1,542 research outputs found

    Direct evidence for the magnetic ordering of Nd ions in NdMn2_2Si2_2 and NdMn2_2Ge2_2 by high resolution inelastic neutron scattering

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    We have investigated the low energy nuclear spin excitations in NdMn2_2Si2_2 and NdMn2_2Ge2_2 by high resolution inelastic neutron scattering. Previous neutron diffraction investigations gave ambiguous results about Nd magnetic ordering at low temperatures. The present element-specific technique gave direct evidence for the magnetic ordering of Nd ions. We found considerable difference in the process of the Nd magnetic ordering at low temperature in NdMn2_2Si2_2 and NdMn2_2Ge2_2. Our results are consistent with those of magnetization and recent neutron diffraction measurements

    Polarisation dependence of magnetic Bragg scattering in YMn2_2O5_5

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    The polarisation dependence of the intensity of elastic magnetic scattering from \ymno\ single crystals has been measured at 25 K in magnetic fields between 1 and 9 T. A significant polarisation dependence was observed in the intensities of magnetic satellite reflections, propagation vector \pv=0.5,0,0.25 measured with both the [100] and [010] axes parallel to the common polarisation and applied field direction. The intensity asymmetries AA observed in sets of orthorhombicly equivalent reflections show systematic relationships which allow the phase relationship between different components of their magnetic interaction vectors to be determined. They fix the orientation relationships between the small yy and zz moments on the \mnfp\ and \mntp\ sub-lattices and lend support to the structure reported by Kim et al. It was found that that A(hkl)≠A(hˉkˉlˉ)A(hkl)\ne A(\bar h\bar k\bar l) which suggests that there is a small modulation of the nuclear structure which has the same wave-vector as the magnetic modulation leading to a small nuclear structure factor for the satellite reflections. The differences A(hkl)−A(hˉkˉlˉ)A(hkl)- A(\bar h\bar k\bar l) observed indicate shifts in the atomic positions of order 0.005 \AA

    Magnetoelastic effects in Jahn-Teller distorted CrF2_2 and CuF2_2 studied by neutron powder diffraction

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    We have studied the temperature dependence of crystal and magnetic structures of the Jahn-Teller distorted transition metal difluorides CrF2_2 and CuF2_2 by neutron powder diffraction in the temperature range 2-280 K. The lattice parameters and the unit cell volume show magnetoelastic effects below the N\'eel temperature. The lattice strain due to the magnetostriction effect couples with the square of the order parameter of the antiferromagnetic phase transition. We also investigated the temperature dependence of the Jahn-Teller distortion which does not show any significant effect at the antiferromagnetic phase transition but increases linearly with increasing temperature for CrF2_2 and remains almost independent of temperature in CuF2_2. The magnitude of magnetovolume effect seems to increase with the low temperature saturated magnetic moment of the transition metal ions but the correlation is not at all perfect

    Multiferroic coupling in nanoscale BiFeO3

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    Using the results of x-ray and neutron diffraction experiments, we show that the ferroelectric polarization, in ~22 nm particles of BiFeO3, exhibits a jump by ~30% around the magnetic transition point T_N (~635 K) and a suppression by ~7% under 5T magnetic field at room temperature (<<T_N). These results confirm presence of strong multiferroic coupling even in nanoscale BiFeO3 and thus could prove to be quite useful for applications based on nanosized devices of BiFeO3.Comment: 4 pages including 4 figures and supplementary data; accepted for publication in Appl. Phys. Let

    Weak ferromagnetism and magnetic phase transitions in Gd2_2CuO4_4

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    We report a polarised neutron study of the magnetic structures and phase trasitions in \gdc\ in low magnetic fields. These experiments have been complemented by integrated intensity measurements with unpolarised neutrons in zero field. Polarised neutron flipping ratio measurements have been made with magnetic fields H=0.05H = 0.05, 0.10 and 0.5 T in the temperature range 4-20 K. These have enabled us to deduce that the anomalous temperature behaviour of the coherent magnetic scattering from the Cu sublattice, which shows sharp intensity minima at \Tcn1 ≈18\approx 18K and \Tcn2 ≈8\approx 8 K, is due to cross-overs in the sign of the interaction between strongly coupled, weakly ferromagnetic, CuO2_2 layers. At \Tcn1\ the coupling changes from ferromagnetic to anti-ferromagnetic and long-range order between layers is temporarily lost. \Tcn2\ is the temperature at which the Gd moments order and a further reorganisation of the interlayer order takes place. The weak ferromagnetism of the CuO layers is found to be due to a small rotation of the Cu moments in the same direction as that in which their coordinating oxygen squares rotate in the tetragonal to orthorhombic distortion of the crystal structure. Further analysis of the flipping ratio measurements has enabled us to model the magnetic structures of the zero-field and the field-induced phases of Gd2_2CuO4_4

    Identification of candidate categories of the International Classification of Functioning Disability and Health (ICF) for a Generic ICF Core Set based on regression modelling

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    Background: The International Classification of Functioning, Disability and Health (ICF) is the framework developed by WHO to describe functioning and disability at both the individual and population levels. While condition-specific ICF Core Sets are useful, a Generic ICF Core Set is needed to describe and compare problems in functioning across health conditions. Methods: The aims of the multi-centre, cross-sectional study presented here were: a) to propose a method to select ICF categories when a large amount of ICF-based data have to be handled, and b) to identify candidate ICF categories for a Generic ICF Core Set by examining their explanatory power in relation to item one of the SF-36. The data were collected from 1039 patients using the ICF checklist, the SF-36 and a Comorbidity Questionnaire. ICF categories to be entered in an initial regression model were selected following systematic steps in accordance with the ICF structure. Based on an initial regression model, additional models were designed by systematically substituting the ICF categories included in it with ICF categories with which they were highly correlated. Results: Fourteen different regression models were performed. The variance the performed models account for ranged from 22.27% to 24.0%. The ICF category that explained the highest amount of variance in all the models was sensation of pain. In total, thirteen candidate ICF categories for a Generic ICF Core Set were proposed. Conclusion: The selection strategy based on the ICF structure and the examination of the best possible alternative models does not provide a final answer about which ICF categories must be considered, but leads to a selection of suitable candidates which needs further consideration and comparison with the results of other selection strategies in developing a Generic ICF Core Set
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