Spherical magnetic nanoparticles: magnetic structure and interparticle interaction

The interaction between spherical magnetic nanoparticles is investigated from micromagnetic simulations and ananlysed in terms of the leading dipolar interaction energy between magnetic dipoles. We focus mainly on the case where the particles present a vortex structure. In a first step the local magnetic structure in the isolated particle is revisited. For particles bearing a uniaxial magnetocrystaline anisotropy, it is shown that the vortex core orientation relative to the easy axis depends on both the particle size and the anisotropy constant. When the particles magnetization present a vortex structure, it is shown that the polarization of the particles by the dipolar field of the other one must be taken into account in the interaction. An analytic form is deduced for the interaction which involves the vortex core magnetization and the magnetic susceptibility which are obtained from the magnetic properties of the isolated particle.Comment: 20 pages, 10 figures Published in Journal of Applied Physics. To be found at: http://link.aip.org/link/?jap/105/07391

Field-induced structure transformation in electrorheological solids

We have computed the local electric field in a body-centered tetragonal (BCT) lattice of point dipoles via the Ewald-Kornfeld formulation, in an attempt to examine the effects of a structure transformation on the local field strength. For the ground state of an electrorheological solid of hard spheres, we identified a novel structure transformation from the BCT to the face-centered cubic (FCC) lattices by changing the uniaxial lattice constant c under the hard sphere constraint. In contrast to the previous results, the local field exhibits a non-monotonic transition from BCT to FCC. As c increases from the BCT ground state, the local field initially decreases rapidly towards the isotropic value at the body-centered cubic lattice, decreases further, reaching a minimum value and increases, passing through the isotropic value again at an intermediate lattice, reaches a maximum value and finally decreases to the FCC value. An experimental realization of the structure transformation is suggested. Moreover, the change in the local field can lead to a generalized Clausius-Mossotti equation for the BCT lattices.Comment: Submitted to Phys. Rev.

Effects of geometric anisotropy on local field distribution: Ewald-Kornfeld formulation

We have applied the Ewald-Kornfeld formulation to a tetragonal lattice of point dipoles, in an attempt to examine the effects of geometric anisotropy on the local field distribution. The various problems encountered in the computation of the conditionally convergent summation of the near field are addressed and the methods of overcoming them are discussed. The results show that the geometric anisotropy has a significant impact on the local field distribution. The change in the local field can lead to a generalized Clausius-Mossotti equation for the anisotropic case.Comment: Accepted for publications, Journal of Physics: Condensed Matte

Polarizable molecular interactions in condensed phase and their equivalent nonpolarizable models

Earlier, using phenomenological approach, we showed that in some cases polarizable models of condensed phase systems can be reduced to nonpolarizable equivalent models with scaled charges. Examples of such systems include ionic liquids, TIPnP-type models of water, protein force fields, and others, where interactions and dynamics of inherently polarizable species can be accurately described by nonpolarizable models. To describe electrostatic interactions, the effective charges of simple ionic liquids are obtained by scaling the actual charges of ions by a factor of 1/sqrt(eps_el), which is due to electronic polarization screening effect; the scaling factor of neutral species is more complicated. Here, using several theoretical models, we examine how exactly the scaling factors appear in theory, and how, and under what conditions, polarizable Hamiltonians are reduced to nonpolarizable ones. These models allow one to trace the origin of the scaling factors, determine their values, and obtain important insights on the nature of polarizable interactions in condensed matter systems.Comment: 43 pages, 3 figure

Lattice-gas model for alkali-metal fullerides: face-centered-cubic structure

A lattice-gas model is suggested for describing the ordering phenomena in alkali-metal fullerides of face-centered-cubic structure assuming the electric charge of alkali ions residing in either octahedral or tetrahedral interstitial sites is completely screened by the first-neighbor C_60 molecules. This approximation allows us to derive an effective ion-ion interaction. The van der Waals interaction between the ion and C_60 molecule is characterized by introducing an additional energy at the tetrahedral sites. This model is investigated by using a three-sublattice mean-field approximation and a simple cluster-variation method. The analysis shows a large variety of phase diagrams when changing the site energy parameter.Comment: 10 twocolumn pages (REVTEX) including 12 PS figure

