41 research outputs found
Asymptotic Capture-Number and Island-Size Distributions for One-Dimensional Irreversible Submonolayer Growth
Using a set of evolution equations [J.G. Amar {\it et al}, Phys. Rev. Lett.
{\bf 86}, 3092 (2001)] for the average gap-size between islands, we calculate
analytically the asymptotic scaled capture-number distribution (CND) for
one-dimensional irreversible submonolayer growth of point islands. The
predicted asymptotic CND is in reasonably good agreement with kinetic
Monte-Carlo (KMC) results and leads to a \textit{non-divergent asymptotic}
scaled island-size distribution (ISD). We then show that a slight modification
of our analytical form leads to an analytic expression for the asymptotic CND
and a resulting asymptotic ISD which are in excellent agreement with KMC
simulations. We also show that in the asymptotic limit the self-averaging
property of the capture zones holds exactly while the asymptotic scaled gap
distribution is equal to the scaled CND.Comment: 4 pages, 1 figure, submitted to Phys. Rev.
A Note on Flux Induced Superpotentials in String Theory
Non-vanishing fluxes in M-theory and string theory compactifications induce a
superpotential in the lower dimensional theory. Gukov has conjectured the
explicit form of this superpotential. We check this conjecture for the
heterotic string compactified on a Calabi-Yau three-fold as well as for warped
M-theory compactifications on Spin(7) holonomy manifolds, by performing a
Kaluza-Klein reduction.Comment: 19 pages, no figure
Scope for new applications for gold arising from the electrocatalytic behaviour of its metastable surface states
Phase Behavior of Aqueous Na-K-Mg-Ca-CI-NO3 Mixtures: Isopiestic Measurements and Thermodynamic Modeling
A comprehensive model has been established for calculating thermodynamic properties of multicomponent aqueous systems containing the Na{sup +}, K{sup +}, Mg{sup 2+}, Ca{sup 2+}, Cl{sup -}, and NO{sub 3}{sup -} ions. The thermodynamic framework is based on a previously developed model for mixed-solvent electrolyte solutions. The framework has been designed to reproduce the properties of salt solutions at temperatures ranging from the freezing point to 300 C and concentrations ranging from infinite dilution to the fused salt limit. The model has been parameterized using a combination of an extensive literature database and new isopiestic measurements for thirteen salt mixtures at 140 C. The measurements have been performed using Oak Ridge National Laboratory's (ORNL) previously designed gravimetric isopiestic apparatus, which makes it possible to detect solid phase precipitation. Water activities are reported for mixtures with a fixed ratio of salts as a function of the total apparent salt mole fraction. The isopiestic measurements reported here simultaneously reflect two fundamental properties of the system, i.e., the activity of water as a function of solution concentration and the occurrence of solid-liquid transitions. The thermodynamic model accurately reproduces the new isopiestic data as well as literature data for binary, ternary and higher-order subsystems. Because of its high accuracy in calculating vapor-liquid and solid-liquid equilibria, the model is suitable for studying deliquescence behavior of multicomponent salt systems
A century of trends in adult human height
Being taller is associated with enhanced longevity, and higher education and earnings. We reanalysed 1472 population-based studies, with measurement of height on more than 18.6 million participants to estimate mean height for people born between 1896 and 1996 in 200 countries. The largest gain in adult height over the past century has occurred in South Korean women and Iranian men, who became 20.2 cm (95% credible interval 17.5-22.7) and 16.5 cm (13.3-19.7) taller, respectively. In contrast, there was little change in adult height in some sub-Saharan African countries and in South Asia over the century of analysis. The tallest people over these 100 years are men born in the Netherlands in the last quarter of 20th century, whose average heights surpassed 182.5 cm, and the shortest were women born in Guatemala in 1896 (140.3 cm; 135.8-144.8). The height differential between the tallest and shortest populations was 19-20 cm a century ago, and has remained the same for women and increased for men a century later despite substantial changes in the ranking of countries
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Evaluation of ground freezing for environmental restoration at waste area grouping 5, Oak Ridge National Laboratory, Oak Ridge, Tennessee
A study to evaluate the feasibility of using ground freezing technology to immobilize tritium contaminants was performed as part of the Waste Area Grouping (WAG) 6 Technology Demonstrations initiated by the WAG 6 Record of Agreement. The study included a review of ground freezing technology, evaluation of this technology for environmental restoration, and identification of key technical issues. A proposed ground freezing demonstration for containment of tritium at a candidate Oak Ridge National Laboratory site was developed. The planning requirements for the demonstration were organized into seven tasks including site selection, site characterization, conceptual design, laboratory evaluation, demonstration design, field implementation, and monitoring design. A brief discussion of each of these tasks is provided. Additional effort beyond the scope of this study is currently being directed to the selection of a demonstration site and the identification of funding
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Mercury removal from solid mixed waste
The removal of mercury from mixed wastes is an essential step in eliminating the temporary storage of large inventories of mixed waste throughout the Department of Energy (DOE) complex. Currently thermal treatment has been identified as a baseline technology and is being developed as part of the DOE Mixed Waste Integrated Program (MWIP). Since thermal treatment will not be applicable to all mercury containing mixed waste and the removal of mercury prior to thermal treatment may be desirable, laboratory studies have been initiated at Oak Ridge National Laboratory (ORNL) to develop alternative remediation technologies capable of removing mercury from certain mixed waste. This paper describes laboratory investigations of the KI/I{sub 2} leaching processes to determine the applicability of this process to mercury containing solid mixed waste
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Removal of mercury from solids using the potassium iodide/iodine leaching process
Potassium iodide (KI) and iodine (I{sub 2}) leaching solutions have been evaluated for use in a process for removing mercury from contaminated mixed waste solids. Most of the experimental work was completed using surrogate waste. During the last quarter of fiscal year 1995, this process was evaluated using an actual mixed waste (storm sewer sediment from the Oak Ridge Y-12 Site). The mercury content of the storm sewer sediment was measured and determined to be approximately 35,000 mg/kg. A solution consisting of 0.2 M I{sub 2} and 0.4 M KI proved to be the most effective leachant used in the experiments when applied for 2 to 4 h at ambient temperature. Over 98% of the mercury was removed from the storm sewer sediment using this solution. Iodine recovery and recycle of the leaching agent were also accomplished successfully. Mathematical model was used to predict the amount of secondary waste in the process. Both surrogate waste and actual waste were used to study the fate of radionuclides (uranium) in the leaching process