Electronic structure of heavily electron-doped BaFe1.7_{1.7}Co0.3_{0.3}As2_2 studied by angle-resolved photoemission

We have performed high-resolution angle-resolved photoemission spectroscopy on heavily electron-doped non-superconducting (SC) BaFe$_{1.7}$Co$_{0.3}$As$_2$. We find that the two hole Fermi surface pockets at the zone center observed in the hole-doped superconducting Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ are absent or very small in this compound, while the two electron pockets at the M point significantly expand due to electron doping by the Co substitution. Comparison of the Fermi surface between non-SC and SC samples indicates that the coexistence of hole and electron pockets connected via the antiferromagnetic wave vector is essential in realizing the mechanism of superconductivity in the iron-based superconductors.Comment: 5 pages, 4 figure

An Intra-pulse feedforward algorithm for improving pulsed microwave stability

During the pulsed operation of the linear accelerator in DCLS (Dalian Coherent Light Source), we found a strong correlation between the klystron modulator's high voltage and the klystron output microwave, with noticeable jitter among adjacent microwaves. Therefore, we propose an intra-pulse feedforward algorithm and implement it in LLRF (Low-Level Radiofrequency) systems. This algorithm assumes that the transfer model of the microwave system is linear within a small range of work points and measures the transfer coefficient of the microwave between the LLRF and klystron. For each pulsed microwave of the klystron output, the LLRF system first calculates the vector deviation between the initial measurement within its pulse and the target. The deviation will be compensated in the LLRF excitation so that the jitter in the later part of the pulsed microwave is suppressed. Experiments have shown that this algorithm can effectively suppress the jitter among adjacent microwaves, e.g., improving the amplitude and phase stability (RMS) from 0.11%/0.2{\deg} to 0.1%/0.05{\deg}. This algorithm can also be applied to other accelerators operating in pulsed modes.Comment: Talk presented at LLRF Workshop 2023 (LLRF2023, arXiv: 2310.03199

The microwave amplitude and phase setting based on event timing for the DCLS

The primary accelerator of DCLS (Dalian Coherent Light Source) operates at a repetition rate of 20 Hz now, and the beam is divided at the end of the linear accelera-tor through Kicker to make two 10 Hz beamlines work simultaneously. For the simultaneous emission FEL of two beamlines, the beam energy of the two beamlines is required to be controlled independently, so we need to set the amplitude and phase of each beamline. This paper implements a microwave amplitude and phase setting function based on event timing. We upgraded the EVG/EVR event timing system and LLRF (Low-Level Radiofrequency) system. Two special event codes and a repetition rate division of 10 Hz are added to the event timing system, and we can set the microwave amplitude and phase by judging the event code in LLRF. We ulti-mately perform the microwave triggering at a repetition rate of 10 Hz for each beamline and validate this function through beam experiments.Comment: Poster presented at LLRF Workshop 2023 (LLRF2023, arXiv: 2310.03199

Implementation of microwave with arbitrary amplitude and phase for the DCLS

In many experiments, the simultaneous emission of multiple wavelengths of FEL (Free-Electron Laser) is significant. For the pulsed-mode FEL facility, we must accelerate multiple electron beams in one microwave pulse, and they may be in different amplitudes and phases in the acceleration field. Therefore, we implement a microwave excitation, whose amplitude and phase have arbitrary shapes in the LLRF (Low-Level Radiofrequency) system. We generate a microwave pulse with step-shaped amplitude and phase for dual beam operation in DCLS (Dalian Coherent Light Source). The microwave system of the primary accelerator has four pulsed LLRF devices, which output excitation to drive four solid-state amplifiers and then excite two 50 MW and two 80 MW klystrons, respectively. Preliminary experiments have shown that this step-shaped microwave can be used for the DCLS twin-bunch operation.Comment: Poster presented at LLRF Workshop 2023 (LLRF2023, arXiv: 2310.03199

Cationic vacancy induced room-temperature ferromagnetism in transparent conducting anatase Ti_{1-x}Ta_xO_2 (x~0.05) thin films

We report room-temperature ferromagnetism in highly conducting transparent anatase Ti1-xTaxO2 (x~0.05) thin films grown by pulsed laser deposition on LaAlO3 substrates. Rutherford backscattering spectrometry (RBS), x-ray diffraction (XRD), proton induced x-ray emission (PIXE), x-ray absorption spectroscopy (XAS) and time-of-flight secondary ion mass spectrometry (TOF-SIMS) indicated negligible magnetic contaminants in the films. The presence of ferromagnetism with concomitant large carrier densities was determined by a combination of superconducting quantum interference device (SQUID) magnetometry, electrical transport measurements, soft x-ray magnetic circular dichroism (SXMCD), XAS, and optical magnetic circular dichroism (OMCD) and was supported by first-principle calculations. SXMCD and XAS measurements revealed a 90% contribution to ferromagnetism from the Ti ions and a 10% contribution from the O ions. RBS/channelling measurements show complete Ta substitution in the Ti sites though carrier activation was only 50% at 5% Ta concentration implying compensation by cationic defects. The role of Ti vacancy and Ti3+ was studied via XAS and x-ray photoemission spectroscopy (XPS) respectively. It was found that in films with strong ferromagnetism, the Ti vacancy signal was strong while Ti3+ signal was absent. We propose (in the absence of any obvious exchange mechanisms) that the localised magnetic moments, Ti vacancy sites, are ferromagnetically ordered by itinerant carriers. Cationic-defect-induced magnetism is an alternative route to ferromagnetism in wide-band-gap semiconducting oxides without any magnetic elements.Comment: 21 pages, 10 figures, to appear in Philosophical Transaction - Royal Soc.

