Anthropogenic Space Weather

Anthropogenic effects on the space environment started in the late 19th century and reached their peak in the 1960s when high-altitude nuclear explosions were carried out by the USA and the Soviet Union. These explosions created artificial radiation belts near Earth that resulted in major damages to several satellites. Another, unexpected impact of the high-altitude nuclear tests was the electromagnetic pulse (EMP) that can have devastating effects over a large geographic area (as large as the continental United States). Other anthropogenic impacts on the space environment include chemical release ex- periments, high-frequency wave heating of the ionosphere and the interaction of VLF waves with the radiation belts. This paper reviews the fundamental physical process behind these phenomena and discusses the observations of their impacts.Comment: 71 pages, 35 figure

Reply to: Possible overestimation of isomer depletion due to contamination

We appreciate the interest of Guo et al., the points that they raise, and the opportunity that we have to provide additional details that are not included in ref. This allows us to strengthen our experimental case while, in parallel, recent developments are improving our theoretical understanding of nuclear excitation by electron capture (NEEC), such as the exploration of a substantial increase in predicted NEEC probability when considering capture by an ion in an excited state (S. Gargiulo et al., submitted) or the impact of the momentum distribution of target electrons (J.R. et al., submitted). In the accompanying Comment, Guo et al. focus on whether potential background contributions were underestimated in our analysis. As discussed below, these concerns are mostly unwarranted; aside from a small systematic uncertainty that could possibly slightly reduce our reported NEEC excitation probability of Pexc = 0.010(3), our original conclusions still stand

Isomer depletion as experimental evidence of nuclear excitation by electron capture

The atomic nucleus and its electrons are often thought of as independent systems that are held together in the atom by their mutual attraction. Their interaction, however, leads to other important effects, such as providing an additional decay mode for excited nuclear states, whereby the nucleus releases energy by ejecting an atomic electron instead of by emitting a 3-ray. This 'internal conversion' has been known for about a hundred years and can be used to study nuclei and their interaction with their electrons. In the inverse process - nuclear excitation by electron capture (NEEC) - a free electron is captured into an atomic vacancy and can excite the nucleus to a higher-energy state, provided that the kinetic energy of the free electron plus the magnitude of its binding energy once captured matches the nuclear energy difference between the two states. NEEC was predicted in 1976 and has not hitherto been observed. Here we report evidence of NEEC in molybdenum-93 and determine the probability and cross-section for the process in a beam-based experimental scenario. Our results provide a standard for the assessment of theoretical models relevant to NEEC, which predict cross-sections that span many orders of magnitude. The greatest practical effect of the NEEC process may be on the survival of nuclei in stellar environments, in which it could excite isomers (that is, long-lived nuclear states) to shorter-lived states. Such excitations may reduce the abundance of the isotope after its production. This is an example of 'isomer depletion', which has been investigated previously through other reactions, but is used here to obtain evidence for NEEC

High-spin, multiparticle isomers in Sb121,123

Isomers in near-spherical Z=51, antimony isotopes are reported here for the first time using fusion-fission reactions between Al27 and a pulsed Hf178 beam of energy, 1150 MeV. γ rays were observed from the decay of isomeric states with half-lives, T1/2=200(30) and 52(3)μs, and angular momenta I=(252) and Iπ=232+, in Sb121,123, respectively. These states are proposed to correspond to ν(h112)2 configurations, coupled to an odd d52 or g72 proton. Nanosecond isomers were also identified at Iπ=192- [T1/2=8.5(5) ns] in Sb121 and Iπ=(152-) [T1/2=37(4) ns] in Sb123. Information on spins and parities of states in these nuclei was obtained using a combination of angular correlation and intensity-balance measurements. The configurations of states in these nuclei are discussed using a combination of spin/energy systematics and shell-model calculations for neighboring tin isotones and antimony isotopes

Coulomb excitation of a 242Am isomeric target: E2 and e3 strengths, rotational alignment, and collective enhancement

