Distortion of Wigner molecules : pair function approach

We considered a two dimensional three electron quantum dot in a magnetic field in the Wigner limit. A unitary coordinate transformation decouples the Hamiltonian (with Coulomb interaction between the electrons included) into a sum of three independent pair Hamiltonians. The eigen-solutions of the pair Hamiltonian provide a spectrum of pair states. Each pair state defines the distance of the two electrons involved in this state. In the ground state for given pair angular momentum $m$, this distance increases with increasing $|m|$. The pair states have to be occupied under consideration of the Pauli exclusion principle, which differs from that for one-electron states and depends on the total spin $S$ and the total orbital angular momentum $M_L=\sum m_i$ (sum over all pair angular momenta). We have shown that the three electrons in the ground state of the Wigner molecule form an equilateral triangle (as might be expected) only, if the state is a quartet ($S=3/2$) and the orbital angular momentum is a magic quantum number ($M_L=3 m ; m=$ integer). Otherwise the triangle in the ground state is isosceles. For $M_L=3 m+1$ one of the sides is longer and for $M_L=3 m-1$ one of the sides is shorter than the other two

Wigner Crystallization of a two dimensional electron gas in a magnetic field: single electrons versus electron pairs at the lattice sites

The ground state energy and the lowest excitations of a two dimensional Wigner crystal in a perpendicular magnetic field with one and two electrons per cell is investigated. In case of two electrons per lattice site, the interaction of the electrons {\em within} each cell is taken into account exactly (including exchange and correlation effects), and the interaction {\em between} the cells is in second order (dipole) van der Waals approximation. No further approximations are made, in particular Landau level mixing and {\em in}complete spin polarization are accounted for. Therefore, our calculation comprises a, roughly speaking, complementary description of the bubble phase (in the special case of one and two electrons per bubble), which was proposed by Koulakov, Fogler and Shklovskii on the basis of a Hartree Fock calculation. The phase diagram shows that in GaAs the paired phase is energetically more favorable than the single electron phase for, roughly speaking, filling factor $f$ larger than 0.3 and density parameter $r_s$ smaller than 19 effective Bohr radii (for a more precise statement see Fig.s 4 and 5). If we start within the paired phase and increase magnetic field or decrease density, the pairs first undergo some singlet- triplet transitions before they break.Comment: 11 pages, 7 figure

Quasi-exact solutions for two interacting electrons in two-dimensional anisotropic dots

We present an analysis of the two-dimensional Schrodinger equation for two electrons interacting via Coulombic force and confined in an anizotropic harmonic potential. The separable case of wy = 2wx is studied particularly carefully. The closed-form expressions for bound-state energies and the corresponding eigenfunctions are found at some particular values of wx. For highly-accurate determination of energy levels at other values of wx, we apply an efficient scheme based on the Frobenius expansion.Comment: 11 pages, 4 figure

Unpaired and spin-singlet paired states of a two-dimensional electron gas in a perpendicular magnetic field

We present a variational study of both unpaired and spin-singlet paired states induced in a two-dimensional electron gas at low density by a perpendicular magnetic field. It is based on an improved circular-cell approximation which leads to a number of closed analytical results. The ground-state energy of the Wigner crystal containing a single electron per cell in the lowest Landau level is obtained as a function of the filling factor $\nu$: the results are in good agreement with those of earlier approaches and predict $\nu_{c} \approx 0.25$ for the upper filling factor at which the solid-liquid transition occurs. A novel localized state of spin-singlet electron pairs is examined and found to be a competitor of the unpaired state for filling factor $\nu >1$. The corresponding phase boundary is quantitatively displayed in the magnetic field-electron density plane.Comment: 19 pages, 8 figures, submitted to Phys. Rev. B on 7th April 2001. to appear in Phys. Rev.

