Fusion and breakup in the reactions of 6,7Li and 9Be

We develop a three body classical trajectory Monte Carlo (CTMC) method to dicsuss the effect of the breakup process on heavy-ion fusion reactions induced by weakly bound nuclei. This method follows the classical trajectories of breakup fragments after the breakup takes place, and thus provides an unambiguous separation between complete and incomplete fusion cross sections. Applying this method to the fusion reaction $^{6}$Li + $^{209}$Bi, we find that there is a significant contribution to the total complete fusion cross sections from the process where all the breakup fragments are captured by the target nucleus (i.e., the breakup followed by complete fusion).Comment: 4 pages, 3 eps figures. Uses espcrc1.sty. To be published in the proceedings of the 8th international conference on clustering aspects of nuclear structure and dynamics, November 24 - 29, 2003, Nara, Japan (Nucl. Phys. A

Validity of the linear coupling approximation in heavy-ion fusion reactions at sub barrier energies

The role of higher order coupling of surface vibrations to the relative motion in heavy-ion fusion reactions at near-barrier energies is investigated. The coupled channels equations are solved to all orders, and also in the linear and the quadratic coupling approximations. Taking $^{64}$Ni + $^{92,96}$Zr reactions as examples, it is shown that all order couplings lead to considerably improved agreement with the experimentally measured fusion cross sections and average angular momenta of the compound nucleus for such heavy nearly symmetric systems. The importance of higher order coupling is also examined for asymmetric systems like $^{16}$O + $^{112}$Cd, $^{144}$Sm, for which previous calculations of the fusion cross section seemed to indicate that the linear coupling approximation was adequate. It is shown that the shape of the barrier distributions and the energy dependence of the average angular momentum can change significantly when the higher order couplings are included, even for systems where measured fusion cross sections may seem to be well reproduced by the linear coupling approximation.Comment: Latex file, 15 pages, 6 figure

Suppression of complete fusion due to breakup in the reactions 10,11^{10,11}B + 209^{209}Bi

Above-barrier cross sections of $\alpha$-active heavy reaction products, as well as fission, were measured for the reactions of $^{10,11}$B with $^{209}$Bi. Detailed analysis showed that the heavy products include components from incomplete fusion as well as complete fusion (CF), but fission originates almost exclusively from CF. Compared with fusion calculations without breakup, the CF cross sections are suppressed by 15% for $^{10}$B and 7% for $^{11}$B. A consistent and systematic variation of the suppression of CF for reactions of the weakly bound nuclei $^{6,7}$Li, $^{9}$Be, $^{10,11}$B on targets of $^{208}$Pb and $^{209}$Bi is found as a function of the breakup threshold energy

Relating breakup and incomplete fusion of weakly-bound nuclei through a classical trajectory model with stochastic breakup

A classical dynamical model that treats break-up stochastically is presented for low energy reactions of weakly-bound nuclei. The three-dimensional model allows a consistent calculation of breakup, incomplete and complete fusion cross sections. The model is assessed by comparing the breakup observables with CDCC quantum mechanical predictions, which are found to be in reasonable agreement. Through the model, it is demonstrated that the breakup probability of the projectile as a function of its distance from the target is of primary importance for understanding complete and incomplete fusion at energies near the Coulomb barrier.Comment: Accepted in Physical Review Letter

Importance of Non-Linear Couplings in Fusion Barrier Distributions and Mean Angular Momenta

The effects of higher order coupling of surface vibrations to the relative motion on heavy-ion fusion reactions at near-barrier energies are investigated. The coupled channels equations are solved to all orders, and also in the linear and the quadratic coupling approximations. It is shown that the shape of fusion barrier distributions and the energy dependence of the average angular momentum of the compound nucleus can significantly change when the higher order couplings are included. The role of octupole vibrational excitation of ^{16}O in the ^{16}O + ^{144}Sm fusion reaction is also discussed using the all order coupled-channels equations.Comment: 8 pages, 6 figures, To be published in the Proceedings of the FUSION 97 Conference, South Durras, Australia, March 1997 (J. Phys. G

Microscopic study of the effect of intrinsic degrees of freedom on fusion

Fusion cross-sections are computed for the $^{40}$Ca$+^{40}$Ca system over a wide energy range with two microscopic approaches where the only phenomenological input is the Skyrme energy density functional. The first method is based on the coupled-channels formalism, using the bare nucleus-nucleus potential calculated with the frozen Hartree-Fock technique and the deformation parameters of vibrational states computed with the time-dependent Hartree-Fock (TDHF) approach. The second method is based on the density-constrained TDHF method to generate nucleus-nucleus potentials from TDHF evolution. Both approaches incorporate the effect of couplings to internal degrees of freedoms in different ways. The predictions are in relatively good agreement with experimental data.Comment: 6 pages, 11 figures. Invited talk to FUSION1

Atomic spectral-product representations of molecular electronic structure: metric matrices and atomic-product composition of molecular eigenfunctions

Recent progress is reported in development of ab initio computational methods for the electronic structures of molecules employing the many-electron eigenstates of constituent atoms in spectral-product forms. The approach provides a universal atomic-product description of the electronic structure of matter as an alternative to more commonly employed valence-bond- or molecular-orbital-based representations. The Hamiltonian matrix in this representation is seen to comprise a sum over atomic energies and a pairwise sum over Coulombic interaction terms that depend only on the separations of the individual atomic pairs. Overall electron antisymmetry can be enforced by unitary transformation when appropriate, rather than as a possibly encumbering or unnecessary global constraint. The matrix representative of the antisymmetrizer in the spectral-product basis, which is equivalent to the metric matrix of the corresponding explicitly antisymmetric basis, provides the required transformation to antisymmetric or linearly independent states after Hamiltonian evaluation. Particular attention is focused in the present report on properties of the metric matrix and on the atomic-product compositions of molecular eigenstates as described in the spectral-product representations. Illustrative calculations are reported for simple but prototypically important diatomic (H_2, CH) and triatomic (H_3, CH_2) molecules employing algorithms and computer codes devised recently for this purpose. This particular implementation of the approach combines Slater-orbital-based one- and two-electron integral evaluations, valence-bond constructions of standard tableau functions and matrices, and transformations to atomic eigenstate-product representations. The calculated metric matrices and corresponding potential energy surfaces obtained in this way elucidate a number of aspects of the spectral-product development, including the nature of closure in the representation, the general redundancy or linear dependence of its explicitly antisymmetrized form, the convergence of the apparently disparate atomic-product and explicitly antisymmetrized atomic-product forms to a common invariant subspace, and the nature of a chemical bonding descriptor provided by the atomic-product compositions of molecular eigenstates. Concluding remarks indicate additional studies in progress and the prognosis for performing atomic spectral-product calculations more generally and efficiently

Dissipative quantum dynamics in low-energy collisions of complex nuclei

Model calculations that include the effects of irreversible, environmental couplings on top of a coupled-channels dynamical description of the collision of two complex nuclei are presented. The Liouville-von Neumann equation for the time-evolution of the density matrix of a dissipative system is solved numerically providing a consistent transition from coherent to decoherent (and dissipative) dynamics during the collision. Quantum decoherence and dissipation are clearly manifested in the model calculations. Energy dissipation, due to the irreversible decay of giant-dipole vibrational states of the colliding nuclei, is shown to result in a hindrance of quantum tunneling and fusion.Comment: Accepted in Physical Review