41 research outputs found

    Strengths of the resonances at 436, 479, 639, 661, and 1279 keV in the 22^{22}Ne(p,γ\gamma)23^{23}Na reaction

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    The 22^{22}Ne(p,γ\gamma)23^{23}Na reaction is included in the neon-sodium cycle of hydrogen burning. A number of narrow resonances in the Gamow window dominates the thermonuclear reaction rate. Several resonance strengths are only poorly known. As a result, the 22^{22}Ne(p,γ\gamma)23^{23}Na thermonuclear reaction rate is the most uncertain rate of the cycle. Here, a new experimental study of the strengths of the resonances at 436, 479, 639, 661, and 1279 keV proton beam energy is reported. The data have been obtained using a tantalum target implanted with 22^{22}Ne. The strengths ωγ\omega\gamma of the resonances at 436, 639, and 661 keV have been determined with a relative approach, using the 479 and 1279 keV resonances for normalization. Subsequently, the ratio of resonance strengths of the 479 and 1279 keV resonances was determined, improving the precision of these two standards. The new data are consistent with, but more precise than, the literature with the exception of the resonance at 661 keV, which is found to be less intense by one order of magnitude. In addition, improved branching ratios have been determined for the gamma decay of the resonances at 436, 479, and 639 keV.Comment: Final version, now using the Kelly et al. (2015) data [15] for normalization; 10 pages, 7 figures, 3 table

    Excitation function shape and neutron spectrum of the Li 7 ( p , n ) Be 7 reaction near threshold

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    The forward-emitted low energy tail of the neutron spectrum generated by the 7Li(p,n)7Be^{7}\mathrm{Li}(p,n)^{7}\mathrm{Be} reaction on a thick target at a proton energy of 1893.6 keV was measured by time-of-flight spectroscopy. The measurement was performed at BELINA (Beam Line for Nuclear Astrophysics) of the Laboratori Nazionali di Legnaro. Using the reaction kinematics and the proton on lithium stopping power the shape of the excitation function is calculated from the measured neutron spectrum. Good agreement with two reported measurements was found. Our data, along with the previous measurements, are well reproduced by the Breit-Wigner single-resonance formula for ss-wave particles. The differential yield of the reaction is calculated and the widely used neutron spectrum at a proton energy of 1912 keV was reproduced. Possible causes regarding part of the 6.5% discrepancy between the ^{197}\mathrm{Au}(n,\ensuremath{\gamma}) cross section measured at this energy by Ratynski and Kappeler [Phys. Rev. C 37, 595 (1988)] and the one obtained using the Evaluated Nuclear Data File version B-VII.1 are given

    Structural, Optical, Magnetic and Electrical Properties of Sputtered ZnO and ZnO:Fe Thin Films: The Role of Deposition Power

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    Structural, optical, magnetic, and electrical properties of zinc oxide (henceforth, ZO) and iron doped zinc oxide (henceforth, ZOFe) films deposited by sputtering technique are described by means of Rutherford backscattering spectrometry, grazing incidence X-ray diffraction, scanning electron microscope (SEM), UV–Vis spectrometer, vibrating sample magnetometer, and room temperature electrical conductivity, respectively. GIXRD analysis revealed that the films were polycrystalline with a hexagonal phase, and all films had a preferred (002) c-axis orientation. The lattice parameters a and c of the wurtzite structure were calculated for all films. The a parameter remains almost the same (around 3 Å), while c parameter varies slightly with increasing Fe content from 5.18 to 5.31 Å throughout the co-deposition process. The optical gap for undoped and doped ZO was obtained from different numerical methods based on the experimental data and it was increased with the increment of the concentration of Fe dopant from 3.26 eV to 3.35 eV. The highest magnetization (4.26 × 10−4 emu/g) and lowest resistivity (4.6 × 107 Ω·cm) values of the ZO films were found to be at an Fe content of 5% at. %. An explanation for the dependence of the optical, magnetic, and electrical properties of the samples on the Fe concentrations is also given. The enhanced magnetic properties such as saturated magnetization and coercivity with optical properties reveal that Fe doped ZO thin films are suitable for magneto-optoelectronic (optoelectronic and spintronics) device applications

    Structural, Optical, Magnetic and Electrical Properties of Sputtered ZnO and ZnO:Fe Thin Films: The Role of Deposition Power

