1,416 research outputs found
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A neutronic feasibility study for LEU conversion of the IR-8 research reactor.
Equilibrium fuel cycle comparisons for the IR-8 research reactor were made for HEU(90%), HEU(36%), and LEU (19.75%) fuel assembly (FA) designs using three dimensional multi-group diffusion theory models benchmarked to detailed Monte Carlo models of the reactor. Comparisons were made of changes in reactivity, cycle length, average {sup 235}U discharge burnup, thermal neutron flux, and control rod worths for the 90% and 36% enriched IRT-3M fuel assembly and the 19.75% enriched IRT-4M fuel assembly with the same fuel management strategy. The results of these comparisons showed that a uranium density of 3.5 g/cm{sup 3} in the fuel meat would be required in the LEU IRT-4M fuel assembly to match the cycle length of the HEU(90%) IRT-3M FA and an LEU density of 3.7 g/cm{sup 3} is needed to match the cycle length of the HEU(36%) IRT-3M FA
Formation of Nanopillar Arrays in Ultrathin Viscous Films: The Critical Role of Thermocapillary Stresses
Experiments by several groups during the past decade have shown that a molten
polymer nanofilm subject to a large transverse thermal gradient undergoes
spontaneous formation of periodic nanopillar arrays. The prevailing explanation
is that coherent reflections of acoustic phonons within the film cause a
periodic modulation of the radiation pressure which enhances pillar growth. By
exploring a deformational instability of particular relevance to nanofilms, we
demonstrate that thermocapillary forces play a crucial role in the formation
process. Analytic and numerical predictions show good agreement with the pillar
spacings obtained in experiment. Simulations of the interface equation further
determine the rate of pillar growth of importance to technological
applications.Comment: 5 pages, 4 figure
Pair Correlations, Short Range Order and Dispersive Excitations in the Quasi-Kagome Quantum Magnet Volborthite
We present spatial and dynamic information on the s=1/2 distorted kagome
antiferromagnet volborthite, Cu3V2O7(OD)2.2D2O, obtained by polarized and
inelastic neutron scattering. The instantaneous structure factor, S(Q), is
dominated by nearest neighbor pair correlations, with short range order at wave
vectors Q1=0.65(3) {\AA}^-1 and Q2=1.15(5) {\AA}^-1 emerging below 5 K. The
excitation spectrum, S(Q,{\omega}), reveals two steep branches dispersing from
Q1 and Q2, and a flat mode at {\omega}=5.0(2) meV. The results allow us to
identify the cross-over at T*=1 K in 51V NMR and specific heat measurements as
the build-up of correlations at Q_1. We compare our data to theoretical models
proposed for volborthite, and demonstrate that the excitation spectrum can be
explained by spin-wave-like excitations with anisotropic exchange parameters,
as also suggested by recent local density calculations.Comment: Rewritten article resubmitted to Phys. Rev. Lett. 021
Nonlinear Dynamics of Capacitive Charging and Desalination by Porous Electrodes
The rapid and efficient exchange of ions between porous electrodes and
aqueous solutions is important in many applications, such as electrical energy
storage by super-capacitors, water desalination and purification by capacitive
deionization (or desalination), and capacitive extraction of renewable energy
from a salinity difference. Here, we present a unified mean-field theory for
capacitive charging and desalination by ideally polarizable porous electrodes
(without Faradaic reactions or specific adsorption of ions) in the limit of
thin double layers (compared to typical pore dimensions). We illustrate the
theory in the case of a dilute, symmetric, binary electrolyte using the
Gouy-Chapman-Stern (GCS) model of the double layer, for which simple formulae
are available for salt adsorption and capacitive charging of the diffuse part
of the double layer. We solve the full GCS mean-field theory numerically for
realistic parameters in capacitive deionization, and we derive reduced models
for two limiting regimes with different time scales: (i) In the
"super-capacitor regime" of small voltages and/or early times where the porous
electrode acts like a transmission line, governed by a linear diffusion
equation for the electrostatic potential, scaled to the RC time of a single
pore. (ii) In the "desalination regime" of large voltages and long times, the
porous electrode slowly adsorbs neutral salt, governed by coupled, nonlinear
diffusion equations for the pore-averaged potential and salt concentration
Experimental Proof of a Magnetic Coulomb Phase
Spin ice materials are magnetic substances in which the spin directions map
onto hydrogen positions in water ice. Recently this analogy has been elevated
to an electromagnetic equivalence, indicating that the spin ice state is a
Coulomb phase, with magnetic monopole excitations analogous to ice's mobile
ionic defects. No Coulomb phase has yet been proved in a real magnetic
material, as the key experimental signature is difficult to resolve in most
systems. Here we measure the scattering of polarised neutrons from the
prototypical spin ice Ho2Ti2O7. This enables us to separate different
contributions to the magnetic correlations to clearly demonstrate the existence
of an almost perfect Coulomb phase in this material. The temperature dependence
of the scattering is consistent with the existence of deconfined magnetic
monopoles connected by Dirac strings of divergent length.Comment: 18 pages, 4 fig
Artesunate reduces but does not prevent posttreatment transmission of Plasmodium falciparum to Anopheles gambiae.
