Absence of ferromagnetism in Mn- and Co-doped ZnO

Following the theoretical predictions of ferromagnetism in Mn- and Co-doped ZnO, several workers reported ferromagnetism in thin films as well as in bulk samples of these materials. While some observe room-temperature ferromagnetism, others find magnetization at low temperatures. Some of the reports, however, cast considerable doubt on the magnetism of Mn- and Co-doped ZnO. In order to conclusively establish the properties of Mn- and Co-doped ZnO, samples with 6 percent and 2 percent dopant concentrations, have been prepared by the low-temperature decomposition of acetate solid solutions. The samples have been characterized by x-ray diffraction, EDAX and spectroscopic methods to ensure that the dopants are substitutional. All the Mn- and Co-doped ZnO samples (prepared at 400 deg C and 500 deg C) fail to show ferromagnetism. Instead, their magnetic properties are best described by a Curie-Weiss type behavior. It appears unlikely that these materials would be useful for spintronics, unless additional carriers are introduced by some means.Comment: 23 pages, 9 figures. submitted to J. Mater. Chem 200

Semientwining Structures and Their Applications

Semientwining structures are proposed as concepts simpler than entwining structures, yet they are shown to have interesting applications in constructing intertwining operators and braided algebras, lifting functors, finding solutions for Yang-Baxter systems, and so forth. While for entwining structures one can associate corings, for semientwining structures one can associate comodule algebra structures where the algebra involved is a bialgebra satisfying certain properties. Remove selecte

Bethe approximation for a system of hard rigid rods: the random locally tree-like layered lattice

We study the Bethe approximation for a system of long rigid rods of fixed length k, with only excluded volume interaction. For large enough k, this system undergoes an isotropic-nematic phase transition as a function of density of the rods. The Bethe lattice, which is conventionally used to derive the self-consistent equations in the Bethe approximation, is not suitable for studying the hard-rods system, as it does not allow a dense packing of rods. We define a new lattice, called the random locally tree-like layered lattice, which allows a dense packing of rods, and for which the approximation is exact. We find that for a 4-coordinated lattice, k-mers with k>=4 undergo a continuous phase transition. For even coordination number q>=6, the transition exists only for k >= k_{min}(q), and is first order.Comment: 10 pages, 10 figure

Distribution of sizes of erased loops for loop-erased random walks

We study the distribution of sizes of erased loops for loop-erased random walks on regular and fractal lattices. We show that for arbitrary graphs the probability $P(l)$ of generating a loop of perimeter $l$ is expressible in terms of the probability $P_{st}(l)$ of forming a loop of perimeter $l$ when a bond is added to a random spanning tree on the same graph by the simple relation $P(l)=P_{st}(l)/l$. On $d$-dimensional hypercubical lattices, $P(l)$ varies as $l^{-\sigma}$ for large $l$, where $\sigma=1+2/z$ for $1<d<4$, where z is the fractal dimension of the loop-erased walks on the graph. On recursively constructed fractals with $\tilde{d} < 2$ this relation is modified to $\sigma=1+2\bar{d}/{(\tilde{d}z)}$, where $\bar{d}$ is the hausdorff and $\tilde{d}$ is the spectral dimension of the fractal.Comment: 4 pages, RevTex, 3 figure

Exact entropy of dimer coverings for a class of lattices in three or more dimensions

We construct a class of lattices in three and higher dimensions for which the number of dimer coverings can be determined exactly using elementary arguments. These lattices are a generalization of the two-dimensional kagome lattice, and the method also works for graphs without translational symmetry. The partition function for dimer coverings on these lattices can be determined also for a class of assignments of different activities to different edges.Comment: 4 pages, 2 figures; added results on partition function when different edges have different weights; modified abstract; added reference