12 research outputs found
Spin fluctuations, magnetic long-range order and Fermi surface gapping in NaxCoO2
In this study an extended low energy phase diagram for NaxCoO2 is
experimentally established with emphasis on the high x range. It is based on
systematic heat capacity studies on both polycrystalline and single crystalline
samples and on uSR measurements. Main features are the existence of mass
enhancement, spin fluctuations without long-range order, and magnetic order
with associated Fermi surface gapping. The latter is seen in the electronic
density of states (DOS) and suppression of nuclear specific heat. While there
is agreement between the band structure and the low energy DOS in the low x
range, in the high x range (x > 0.6) the thermodynamically determined DOS is
approximately three times that deduced from the angle-resolved photoemission
spectroscopy (ARPES)-measured band dispersion or local-density approximation
(LDA) calculations.Comment: 9 pages, 5 figure
NaxCoO2: Enhanced low-energy excitations of electrons on a 2D triangular lattice
To elucidate the low-energy excitation spectrum of correlated electrons on a
2D triangular lattice, we have studied the electrical resistance and specific
heat down to 0.5 K and in magnetic fields up to 14 T, in NaxCoO2 samples with a
Na content ranging from x \approx 0.5 to 0.82. Two distinct regimes are
observed: for x from about 0.6 to x \approx 0.75 the specific heat is strongly
enhanced, with a pronounced upturn of C/T below about 10 K, reaching 47 mJ/(mol
K^2). This enhancement is suppressed in a magnetic field indicative of strong
low-energy spin fluctuations. At higher Na content the fluctuations are reduced
and mu-SR data confirm the SDW ground state below 22 K and the much reduced
heat capacity is field independent.Comment: Accepted in Physica