585 research outputs found
High-order terms in the renormalized perturbation theory for the Anderson impurity model
We study the renormalized perturbation theory of the single-impurity Anderson
model, particularly the high-order terms in the expansion of the self-energy in
powers of the renormalized coupling . Though the presence of
counter-terms in the renormalized theory may appear to complicate the
diagrammatics, we show how these can be seamlessly accommodated by carrying out
the calculation order-by-order in terms of skeleton diagrams. We describe how
the diagrams pertinent to the renormalized self-energy and four-vertex can be
automatically generated, translated into integrals and numerically integrated.
To maximize the efficiency of our approach we introduce a generalized
-particle/hole propagator, which is used to analytically simplify the
resultant integrals and reduce the dimensionality of the integration. We
present results for the self-energy and spectral density to fifth order in
, for various values of the model asymmetry, and compare them to a
Numerical Renormalization Group calculation.Comment: 11 pages, 8 figure
Direct laser printing of thin-film polyaniline devices
We report the fabrication of electrically functional polyaniline thin-film
microdevices. Polyaniline films were printed in the solid phase by Laser
Induced Forward Transfer directly between Au electrodes on a Si/SiO2 substrate.
To apply solid-phase deposition, aniline was in situ polymerized on quartz
substrates. Laser deposition preserves the morphology of the films and delivers
sharp features with controllable dimensions. The electrical characteristics of
printed polyaniline present ohmic behavior, allowing for electroactive
applications. Results on gas sensing of ammonia are presented.Comment: In Pres
"My Invisalign experience" content, metrics and comment sentiment analysis of the most popular patient testimonials on YouTube
"My Invisalign experience" content, metrics and comment sentiment analysis of the most popular patient testimonials on YouTube
Dental Research Waste in Design, Analysis, and Reporting: A Scoping Review.
Research waste is highly prevalent across biomedical investigations. We aimed to assess the evidence on the extent of research waste in dental research. We performed a scoping review of empirical evaluations of dental studies assessing the prevalence and impact of limitations in design, conduct, analysis, and reporting of research. PubMed was searched using specific terms to retrieve studies dealing with design, conduct, analysis, and reporting of studies in dentistry, with no year or language restrictions. Of the 1,807 publications identified from the search and from manual searches, 71 were included in this review. The topic and article selection was based on the expert opinion of the authors. The existing evidence suggests that, although there are improvements over time, substantial deficiencies in all areas (design, conduct, analysis, reporting) were prevalent in dental research publications. Waste in research is a multifaceted problem without a simple solution. However, an appreciation of optimal research design and execution is a prerequisite and should be underpinned by policies that include appropriate training in research methods and properly aligned incentives
A simple model to estimate atmospheric concentrations of aerosol chemical species based on snow core chemistry at Summit, Greenland
A simple model is presented to estimate atmospheric concentrations of chemical species that exist primarily as aerosols based on snow core/ice core chemistry at Summit, Greenland. The model considers the processes of snow, fog, and dry deposition. The deposition parameters for each of the processes are estimated for SO42− and Ca2+ and are based on experiments conducted during the 1993 and 1994 summer field seasons. The seasonal mean atmospheric concentrations are estimated based on the deposition parameters and snow cores obtained during the field seasons. The ratios of the estimated seasonal mean airborne concentration divided by the measured mean concentration ( ) for SO42− over the 1993 and 1994 field seasons are 0.85 and 0.95, respectively. The ratios for Ca2+ are 0.45 and 0.90 for the 1993 and 1994 field seasons. The uncertainties in the estimated atmospheric concentrations range from 30% to 40% and are due to variability in the input parameters. The model estimates the seasonal mean atmospheric SO42− and Ca2+ concentrations to within 15% and 55%, respectively. Although the model is not directly applied to ice cores, the application of the model to ice core chemical signals is briefly discussed
Modeling of the processing and removal of trace gas and aerosol species by Arctic radiation fogs and comparison with measurements
A Lagrangian radiation fog model is applied to a fog event at Summit, Greenland. The model simulates the formation and dissipation of fog. Included in the model are detailed gas and aqueous phase chemistry, and deposition of chemical species with fog droplets. Model predictions of the gas phase concentrations of H2O2, HCOOH, SO2, and HNO3 as well as the fog fluxes of S(VI), N(V), H2O2, and water are compared with measurements. The predicted fluxes of S(VI), N(V), H2O2, and fog water generally agree with measured values. Model results show that heterogeneous SO2 oxidation contributes to approximately 40% of the flux of S(VI) for the modeled fog event, with the other 60% coming from preexisting sulfate aerosol. The deposition of N(V) with fog includes contributions from HNO3 and NO2 initially present in the air mass. HNO3 directly partitions into the aqueous phase to create N(V), and NO2 forms N(V) through reaction with OH and the nighttime chemistry set of reactions which involves N2O5 and water vapor. PAN contributes to N(V) by gas phase decomposition to NO2, and also by direct aqueous phase decomposition. The quantitative contributions from each path are uncertain since direct measurements of PAN and NO2 are not available for the fog event. The relative contributions are discussed based on realistic ranges of atmospheric concentrations. Model results suggest that in addition to the aqueous phase partitioning of the initial HNO3 present in the air mass, the gas phase decomposition of PAN and subsequent reactions of NO2 with OH as well as nighttime nitrate chemistry may play significant roles in depositing N(V) with fog. If a quasi-liquid layer exists on snow crystals, it is possible that the reactions taking place in fog droplets also occur to some extent in clouds as well as at the snow surface
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