suggest that (i) the IITM lidar can also be a useful remote sensor for aerosol characterisation studies from polarisation measurements, and some important physical properties of clouds in the lower atmosphere over the station, and (ii) there exists a correspondence between boundary-layer aerosol content and SW monsoon precipitation over Pune, which is explained in terms of the type of aerosols and the environmental and meteorological processes, particularly during premonsoon and monsoon months prevailing over the experimental station