373 research outputs found
Cluster ionization via two-plasmon excitation
We calculate the two-photon ionization of clusters for photon energies near
the surface plasmon resonance. The results are expressed in terms of the
ionization rate of a double plasmon excitation, which is calculated
perturbatively. For the conditions of the experiment by Schlipper et al., we
find an ionization rate of the order of 0.05-0.10 fs^(-1). This rate is used to
determine the ionization probability in an external field in terms of the
number of photons absorbed and the duration of the field. The probability also
depends on the damping rate of the surface plasmon. Agreement with experiment
can only be achieved if the plasmon damping is considerably smaller than its
observed width in the room-temperature single-photon absorption spectrum.Comment: 17 pages and 6 PostScript figure
Anisotropic splitting of intersubband spin plasmons in quantum wells with bulk and structural inversion asymmetry
In semiconductor heterostructures, bulk and structural inversion asymmetry
and spin-orbit coupling induce a k-dependent spin splitting of valence and
conduction subbands, which can be viewed as being caused by momentum-dependent
crystal magnetic fields. This paper studies the influence of these effective
magnetic fields on the intersubband spin dynamics in an asymmetric n-type
GaAs/AlGaAs quantum well. We calculate the dispersions of intersubband spin
plasmons using linear response theory. The so-called D'yakonov-Perel'
decoherence mechanism is inactive for collective intersubband excitations,
i.e., crystal magnetic fields do not lead to decoherence of spin plasmons.
Instead, we predict that the main signature of bulk and structural inversion
asymmetry in intersubband spin dynamics is a three-fold, anisotropic splitting
of the spin plasmon dispersion. The importance of many-body effects is pointed
out, and conditions for experimental observation with inelastic light
scattering are discussed.Comment: 8 pages, 6 figure
Intersubband spin-density excitations in quantum wells with Rashba spin splitting
In inversion-asymmetric semiconductors, spin-orbit coupling induces a
k-dependent spin splitting of valence and conduction bands, which is a
well-known cause for spin decoherence in bulk and heterostructures.
Manipulating nonequilibrium spin coherence in device applications thus requires
understanding how valence and conduction band spin splitting affects carrier
spin dynamics. This paper studies the relevance of this decoherence mechanism
for collective intersubband spin-density excitations (SDEs) in quantum wells. A
density-functional formalism for the linear spin-density matrix response is
presented that describes SDEs in the conduction band of quantum wells with
subbands that may be non-parabolic and spin-split due to bulk or structural
inversion asymmetry (Rashba effect). As an example, we consider a 40 nm
GaAs/AlGaAs quantum well, including Rashba spin splitting of the conduction
subbands. We find a coupling and wavevector-dependent splitting of the
longitudinal and transverse SDEs. However, decoherence of the SDEs is not
determined by subband spin splitting, due to collective effects arising from
dynamical exchange and correlation.Comment: 10 pages, 4 figure
Thermodynamics as an alternative foundation for zero-temperature density functional theory and spin density functional theory
Thermodynamics provides a transparent definition of the free energy of
density functional theory (DFT), and of its derivatives - the potentials, at
finite temperatures T. By taking the T to 0 limit, it is shown here that both
DFT and spin-dependent DFT (for ground states) suffer from precisely the same
benign ambiguities: (a) charge and spin quantization lead to "up to a constant"
indeterminacies in the potential and the magnetic field respectively, and (b)
the potential in empty subspaces is undetermined but irrelevant. Surprisingly,
these simple facts were inaccessible within the standard formulation, leading
to recent discussions of apparent difficulties within spin-DFT.Comment: RevTeX, to appear in Phys. Rev.