Many-body nodal hypersurface and domain averages for correlated wave functions

We outline the basic notions of nodal hypersurface and domain averages for antisymmetric wave functions. We illustrate their properties and analyze the results for a few electron explicitly solvable cases and discuss possible further developments

Roto-vibrational spectrum and Wigner crystallization in two-electron parabolic quantum dots

We provide a quantitative determination of the crystallization onset for two electrons in a parabolic two-dimensional confinement. This system is shown to be well described by a roto-vibrational model, Wigner crystallization occurring when the rotational motion gets decoupled from the vibrational one. The Wigner molecule thus formed is characterized by its moment of inertia and by the corresponding sequence of rotational excited states. The role of a vertical magnetic field is also considered. Additional support to the analysis is given by the Hartree-Fock phase diagram for the ground state and by the random-phase approximation for the moment of inertia and vibron excitations.Comment: 10 pages, 8 figures, replaced by the published versio

Quantum-dot lithium in zero magnetic field: Electronic properties, thermodynamics, and a liquid-solid transition in the ground state

Energy spectra, electron densities, pair correlation functions and heat capacity of a quantum-dot lithium in zero external magnetic field (a system of three interacting two-dimensional electrons in a parabolic confinement potential) are studied using the exact diagonalization approach. A particular attention is given to a Fermi-liquid -- Wigner-solid transition in the ground state of the dot, induced by the intra-dot Coulomb interaction.Comment: 12 pages, incl. 16 figure

Planar Dirac Electron in Coulomb and Magnetic Fields

The Dirac equation for an electron in two spatial dimensions in the Coulomb and homogeneous magnetic fields is discussed. For weak magnetic fields, the approximate energy values are obtained by semiclassical method. In the case with strong magnetic fields, we present the exact recursion relations that determine the coefficients of the series expansion of wave functions, the possible energies and the magnetic fields. It is found that analytic solutions are possible for a denumerably infinite set of magnetic field strengths. This system thus furnishes an example of the so-called quasi-exactly solvable models. A distinctive feature in the Dirac case is that, depending on the strength of the Coulomb field, not all total angular momentum quantum number allow exact solutions with wavefunctions in reasonable polynomial forms. Solutions in the nonrelativistic limit with both attractive and repulsive Coulomb fields are briefly discussed by means of the method of factorization.Comment: 18 pages, RevTex, no figure

Formation and control of electron molecules in artificial atoms: Impurity and magnetic-field effects

Interelectron interactions and correlations in quantum dots can lead to spontaneous symmetry breaking of the self-consistent mean field resulting in formation of Wigner molecules. With the use of spin-and-space unrestricted Hartree-Fock (sS-UHF) calculations, such symmetry breaking is discussed for field-free conditions, as well as under the influence of an external magnetic field. Using as paradigms impurity-doped (as well as the limiting case of clean) two-electron quantum dots (which are analogs to helium-like atoms), it is shown that the interplay between the interelectron repulsion and the electronic zero-point kinetic energy leads, for a broad range of impurity parameters, to formation of a singlet ground-state electron molecule, reminiscent of the molecular picture of doubly-excited helium. Comparative analysis of the conditional probability distributions for the sS-UHF and the exact solutions for the ground state of two interacting electrons in a clean parabolic quantum dot reveals that both of them describe formation of an electron molecule with similar characteristics. The self-consistent field associated with the triplet excited state of the two-electron quantum dot (clean as well as impurity-doped) exhibits symmetry breaking of the Jahn-Teller type, similar to that underlying formation of nonspherical open-shell nuclei and metal clusters. Furthermore, impurity and/or magnetic-field effects can be used to achieve controlled manipulation of the formation and pinning of the discrete orientations of the Wigner molecules. Impurity effects are futher illustrated for the case of a quantum dot with more than two electrons.Comment: Latex/Revtex, 10 pages with 4 gif figures. Small changes to explain the difference between Wigner and Jahn-Teller electron molecules. A complete version of the paper with high quality figures inside the text is available at http://shale.physics.gatech.edu/~costas/qdhelium.html For related papers, see http://www.prism.gatech.edu/~ph274c

Exchange-correlation vector potentials and vorticity-dependent exchange-correlation energy densities in two-dimensional systems

We present a new approach how to calculate the scalar exchange-correlation potentials and the vector exchange-correlation potentials from current-carrying ground states of two-dimensional quantum dots. From these exchange-correlation potentials we derive exchange-correlation energy densities and examine their vorticity (or current) dependence. Compared with parameterizations of current-induced effects in literature we find an increased significance of corrections due to paramagnetic current densities.Comment: 5 figures, submitted to PR