How quickly do cloud droplets form on atmospheric particles?

International audienceThe influence of aerosols on cloud properties is an important modulator of the climate system. Traditional Köhler theory predicts the equilibrium concentration of cloud condensation nuclei (CCN); however, it is not known to what extent particles exist in the atmosphere that may be prevented from acting as CCN by kinetic limitations. We measured the rate of cloud droplet formation on atmospheric particles sampled at four sites across the United States during the summer of 2006: Great Smoky Mountain National Park, TN; Bondville, IL; Houston, TX; and the Atmospheric Radiation Measurement Program Southern Great Plains site near Lamont, OK. We express droplet growth rates with the mass accommodation coefficient (?), and report values of ? measured in the field normalized to the mean ? measured for lab-generated ammonium sulfate (AS) particles (i.e., ?'=?/?AS). Overall, 61% of ambient CCN grew at a rate similar to AS. We report the fraction of CCN that were "low-?'" (?'?0.33). Of the 16 days during which these measurements were made, 7 had relatively few low-?'CCN (77% during at least one ~30 min period). Day to day variability was greatest in Tennessee and Illinois, and low-?' CCN were most prevalent on days when back trajectories suggested that air was arriving from aloft. The highest fractions of low-?' CCN in Houston and Illinois occurred around local noon, and decreased later in the day. These results suggest that for some air masses, accurate quantification of CCN concentrations may need to account for kinetic limitations

The Influence of Superpositional Wave Function Oscillations on Shor's Quantum Algorithm

We investigate the influence of superpositional wave function oscillations on the performance of Shor's quantum algorithm for factorization of integers. It is shown that the wave function oscillations can destroy the required quantum interference. This undesirable effect can be routinely eliminated using a resonant pulse implementation of quantum computation, but requires special analysis for non-resonant implementations.Comment: 4 pages, NO figures, revte

Limitations of Quantum Simulation Examined by Simulating a Pairing Hamiltonian using Nuclear Magnetic Resonance

Quantum simulation uses a well-known quantum system to predict the behavior of another quantum system. Certain limitations in this technique arise, however, when applied to specific problems, as we demonstrate with a theoretical and experimental study of an algorithm to find the low-lying spectrum of a Hamiltonian. While the number of elementary quantum gates does scale polynomially with the size of the system, it increases inversely to the desired error bound $\epsilon$. Making such simulations robust to decoherence using fault-tolerance constructs requires an additional factor of $1/ \epsilon$ gates. These constraints are illustrated by using a three qubit nuclear magnetic resonance system to simulate a pairing Hamiltonian, following the algorithm proposed by Wu, Byrd, and Lidar.Comment: 6 pages, 2 eps figure

Quantum Bit Regeneration

Decoherence and loss will limit the practicality of quantum cryptography and computing unless successful error correction techniques are developed. To this end, we have discovered a new scheme for perfectly detecting and rejecting the error caused by loss (amplitude damping to a reservoir at T=0), based on using a dual-rail representation of a quantum bit. This is possible because (1) balanced loss does not perform a ``which-path'' measurement in an interferometer, and (2) balanced quantum nondemolition measurement of the ``total'' photon number can be used to detect loss-induced quantum jumps without disturbing the quantum coherence essential to the quantum bit. Our results are immediately applicable to optical quantum computers using single photonics devices.Comment: 4 pages, postscript only, figures available at http://feynman.stanford.edu/qcom

Ethyl cyanide on Titan: Spectroscopic detection and mapping using ALMA

We report the first spectroscopic detection of ethyl cyanide (C$_2$H$_5$CN) in Titan's atmosphere, obtained using spectrally and spatially resolved observations of multiple emission lines with the Atacama Large Millimeter/submillimeter array (ALMA). The presence of C$_2$H$_5$CN in Titan's ionosphere was previously inferred from Cassini ion mass spectrometry measurements of C$_2$H$_5$CNH$^+$. Here we report the detection of 27 rotational lines from C$_2$H$_5$CN (in 19 separate emission features detected at $>3\sigma$ confidence), in the frequency range 222-241 GHz. Simultaneous detections of multiple emission lines from HC$_3$N, CH$_3$CN and CH$_3$CCH were also obtained. In contrast to HC$_3$N, CH$_3$CN and CH$_3$CCH, which peak in Titan's northern (spring) hemisphere, the emission from C$_2$H$_5$CN is found to be concentrated in the southern (autumn) hemisphere, suggesting a distinctly different chemistry for this species, consistent with a relatively short chemical lifetime for C$_2$H$_5$CN. Radiative transfer models show that most of the C$_2$H$_5$CN is concentrated at altitudes 300-600 km, suggesting production predominantly in the mesosphere and above. Vertical column densities are found to be in the range (2-5)$\times10^{14}$ cm$^{-2}$.Comment: Published in 2015, ApJL, 800, L1

Doubling of the bands in overdoped Bi2Sr2CaCu2O8-probable evidence for c-axis bilayer coupling

We present high resolution ARPES data of the bilayer superconductor Bi2Sr2CaCu2O8 (Bi2212) showing a clear doubling of the near EF bands. This splitting approaches zero along the (0,0)-(pi,pi) nodal line and is not observed in single layer Bi2Sr2CuO6 (Bi2201), suggesting that the splitting is due to the long sought after bilayer splitting effect. The splitting has a magnitude of approximately 75 meV near the middle of the zone, extrapolating to about 100 meV near the (pi,0) poin

Ferromagnetic Enhancement of CE-type Spin Ordering in (Pr,Ca)MnO3_3

We present resonant soft X-ray scattering (RSXS) results from small band width manganites (Pr,Ca)MnO$_3$, which show that the CE-type spin ordering (SO) at the phase boundary is stabilized only below the canted antiferromagnetic transition temperature and enhanced by ferromagnetism in the macroscopically insulating state (FM-I). Our results reveal the fragility of the CE-type ordering that underpins the colossal magnetoresistance (CMR) effect in this system, as well as an unexpected cooperative interplay between FM-I and CE-type SO which is in contrast to the competitive interplay between the ferromagnetic metallic (FM-M) state and CE-type ordering.Comment: Accepted for publication in Phys. Rev. Let