Magnetic fluctuations in n-type high-TcT_c superconductors reveal breakdown of fermiology

By combining experimental measurements of the quasiparticle and dynamical magnetic properties of optimally electron-doped Pr$_{0.88}$LaCe$_{0.12}$CuO$_4$ with theoretical calculations we demonstrate that the conventional fermiology approach cannot possibly account for the magnetic fluctuations in these materials. In particular, we perform tunneling experiments on the very same sample for which a dynamical magnetic resonance has been reported recently and use photoemission data by others on a similar sample to characterize the fermionic quasiparticle excitations in great detail. We subsequently use this information to calculate the magnetic response within the conventional fermiology framework as applied in a large body of work for the hole-doped superconductors to find a profound disagreement between the theoretical expectations and the measurements: this approach predicts a step-like feature rather than a sharp resonance peak, it underestimates the intensity of the resonance by an order of magnitude, it suggests an unreasonable temperature dependence of the resonance, and most severely, it predicts that most of the spectral weight resides in incommensurate wings which are a key feature of the hole-doped cuprates but have never been observed in the electron-doped counterparts. Our findings strongly suggest that the magnetic fluctuations reflect the quantum-mechanical competition between antiferromagnetic and superconducting orders.Comment: 10 pages, 9 figures, 1 tabl

Magnetic quantum oscillations in YBa2_2Cu3_3O6.61_{6.61} and YBa2_2Cu3_3O6.69_{6.69} in fields of up to 85 T; patching the hole in the roof of the superconducting dome

We measure magnetic quantum oscillations in the underdoped cuprates YBa$_2$Cu$_3$O$_{6+x}$ with $x=0.61$, 0.69, using fields of up to 85 T. The quantum-oscillation frequencies and effective masses obtained suggest that the Fermi energy in the cuprates has a maximum at $p\approx 0.11-0.12$. On either side, the effective mass may diverge, possibly due to phase transitions associated with the T=0 limit of the metal-insulator crossover (low-$p$ side), and the postulated topological transition from small to large Fermi surface close to optimal doping (high $p$ side)

Influence of definition based versus pragmatic birth registration on international comparisons of perinatal and infant mortality: population based retrospective study

Objectives To examine variations in the registration of extremely low birthweight and early gestation births and to assess their effect on perinatal and infant mortality rankings of industrialised countries

No Ending Point in The Bragg-to-Vortex Glass Phase Transition Line at Low Temperatures

We have measured the magnetic hysteresis loops and the magnetic relaxation for $Bi_2Sr_2CaCu_2O_{8+\delta}$ (Bi-2212) single crystals which exhibit the second magnetization peak effect. Although no second peak effect is observed below 20 K in the measurement with fast field sweeping rate, it is found that the second peak effect will appear again after long time relaxation or in a measurement with very slow field sweeping rate at 16 K. It is anticipated that the peak effect will appear at very low temperatures (approaching zero K) when the relaxation time is long enough. We attribute this phenomenon to the profile of the interior magnetic field and conclude that the phase transition line of Bragg glass to vortex glass has no ending point at low temperatures.Comment: 4 pages, 5 figure

Electron-Spin Excitation Coupling in an Electron Doped Copper Oxide Superconductor

High-temperature (high-Tc) superconductivity in the copper oxides arises from electron or hole doping of their antiferromagnetic (AF) insulating parent compounds. The evolution of the AF phase with doping and its spatial coexistence with superconductivity are governed by the nature of charge and spin correlations and provide clues to the mechanism of high-Tc superconductivity. Here we use a combined neutron scattering and scanning tunneling spectroscopy (STS) to study the Tc evolution of electron-doped superconducting Pr0.88LaCe0.12CuO4-delta obtained through the oxygen annealing process. We find that spin excitations detected by neutron scattering have two distinct modes that evolve with Tc in a remarkably similar fashion to the electron tunneling modes in STS. These results demonstrate that antiferromagnetism and superconductivity compete locally and coexist spatially on nanometer length scales, and the dominant electron-boson coupling at low energies originates from the electron-spin excitations.Comment: 30 pages, 12 figures, supplementary information include

Influence of rotational distortions on Li⁺- and Na⁺- intercalation in anti-NASICON Fe₂(MoO₄)₃

Anti-NASICON Fe₂(MoO₄)₃ (<i>P</i>2₁/<i>c</i>) shows significant structural and electrochemical differences in the intercalation of Li⁺ and Na⁺ ions. To understand the origin of this behavior, we have used a combination of in situ X-ray and high-resolution neutron diffraction, total scattering, electrochemical measurements, density functional theory calculations, and symmetry-mode analysis. We find that for Li⁺-intercalation, which proceeds via a two-phase monoclinic-to-orthorhombic (<i>Pbcn</i>) phase transition, the host lattice undergoes a concerted rotation of rigid polyhedral subunits driven by strong interactions with the Li⁺ ions, leading to an ordered lithium arrangement. Na⁺-intercalation, which proceeds via a two-stage solid solution insertion into the monoclinic structure, similarly produces rotations of the lattice polyhedral subunits. However, using a combination of total neutron scattering data and density functional theory calculations, we find that while these rotational distortions upon Na⁺-intercalation are fundamentally the same as for Li⁺-intercalation, they result in a far less coherent final structure, with this difference attributed to the substantial difference between the ionic radii of the two alkali metals