Coherent photodissociation reactions: Observation by a novel picosecond polarization technique

In this communication, we wish to report on a novel picosecond polarization method for measuring the degree of rotational coherence that is preserved in photodissociation reactions. The systems studied here are jet-cooled van der Waals molecules; stilbene [4-6] bound [5] to He or Ne with a 1:1 composition.[7

Quantum statistical effects in multi-channel wave packet scattering of non-interacting identical particles

For a number of non-interacting identical particles entering a multi-channel scatterer in various wave packet states, we construct a generating function for the probabilities of various scattering outcomes. This is used to evaluate the mean numbers of particles $\overline{n}_m$ scattered into a given ($m$-th) channel, single-channel statistics, and inter-channel correlations. We show that for initially uncorrelated particles, indistinguishability changes single channel statistics without altering the the value of $\overline{n}_m$. For uncorrelated bosons and fermions, bunching and anti-bunching behaviour can be detected in the extreme-case probabilities, to have all particles scattered into the same channel, or none of particles scattered into a channel, or channels. As an example, we consider a cavity with a single long-lived resonance accessible to the particles, which allows them to "pile up" inside the scatterer

Theory of one-dimensional double-barrier quantum pump in two-frequency signal regime

A one-dimensional system with two $\delta$-like barriers or wells bi-chromaticaly oscillating at frequencies $\omega$ and $2\omega$ is considered. The alternating signal leads to the direct current across the structure (even in a symmetric system). The properties of this quantum pump are studied in a wide range of the system parameters.Comment: 4 pages, 5 figure

Ultrafast vectorial and scalar dynamics of ionic clusters: Azobenzene solvated by oxygen

The ultrafast dynamics of clusters of trans-azobenzene anion (A–) solvated by oxygen molecules was investigated using femtosecond time-resolved photoelectron spectroscopy. The time scale for stripping off all oxygen molecules from A– was determined by monitoring in real time the transient of the A– rise, following an 800 nm excitation of A– (O2)n, where n=1–4. A careful analysis of the time-dependent photoelectron spectra strongly suggests that for n>1 a quasi-O4 core is formed and that the dissociation occurs by a bond cleavage between A– and conglomerated (O2)n rather than a stepwise evaporation of O2. With time and energy resolutions, we were able to capture the photoelectron signatures of transient species which instantaneously rise (2- for A–O2 and A·O4-·(O2)n–2 for A–(O2)n, where n=2–4. Subsequent to an ultrafast electron recombination, A– rises with two distinct time scales: a subpicosecond component reflecting a direct bond rupture of the A–-(O2)n nuclear coordinate and a slower component (1.6–36 ps, increasing with n) attributed to an indirect channel exhibiting a quasistatistical behavior. The photodetachment transients exhibit a change in the transition dipole direction as a function of time delay. Rotational dephasing occurs on a time scale of 2–3 ps, with a change in the sign of the transient anisotropy between A–O2 and the larger clusters. This behavior is a key indicator of an evolving cluster structure and is successfully modeled by calculations based on the structures and inertial motion of the parent clusters

Properties of 1D two-barrier quantum pump with harmonically oscillating barriers

We study a one-dimensional quantum pump composed of two oscillating delta-functional barriers. The linear and non-linear regimes are considered. The harmonic signal applied to any or both barriers causes the stationary current. The direction and value of the current depend on the frequency, distance between barriers, value of stationary and oscillating parts of barrier potential and the phase shift between alternating voltages.Comment: 7 pages, 8 figure

Quasiclassical negative magnetoresistance of a 2D electron gas: interplay of strong scatterers and smooth disorder

We study the quasiclassical magnetotransport of non-interacting fermions in two dimensions moving in a random array of strong scatterers (antidots, impurities or defects) on the background of a smooth random potential. We demonstrate that the combination of the two types of disorder induces a novel mechanism leading to a strong negative magnetoresistance, followed by the saturation of the magnetoresistivity $\rho_{xx}(B)$ at a value determined solely by the smooth disorder. Experimental relevance to the transport in semiconductor heterostructures is discussed.Comment: 4 pages, 2 figure

Directed transport born from chaos in asymmetric antidot structures

It is shown that a polarized microwave radiation creates directed transport in an asymmetric antidot superlattice in a two dimensional electron gas. A numerical method is developed that allows to establish the dependence of this ratchet effect on several parameters relevant for real experimental studies. It is applied to the concrete case of a semidisk Galton board where the electron dynamics is chaotic in the absence of microwave driving. The obtained results show that high currents can be reached at a relatively low microwave power. This effect opens new possibilities for microwave control of transport in asymmetric superlattices.Comment: 8 pages, 10 figure

Quasiclassical magnetotransport in a random array of antidots

We study theoretically the magnetoresistance $\rho_{xx}(B)$ of a two-dimensional electron gas scattered by a random ensemble of impenetrable discs in the presence of a long-range correlated random potential. We believe that this model describes a high-mobility semiconductor heterostructure with a random array of antidots. We show that the interplay of scattering by the two types of disorder generates new behavior of $\rho_{xx}(B)$ which is absent for only one kind of disorder. We demonstrate that even a weak long-range disorder becomes important with increasing $B$. In particular, although $\rho_{xx}(B)$ vanishes in the limit of large $B$ when only one type of disorder is present, we show that it keeps growing with increasing $B$ in the antidot array in the presence of smooth disorder. The reversal of the behavior of $\rho_{xx}(B)$ is due to a mutual destruction of the quasiclassical localization induced by a strong magnetic field: specifically, the adiabatic localization in the long-range Gaussian disorder is washed out by the scattering on hard discs, whereas the adiabatic drift and related percolation of cyclotron orbits destroys the localization in the dilute system of hard discs. For intermediate magnetic fields in a dilute antidot array, we show the existence of a strong negative magnetoresistance, which leads to a nonmonotonic dependence of $\rho_{xx}(B)$.Comment: 21 pages, 13 figure