159 research outputs found
Magnetic and electrical properties of dhcp NpPd3 and U(1-x)Np(x)Pd3
We have made an extensive study of the magnetic and electrical properties of
double-hexagonal closepacked NpPd3 and a range of U(1-x)Np(x)Pd3 compounds with
x=0.01, 0.02, 0.05, and 0.50 using magnetization, magnetic susceptibility,
electrical resistivity, and heat capacity measurements on polycrystalline
samples, performed in the temperature range 2-300 K and in magnetic fields up
to 9 T. Two transitions are observed in NpPd3 at T=10 and 30 K. Dilute Np
samples (x<0.05) exhibit quadrupolar transitions, with the transition
temperatures reduced from those of pure UPd3.Comment: 10 pages, 18 figure
Magnetic and electrical properties of (Pu,Lu)Pd3
We present measurements of the magnetic susceptibility, heat capacity and
electrical resistivity of PuLuPd, with =0, 0.1, 0.2, 0.5,
0.8 and 1. PuPd is an antiferromagnetic heavy fermion compound with
~K. With increasing Lu doping, both the Kondo and RKKY interaction
strengths fall, as judged by the Sommerfeld coefficient and N\'eel
temperature . Fits to a crystal field model of the resistivity also
support these conclusions. The paramagnetic effective moment
increases with Lu dilution, indicating a decrease in the
Kondo screening. In the highly dilute limit, approaches
the value predicted by intermediate coupling calculations. In conjunction with
an observed Schottky peak at 60~K in the magnetic heat capacity,
corresponding to a crystal field splitting of 12~meV, a mean-field
intermediate coupling model with nearest neighbour interactions has been
developed.Comment: 13 pages, 13 figure
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