Competitions of magnetism and superconductivity in FeAs-based materials

Using the numerical unrestricted Hartree-Fock approach, we study the ground state of a two-orbital model describing newly discovered FeAs-based superconductors. We observe the competition of a $(0, \pi)$ mode spin-density wave and the superconductivity as the doping concentration changes. There might be a small region in the electron-doping side where the magnetism and superconductivity coexist. The superconducting pairing is found to be spin singlet, orbital even, and mixed s$_{xy}$ + d$_{x^{2}-y^{2}}$ wave (even parity).Comment: 5 pages, 3 figure

Ultrahigh Surface Area Three-Dimensional Porous Graphitic Carbon from Conjugated Polymeric Molecular Framework

Porous graphitic carbon is essential for many applications such as energy storage devices, catalysts, and sorbents. However, current graphitic carbons are limited by low conductivity, low surface area, and ineffective pore structure. Here we report a scalable synthesis of porous graphitic carbons using a conjugated polymeric molecular framework as precursor. The multivalent cross-linker and rigid conjugated framework help to maintain micro- and mesoporous structures, while promoting graphitization during carbonization and chemical activation. The above unique design results in a class of highly graphitic carbons at temperature as low as 800 ??C with record-high surface area (4073 m2 g-1), large pore volume (2.26 cm-3), and hierarchical pore architecture. Such carbons simultaneously exhibit electrical conductivity >3 times more than activated carbons, very high electrochemical activity at high mass loading, and high stability, as demonstrated by supercapacitors and lithium-sulfur batteries with excellent performance. Moreover, the synthesis can be readily tuned to make a broad range of graphitic carbons with desired structures and compositions for many applications.clos

Spin-Gap Proximity Effect Mechanism of High Temperature Superconductivity

When holes are doped into an antiferromagnetic insulator they form a slowly fluctuating array of ``topological defects'' (metallic stripes) in which the motion of the holes exhibits a self-organized quasi one-dimensional electronic character. The accompanying lateral confinement of the intervening Mott-insulating regions induces a spin gap or pseudogap in the environment of the stripes. We present a theory of underdoped high temperature superconductors and show that there is a {\it local} separation of spin and charge, and that the mobile holes on an individual stripe acquire a spin gap via pair hopping between the stripe and its environment; i.e. via a magnetic analog of the usual superconducting proximity effect. In this way a high pairing scale without a large mass renormalization is established despite the strong Coulomb repulsion between the holes. Thus the {\it mechanism} of pairing is the generation of a spin gap in spatially-confined {\it Mott-insulating} regions of the material in the proximity of the metallic stripes. At non-vanishing stripe densities, Josephson coupling between stripes produces a dimensional crossover to a state with long-range superconducting phase coherence. This picture is established by obtaining exact and well-controlled approximate solutions of a model of a one-dimensional electron gas in an active environment. An extended discussion of the experimental evidence supporting the relevance of these results to the cuprate superconductors is given.Comment: 30 pages, 2 figure

Observation of ηc→ωω\eta_c\to\omega\omega in J/ψ→γωωJ/\psi\to\gamma\omega\omega

Using a sample of $(1310.6\pm7.0)\times10^6$ $J/\psi$ events recorded with the BESIII detector at the symmetric electron positron collider BEPCII, we report the observation of the decay of the $(1^1 S_0)$ charmonium state $\eta_c$ into a pair of $\omega$ mesons in the process $J/\psi\to\gamma\omega\omega$. The branching fraction is measured for the first time to be $\mathcal{B}(\eta_c\to\omega\omega)= (2.88\pm0.10\pm0.46\pm0.68)\times10^{-3}$, where the first uncertainty is statistical, the second systematic and the third is from the uncertainty of $\mathcal{B}(J/\psi\to\gamma\eta_c)$. The mass and width of the $\eta_c$ are determined as $M=(2985.9\pm0.7\pm2.1)\,$MeV/$c^2$ and $\Gamma=(33.8\pm1.6\pm4.1)\,$MeV.Comment: 13 pages, 6 figure

Measurement of proton electromagnetic form factors in e+e−→ppˉe^+e^- \to p\bar{p} in the energy region 2.00-3.08 GeV

The process of $e^+e^- \rightarrow p\bar{p}$ is studied at 22 center-of-mass energy points ($\sqrt{s}$) from 2.00 to 3.08 GeV, exploiting 688.5~pb$^{-1}$ of data collected with the BESIII detector operating at the BEPCII collider. The Born cross section~($\sigma_{p\bar{p}}$) of $e^+e^- \rightarrow p\bar{p}$ is measured with the energy-scan technique and it is found to be consistent with previously published data, but with much improved accuracy. In addition, the electromagnetic form-factor ratio ($|G_{E}/G_{M}|$) and the value of the effective ($|G_{\rm{eff}}|$), electric ($|G_E|$) and magnetic ($|G_M|$) form factors are measured by studying the helicity angle of the proton at 16 center-of-mass energy points. $|G_{E}/G_{M}|$ and $|G_M|$ are determined with high accuracy, providing uncertainties comparable to data in the space-like region, and $|G_E|$ is measured for the first time. We reach unprecedented accuracy, and precision results in the time-like region provide information to improve our understanding of the proton inner structure and to test theoretical models which depend on non-perturbative Quantum Chromodynamics