8 research outputs found
Dynamics of Excited Electrons in Copper and Ferromagnetic Transition Metals: Theory and Experiment
Both theoretical and experimental results for the dynamics of photoexcited
electrons at surfaces of Cu and the ferromagnetic transition metals Fe, Co, and
Ni are presented. A model for the dynamics of excited electrons is developed,
which is based on the Boltzmann equation and includes effects of
photoexcitation, electron-electron scattering, secondary electrons (cascade and
Auger electrons), and transport of excited carriers out of the detection
region. From this we determine the time-resolved two-photon photoemission
(TR-2PPE). Thus a direct comparison of calculated relaxation times with
experimental results by means of TR-2PPE becomes possible. The comparison
indicates that the magnitudes of the spin-averaged relaxation time \tau and of
the ratio \tau_\uparrow/\tau_\downarrow of majority and minority relaxation
times for the different ferromagnetic transition metals result not only from
density-of-states effects, but also from different Coulomb matrix elements M.
Taking M_Fe > M_Cu > M_Ni = M_Co we get reasonable agreement with experiments.Comment: 23 pages, 11 figures, added a figure and an appendix, updated
reference
Developing 1D nanostructure arrays for future nanophotonics
There is intense and growing interest in one-dimensional (1-D) nanostructures from the perspective of their synthesis and unique properties, especially with respect to their excellent optical response and an ability to form heterostructures. This review discusses alternative approaches to preparation and organization of such structures, and their potential properties. In particular, molecular-scale printing is highlighted as a method for creating organized pre-cursor structure for locating nanowires, as well as vaporâliquidâsolid (VLS) templated growth using nano-channel alumina (NCA), and deposition of 1-D structures with glancing angle deposition (GLAD). As regards novel optical properties, we discuss as an example, finite size photonic crystal cavity structures formed from such nanostructure arrays possessing highQand small mode volume, and being ideal for developing future nanolasers
Close coupling results for inelastic collisions of NH3 and Ar: a stringent test of a spectroscopic potential
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