A 98% pure242mAm (K = 5-, t1/2 = 141 years) isomeric target was Coulomb excited with a 170.5-MeV 40Ar beam. The selectivity of Coulomb excitation, coupled with the sensitivity of Gammasphere plus CHICO, was sufficient to identify 46 new states up to spin 18h{stroke} in at least four rotational bands; 11 of these new states lie in the isomer band, 13 in a previously unknown yrast Kπ = 6- rotational band, and 13 in a band tentatively identified as the predicted yrast Kπ = 5+ band. The rotational bands based on the Kπ = 5- isomer and the 6-bandhead were populated by Coulomb excitation with unexpectedly equal cross sections. The γ -ray yields are reproduced by Coulomb excitation calculations using a two-particle plus rotor model (PRM), implying nearly complete ΔK = 1 mixing of the two almost-degenerate rotational bands, but recovering the Alaga rule for the unperturbed states. The degeneracy of the 5- and 6- bands allows for precise determination of the mixing interaction strength V, which approaches the strong-mixing limit; this agrees with the 50% attenuation of the Coriolis matrix element assumed in the model calculations. The fractional admixture of the I πK= 6-6 state in the nominal 6-5 isomer band state is measured within the PRM as 45.6+0.3-1.1%. The E2 and M1 strengths coupling the 5- and 6- bands are enhanced significantly by the mixing, while E1 and E2 couplings to other low-K bands are not measurably enhanced. The yields of the 5+ band are reproduced by an E3 strength of ≈15 W.u., competitive with the interband E2 strength. Alignments of the identified two-particle Nilsson states in 242Am are compared with the single-particle alignments in 241Am

Rotational alignments in Np235 and the possible role of j15/2 neutrons

The role j15/2 neutron orbitals play in the transuranic region of actinides has been studied by exploring γ-ray transitions between yrast states in Np235, populated utilizing the nucleon-transfer reaction Np237(Sn116,Sn118). Two rotational sequences, presumably the two signatures of the ground-state band, have been delineated to high spin for the first time, with the α=+1/2 and α=-1/2 signature partners reaching 49/2 (tentatively 53/2+) and 47/2+ (tentatively 51/2+), respectively. Definite isotopic assignments for these in-band transitions were established through γ-ray cross correlations between Np235 and Sn118 and events where at least three γ rays corresponding to neptunium-like particles were detected. These transitions reveal clear upbends in the aligned angular momentum and kinematic moment of inertia plots; such a phenomenon could indicate a strong interaction between an aligned νj15/2 configuration crossing the ground-state band in Np235, which is based on a πi13/2 orbital. However, the lack of any signature splitting over the observed frequency range of the Np235 rotational sequences cannot remove the possibility of a πh9/2 assignment for the observed band. The role of the νj15/2 and πi13/2 alignment mechanisms in the deformed U-Pu region is discussed in light of the current spectroscopic data and in the context of the cranked-shell model

New structures in 178Hf and coulomb excitation of isomers

A 985 MeV 178Hf beam was Coulomb excited by a 208Pb target at the ATLAS accelerator of Argonne National Laboratory. Gammasphere and the CHICO particle detector recorded particle-γ coincidence data. The aim was to populate and determine the mechanism of previously observed Coulomb excitation of the Kπ = 6+ (t1/2 = 77 ns), 8- (4 s) and 16+ (31 y) isomer bands. New rotational bands were identified including an aligned band which appears to mix with the ground-state band (GSB) and the γ-vibrational band above ∼ 12 ℏ of angular momentum. Newly observed γ-decay transitions into the three isomer bands may elucidate the K-mixing which allows Coulomb excitation of these isomer bands, but direct decays from the GSB into the 16+ isomer band have not yet been confirmed

Spectroscopy of Rf257

The isotope Rf257 was produced in the fusion-evaporation reaction Pb208(Ti50,n)Rf257. Reaction products were separated and identified by mass. Delayed spectroscopy of Rf257 and its decay products was performed. A partial decay scheme with configuration assignments is proposed based on α hindrance factors. The excitation energy of the 1/2+[620] configuration in No253 is proposed. The energy of this 1/2+ state in a series of N=151 isotones increases with nuclear charge, reflecting an increase in the N=152 gap. This gap is deduced to grow substantially from 850 to 1400 keV between Z=94 and 102. An isomeric state in Rf257, with a half-life of 160-31+42μs, was discovered by detecting internal conversion electrons followed by α decay. It is interpreted as a three-quasiparticle high-K isomer. A second group of internal conversion electrons, with a half-life of 4.1-1.3+2.4 s, followed by α decay, was also observed. These events might originate from the decay of excited states in Lr257, populated by electron-capture decay of Rf257. Fission of Rf257 was unambiguously detected, with a branching ratio of bRfSF=0.02±0.01

First direct observation of enhanced octupole collectivity in 146Ba

The octupole strength present in the neutron-rich, radiocative nucleus 146Ba has been experimentally determined for the first time using Coulomb excitation. To achieve this, A=146 fission fragments from CARIBU were post-accelerated by the Argonne Tandem Linac Accelerator System (ATLAS) and impinged on a thin 208Pb target. Using the GRETINA γ-ray spectrometer and the CHICO2 heavy-ion counter, the reduced transition probability B(E3; 3-→0+) was determined as 48(+21-29) W.u. The new result provides further experimental evidence for the presence of a region of octupole deformation surrounding the neutron-rich barium isotopes