Broken Symmetry in Density-Functional Theory: Analysis and Cure
We present a detailed analysis of the broken-symmetry mean-field solutions
using a four-electron rectangular quantum dot as a model system. Comparisons of
the density-functional theory predictions with the exact ones show that the
symmetry breaking results from the single-configuration wave function used in
the mean-field approach. As a general cure we present a scheme that
systematically incorporates several configurations into the density-functional
theory and restores the symmetry. This cure is easily applicable to any
density-functional approach.Comment: 4 pages, 4 figures, submitted to PR
Asymptotically exact dispersion relations for collective modes in a confined charged Fermi liquid
Using general local conservations laws we derive dispersion relations for
edge modes in a slab of electron liquid confined by a symmetric potential. The
dispersion relations are exact up to , where is a wave
vector and is an effective screening length. For a harmonic external
potential the dispersion relations are expressed in terms of the {\em exact}
static pressure and dynamic shear modulus of a homogeneous liquid with the
density taken at the slab core. We also derive a simple expression for the
frequency shift of the dipole (Kohn) modes in nearly parabolic quantum dots in
a magnetic field.Comment: RevTeX4, 4 pages. Revised version with new results on quantum qots
and wires. Published in Phys.Rev.
Self-consistent Overhauser model for the pair distribution function of an electron gas in dimensionalities D=3 and D=2
We present self-consistent calculations of the spin-averaged pair
distribution function for a homogeneous electron gas in the paramagnetic
state in both three and two dimensions, based on an extension of a model that
was originally proposed by A. W. Overhauser [Can. J. Phys. {\bf 73}, 683
(1995)] and further evaluated by P. Gori-Giorgi and J. P. Perdew [Phys. Rev. B
{\bf 64}, 155102 (2001)]. The model involves the solution of a two-electron
scattering problem via an effective Coulombic potential, that we determine
within a self-consistent Hartree approximation. We find numerical results for
that are in excellent agreement with Quantum Monte Carlo data at low and
intermediate coupling strength , extending up to in
dimensionality D=3. However, the Hartree approximation does not properly
account for the emergence of a first-neighbor peak at stronger coupling, such
as at in D=2, and has limited accuracy in regard to the spin-resolved
components and . We also
report calculations of the electron-electron s-wave scattering length, to test
an analytical expression proposed by Overhauser in D=3 and to present new
results in D=2 at moderate coupling strength. Finally, we indicate how this
approach can be extended to evaluate the pair distribution functions in
inhomogeneous electron systems and hence to obtain improved
exchange-correlation energy functionals.Comment: 14 pages, 7 figuers, to apear in Physical Review
Current-Density Functional Theory of the Response of Solids
The response of an extended periodic system to a homogeneous field (of
wave-vector ) cannot be obtained from a time-dependent density
functional theory (TDDFT) calculation, because the
Runge-Gross theorem does not apply. Time-dependent {\em current}-density
functional theory is needed and demonstrates that one key ingredient missing
from TDDFT is the macroscopic current. In the low-frequency limit, in certain
cases, density polarization functional theory is recovered and a formally exact
expression for the polarization functional is given.Comment: 5 pages, accepted in PR
Thermal Density Functional Theory in Context
This chapter introduces thermal density functional theory, starting from the
ground-state theory and assuming a background in quantum mechanics and
statistical mechanics. We review the foundations of density functional theory
(DFT) by illustrating some of its key reformulations. The basics of DFT for
thermal ensembles are explained in this context, as are tools useful for
analysis and development of approximations. We close by discussing some key
ideas relating thermal DFT and the ground state. This review emphasizes thermal
DFT's strengths as a consistent and general framework.Comment: Submitted to Spring Verlag as chapter in "Computational Challenges in
Warm Dense Matter", F. Graziani et al. ed
Expression analysis of the TAB2 protein in adult mouse tissues
Background: The Interleukin-1 (IL-1) signaling component TAK1 binding protein 2 (TAB2) plays a role in activating the NFκB and JNK signaling pathways. Additionally, TAB2 functions in the nucleus as a repressor of NFκB-mediated gene regulation. Objective: To obtain insight into the function of TAB2 in the adult mouse, we analyzed the in vivo TAB2 expression pattern. Materials and methods: Cell lines and adult mouse tissues were analyzed for TAB2 protein expression and localization. Results: Immunohistochemical staining for TAB2 protein revealed expression in the vascular endothelium of most tissues, hematopoietic cells and brain cells. While TAB2 is localized in both the nucleus and the cytoplasm in cell lines, cytoplasmic localization predominates in hematopoietic tissues in vivo. Conclusions: The TAB2 expression pattern shows striking similarities with previously reported IL-1 receptor expression and NFκB activation patterns, suggesting that TAB2 in vivo is playing a role in these signaling pathways
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