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    Structural, optical, magnetic, and electrical properties of zinc oxide (henceforth, ZO) and iron doped zinc oxide (henceforth, ZOFe) films deposited by sputtering technique are described by means of Rutherford backscattering spectrometry, grazing incidence X-ray diffraction, scanning electron microscope (SEM), UV–Vis spectrometer, vibrating sample magnetometer, and room temperature electrical conductivity, respectively. GIXRD analysis revealed that the films were polycrystalline with a hexagonal phase, and all films had a preferred (002) c-axis orientation. The lattice parameters a and c of the wurtzite structure were calculated for all films. The a parameter remains almost the same (around 3 Å), while c parameter varies slightly with increasing Fe content from 5.18 to 5.31 Å throughout the co-deposition process. The optical gap for undoped and doped ZO was obtained from different numerical methods based on the experimental data and it was increased with the increment of the concentration of Fe dopant from 3.26 eV to 3.35 eV. The highest magnetization (4.26 × 10−4 emu/g) and lowest resistivity (4.6 × 107 Ω·cm) values of the ZO films were found to be at an Fe content of 5% at. %. An explanation for the dependence of the optical, magnetic, and electrical properties of the samples on the Fe concentrations is also given. The enhanced magnetic properties such as saturated magnetization and coercivity with optical properties reveal that Fe doped ZO thin films are suitable for magneto-optoelectronic (optoelectronic and spintronics) device applications

    Optimal geometric parameters of ordered arrays of nanoprisms for enhanced sensitivity in localized plasmon based sensors

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    Plasmonic sensors based on ordered arrays of nanoprisms are optimized in terms of their geometric parameters like size, height, aspect ratio for Au, Ag or Au0.5-Ag0.5 alloy to be used in the visible or near IR spectral range. The two figures of merit used for the optimization are the bulk and the surface sensitivity: the first is important for optimizing the sensing to large volume analytes whereas the latter is more important when dealing with small bio-molecules immobilized in close proximity to the nanoparticle surface. A comparison is made between experimentally obtained nanoprisms arrays and simulated ones by using Finite Elements Methods (FEM) techniques

    Emission Rate Modification and Quantum Efficiency Enhancement of Er3+Emitters by Near-Field Coupling with Nanohole Arrays

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    The control of the spontaneous emission properties of quantum emitters with limited losses by near-field coupling with plasmons-supporting nanostructures is one of the keys for next-generation high-efficiency and high-coherence plasmonic devices. In the present work, gold nanohole arrays are demonstrated to be an effective plasmonic system for controlling radiative rate and quantum efficiency of the 1540 nm emission of Er3+ ions embedded in silica. Finite element method electrodynamic simulations were used to describe the interaction between dipolar Er3+ emitters and the nanohole arrays. The results are in agreement with those of photoluminescence measurements performed in different coupling configurations. Particularly, we demonstrated that owing to the combination of strong emission enhancement and low level of ohmic losses in the metal, nanohole arrays are able to enhance the far-field photon yield up to 74%. This in turn is related to an extremely high far-field quantum efficiency: more than 90% of the emitted photons reach the far-field for the most efficient configurations investigated in which the extraordinary optical transmission peak of the nanohole array is matched with the Er3+ emission

    Correlation between in situ structural and optical characterization of the semiconductor-to-metal phase transition of VO2 thin films on sapphire

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    A detailed structural investigation of the semiconductor-to-metal transition (SMT) in vanadium dioxide thin films deposited on sapphire substrates by pulsed laser deposition was performed by in situ temperature-dependent X-ray diffraction (XRD) measurements. The structural results are correlated with those of infrared radiometry measurements in the SWIR (2.5-5 μm) and LWIR (8-10.6 μm) spectral ranges. The main results indicate a good agreement between XRD and optical analysis, therefore demonstrating that the structural transition from monoclinic to tetragonal phases is the dominating mechanism for controlling the global properties of the SMT transition. The picture that emerges is a SMT transition in which the two phases (monoclinic and tetragonal) coexist during the transition. Finally, the thermal hysteresis, measured for thin films with different thickness, showed a clear dependence of the transition temperature and the width of the hysteresis loop on the film thickness and on the size of the crystallites

    Double-Langmuir model for optimized nanohole array-based plasmonic biosensors

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    The sensing mechanism of plasmonic nanohole arrays is investigated and a novel model is proposed to interpret their optical response over a wide dynamic range of concentrations (10^-13 - 10^-5 M), based on a double- Langmuir model. This model describes the signal response of the analyte binding as the sum of two independent contributions which are related to two different surface regions of the biosensor, namely the top gold surface of the nanohole array and the lateral gold area inside the nanoholes. Numerical simulations highlight the different near-field behaviour of these two regions and their very different refractive index sensitivities, which both support the double-Langmuir model. This is corroborated by experimental biosensing measurements with gold nanohole arrays with hexagonal symmetry, synthesized by nanosphere lithography. Their sensing performances are optimized by numerical simulations by changing their geometrical parameters (i.e., lattice constant, nanohole diameter and height) in order to achieve a maximum sensitivity. For the biosensing experiments, the biotin-streptavidin complex is used as a benchmark test for the optimized nanohole array and a robust calibration is provided by the double-Langmuir model obtaining a limit of detection of 0.3 ng/mL, which corresponds to an absolute analyte quantity of 0.02 fmol
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