Dynamics of Lennard-Jones clusters: A characterization of the activation-relaxation technique

The potential energy surface (PES) of Lennard-Jones clusters is investigated using the activation-relaxation technique (ART). This method defines events in the configurational energy landscape as a two-step process: (a) a configuration is first activated from a local minimum to a nearby saddle-point and (b) is then relaxed to a new minimum. Although ART has been applied with success to a wide range of materials such as a-Si, a-SiO2 and binary Lennard-Jones glasses, questions remain regarding the biases of the technique. We address some of these questions in a detailed study of ART-generated events in Lennard-Jones (LJ) clusters, a system for which much is already known. In particular, we study the distribution of saddle-points, the pathways between configurations, and the reversibility of paths. We find that ART can identify all trajectories with a first-order saddle point leaving a given minimum, is fully reversible, and samples events following the Boltzmann weight at the saddle point.Comment: 8 pages, 7 figures in postscrip

Indications of flow near maximum compression in layered DT implosions at the National Ignition Facility

An accurate understanding of burn dynamics in implosions of cryogenically layered deuterium and tritium (DT) filled capsules, obtained partly through precision diagnosis of these experiments, is essential for assessing the impediments to achieving ignition at the National Ignition Facility (NIF). We present measurements of neutrons from such implosions. The apparent ion temperatures (Tion) are inferred from the variance of the primary neutron spectrum. Consistently higher DT than DD Tions are observed, and the difference is seen to increase with increasing apparent DT Tion. The line-of-sight r.m.s. variations of both DD and DT Tion are small, ~150 eV, indicating an isotropic source. DD neutron yields are consistently high relative to the DT neutron yields given the observed Tions. Spatial and temporal variations of the DT temperature and density, DD-DT differential attenuation in the surrounding DT fuel, and fluid motion variations contribute to DT Tion > DD Tion, but are in a 1D model insufficient to explain the data. We hypothesize that in a 3D interpretation, these effects combined could explain the results