Combination therapy that includes artemisinin derivatives cures most falciparum malaria infections. Lowering transmission by reducing gametocyte infectivity would be an additional benefit. To examine the effect of such therapy on transmission, Gambian children with Plasmodium falciparum malaria were treated with standard regimens of chloroquine or pyrimethamine-sulfadoxine alone or in combination with 1 or 3 doses of artesunate. The infectivity to mosquitoes of gametocytes in peripheral blood was determined 4 or 7 days after treatment. Infection of mosquitoes was observed in all treatment groups and was positively associated with gametocyte density. The probability of transmission was lowest in those who received pyrimethamine-sulfadoxine and 3 doses of artesunate, and it was 8-fold higher in the group that received pyrimethamine-sulfadoxine alone. Artesunate reduced posttreatment infectivity dramatically but did not abolish it completely. The study raises questions about any policy to use pyrimethamine-sulfadoxine alone as the first-line treatment for malaria
Spin correlations in Ca3Co2O6: A polarised-neutron diffraction and Monte Carlo study
We present polarised-neutron diffraction measurements of the Ising-like
spin-chain compound Ca3Co2O6 above and below the magnetic ordering temperature
TN. Below TN, a clear evolution from a single-phase spin-density wave (SDW)
structure to a mixture of SDW and commensurate antiferromagnet (CAFM)
structures is observed on cooling. For a rapidly-cooled sample, the majority
phase at low temperature is the SDW, while if the cooling is performed
sufficiently slowly, then the SDW and the CAFM structure coexist between 1.5
and 10 K. Above TN, we use Monte Carlo methods to analyse the magnetic diffuse
scattering data. We show that both intra- and inter-chain correlations persist
above TN, but are essentially decoupled. Intra-chain correlations resemble the
ferromagnetic Ising model, while inter-chain correlations resemble the
frustrated triangular-lattice antiferromagnet. Using previously-published bulk
property measurements and our neutron diffraction data, we obtain values of the
ferromagnetic and antiferromagnetic exchange interactions and the single-ion
anisotropy.Comment: 10 pages, 7 figure
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Greek research reactor performance characteristics after addition of beryllium reflector and LEU fuel
The GRR-1 is a 5-MW pool-type, light-water-moderated and-cooled reactor fueled with MTR-type fuel elements. Recently received Be reflector blocks will soon be added to the core to add additional reactivity until fresh LEU fuel arrives. REBUS-3 xy fuel cycle analyses, using burnup dependent cross sections, were performed to assist in fuel management decisions for the water- and Be-reflected HEU nonequilibrium cores. Cross sections generated by EPRI-CELL have been benchmarked to identical VIM Monte Carlo models. The size of the Be-reflected LEU core has been reduced to 30 elements compared to 35 for the HEU water-reflected core, and an equilibrium cycle calculation has been performed
Spin correlations and exchange in square lattice frustrated ferromagnets
The J1-J2 model on a square lattice exhibits a rich variety of different
forms of magnetic order that depend sensitively on the ratio of exchange
constants J2/J1. We use bulk magnetometry and polarized neutron scattering to
determine J1 and J2 unambiguously for two materials in a new family of vanadium
phosphates, Pb2VO(PO4)2 and SrZnVO(PO4)2, and we find that they have
ferromagnetic J1. The ordered moment in the collinear antiferromagnetic ground
state is reduced, and the diffuse magnetic scattering is enhanced, as the
predicted bond-nematic region of the phase diagram is approached.Comment: 4 pages, 4 figure
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