2,936 research outputs found
First-order nature of the ferromagnetic phase transition in (La-Ca)MnO_3 near optimal doping
Neutron scattering has been used to study the nature of the ferromagnetic
transition in single crystals of La_0.7Ca_0.3MnO_3 and La_0.8Ca_0.2MnO_3, and
polycrystalline samples of La_0.67Ca_0.33MnO_3 and La_5/8Ca_3/8MnO_3 where the
naturally occurring O-16 can be replaced with the O-18 isotope. Small angle
neutron scattering on the x=0.3 single crystal reveals a discontinuous change
in the scattering at the Curie temperature for wave vectors below ~0.065 A^-1.
Strong relaxation effects are observed for this domain scattering, for the
magnetic order parameter, and for the quasielastic scattering, demonstrating
that the transition is not continuous in nature. There is a large oxygen
isotope effect observed for the T_C in the polycrystalline samples. For the
optimally doped x=3/8 sample we observed T_C(O-16)=266.5 K and T_C(O-18)=261.5
K at 90% O-18 substitution. The temperature dependence of the spin-wave
stiffness is found to be identical for the two samples despite changes in T_C.
Hence, T_C is not solely determined by the magnetic subsystem, but instead the
ferromagnetic phase is truncated by the formation of polarons which cause an
abrupt transition to the paramagnetic, insulating state. Application of
uniaxial stress in the x=0.3 single crystal sharply enhances the polaron
scattering at room temperature. Measurements of the phonon density-of-states
show only modest differences above and below T_C and between the two different
isotopic samples.Comment: 13 pages, 16 figures, submitted to Phys. Rev.
Interplay of charge and spin correlations in nickel perovskites
Analyzing the motion of low--spin holes in a high--spin
background, we derive a sort of generalized t--J Hamiltonian for the planes of Sr--doped nickelates. In addition to the rather complex
carrier--spin and spin--spin couplings we take into account the coupling of the
doped holes to in--plane oxygen breathing modes by a Holstein--type interaction
term. Because of strong magnetic confinement effects the holes are nearly
entirely prelocalized and the electron--phonon coupling becomes much more
effective in forming polarons than in the isostructural cuprates. In the light
of recent experiments on we discuss how the variety of
the observed transport and charge/spin--ordering phenomena can be qualitatively
understood in terms of our model Hamiltonian.Comment: 2 pages, LTpaper.sty, Proc. XXI Int. Conf. on Low Temp. Phys. Prague
9
X-ray induced electronic structure change in CuIrS
The electronic structure of CuIrS has been investigated using various
bulk-sensitive x-ray spectroscopic methods near the Ir -edge: resonant
inelastic x-ray scattering (RIXS), x-ray absorption spectroscopy in the partial
fluorescence yield (PFY-XAS) mode, and resonant x-ray emission spectroscopy
(RXES). A strong RIXS signal (0.75 eV) resulting from a charge-density-wave gap
opening is observed below the metal-insulator transition temperature of 230 K.
The resultant modification of electronic structure is consistent with the
density functional theory prediction. In the spin- and charge- dimer disordered
phase induced by x-ray irradiation below 50 K, we find that a broad peak around
0.4 eV appears in the RIXS spectrum.Comment: 4 pages and 4 figure
Electromagnons in multiferroic YMn2O5 and TbMn2O5
Based on temperature dependent far infrared transmission spectra of YMn2O5
and TbMn2O5 single crystals, we report the observation of electric
dipole-active magnetic excitations, or electromagnons, in these multiferroics.
Electromagnons are found to be directly responsible for the step-like anomaly
of the static dielectric constant at the commensurate--incommensurate magnetic
transition and are the origin of the colossal magneto-dielectric effect
reported in these multiferroics.Comment: 4 pages, 4 figures, submitte
Strengthening the Cohomological Crepant Resolution Conjecture for Hilbert-Chow morphisms
Given any smooth toric surface S, we prove a SYM-HILB correspondence which
relates the 3-point, degree zero, extended Gromov-Witten invariants of the
n-fold symmetric product stack [Sym^n(S)] of S to the 3-point extremal
Gromov-Witten invariants of the Hilbert scheme Hilb^n(S) of n points on S. As
we do not specialize the values of the quantum parameters involved, this result
proves a strengthening of Ruan's Cohomological Crepant Resolution Conjecture
for the Hilbert-Chow morphism from Hilb^n(S) to Sym^n(S) and yields a method of
reconstructing the cup product for Hilb^n(S) from the orbifold invariants of
[Sym^n(S)].Comment: Revised versio
Melting of Quasi-Two-Dimensional Charge Stripes in La5/3Sr1/3NiO4
Commensurability effects for nickelates have been studied by the first
neutron experiments on La5/3Sr1/3NiO4. Upon cooling, this system undergoes
three successive phase transitions associated with quasi-two-dimensional (2D)
commensurate charge and spin stripe ordering in the NiO planes. The two
lower temperature phases (denoted as phase II and III) are stripe lattice
states with quasi-long-range in-plane charge correlation. When the lattice of
2D charge stripes melts, it goes through an intermediate glass state (phase I)
before becoming a disordered liquid state. This glass state shows short-range
charge order without spin order, and may be called a "stripe glass" which
resembles the hexatic/nematic state in 2D melting.Comment: 10 pages, RevTex, 4 figures available on request to
[email protected]
Structural and Magnetic Characterization of Large Area, Free-Standing Thin Films of Magnetic Ion Intercalated Dichalcogenides Mn0.25TaS2 and Fe0.25TaS2
Free-standing thin films of magnetic ion intercalated transition metal
dichalcogenides are produced using ultramicrotoming techniques. Films of
thicknesses ranging from 30nm to 250nm were achieved and characterized using
transmission electron diffraction and X-ray magnetic circular dichroism.
Diffraction measurements visualize the long range crystallographic ordering of
the intercalated ions, while the dichroism measurements directly assess the
orbital contributions to the total magnetic moment. We thus verify the
unquenched orbital moment in Fe0.25TaS2 and measure the fully quenched orbital
contribution in Mn0.25TaS2. Such films can be used in a wide variety of
ultrafast X-ray and electron techniques that benefit from transmission
geometries, and allow measurements of ultrafast structural, electronic, and
magnetization dynamics in space and time
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