Multi-band optical-NIR variability of blazars on diverse timescales

To search for optical variability on a wide range of timescales, we have carried out photometric monitoring of two flat spectrum radio quasars, 3C 454.3 and 3C 279, plus one BL Lac, S5 0716+714, all of which have been exhibiting remarkably high activity and pronounced variability at all wavelengths. CCD magnitudes in B, V, R and I pass-bands were determined for $\sim$ 7000 new optical observations from 114 nights made during 2011 - 2014, with an average length of $\sim$ 4 h each, at seven optical telescopes: four in Bulgaria, one in Greece, and two in India. We measured multiband optical flux and colour variations on diverse timescales. Discrete correlation functions were computed among B, V, R, and I observations, to search for any time delays. We found weak correlations in some cases with no significant time lags. The structure function method was used to estimate any characteristic time-scales of variability. We also investigated the spectral energy distribution of the three blazars using B, V, R, I, J and K pass-band data. We found that the sources almost always follows a bluer-when-brighter trend. We discuss possible physical causes of the observed spectral variability.Comment: Accepted for publication in MNRAS, 16 pages, 11 figures, 5 tables, plus supplementary material containing additional figures and tables (please contact authors for it

The prompt X-ray emission of GRB011211: possible evidence of a transient absorption feature

We report on observation results of the prompt X- and gamma-ray emission from GRB011211. This event was detected with the Gamma-Ray Burst Monitor and one of the Wide Field Cameras aboard the BeppoSAX satellite. The optical counterpart to the GRB was soon identified and its redshift determined (z = 2.140), while with the XMM-Newton satellite, the X-ray afterglow emission was detected. Evidence of soft X-ray emission lines was reported by Reeves et al. (2002), but not confirmed by other authors. In investigating the spectral evolution of the prompt emission we find the possible evidence of a transient absorption feature at 6.9^{+0.6}_{-0.5} keV during the rise of the primary event. The significance of the feature is derived with non parametric tests and numerical simulations, finding a chance probability which ranges from 3x10^{-3} down to 4x10^{-4}. The feature shows a Gaussian profile and an equivalent width of 1.2^{+0.5}_{-0.6} keV. We discuss our results and their possible interpretation.Comment: 23 pages, 3 Tables, 6 Figures. Accepted for publication in Astrophysical Journa

The X-ray afterglow of the Gamma-ray burst of May 8, 1997: spectral variability and possible evidence of an iron line

We report the possible detection (99.3% of statistical significance) of redshifted Fe iron line emission in the X-ray afterglow of Gamma-ray burst GRB970508 observed by BeppoSAX. Its energy is consistent with the redshift of the putative host galaxy determined from optical spectroscopy. The line disappeared about 1 day after the burst. We have also analyzed the spectral variability during the outburst event that characterizes the X-ray afterglow of this GRB. The spectrum gets harder during the flare, turning to steep when the flux decreases. The variability, intensity and width of the line indicate that the emitting region should have a mass approximately greater than 0.5 solar masses (assuming the iron abundance similar to its solar value), a size of about 3 times 10^15 cm, be distributed anisotropically, and be moving with sub-relativistic speed. In contrast to the fairly clean environment expected in the merging of two neutron stars, the observed line properties would imply that the site of the burst is embedded in a large mass of material, consistent with pre-explosion ejecta of a very massive star. This material could be related with the outburst observed in the afterglow 1 day after the GRB and with the spectral variations measured during this phase.Comment: To appear in The Astrophysical Journal Letters, AASTEX LateX, 2 PostScript figure

The Temperature Distribution in Turbulent Interstellar Gas

We discuss the temperature distribution in a two-dimensional, thermally unstable numerical simulation of the warm and cold gas in the Galactic disk, including the magnetic field, self-gravity, the Coriolis force, stellar energy injection and a realistic cooling function. We find that ~50% of the turbulent gas mass has temperatures in what would be the thermally unstable range if thermal instability were to be considered alone. This appears to be a consequence of there being many other forces at play than just thermal pressure. We also point out that a bimodal temperature pdf is a simple consequence of the form of the interstellar cooling function and is not necessarily a signature of discontinuous phase transitions.Comment: video address has been update

Spin-boson models for quantum decoherence of electronic excitations of biomolecules and quantum dots in a solvent

We give a theoretical treatment of the interaction of electronic excitations (excitons) in biomolecules and quantum dots with the surrounding polar solvent. Significant quantum decoherence occurs due to the interaction of the electric dipole moment of the solute with the fluctuating electric dipole moments of the individual molecules in the solvent. We introduce spin boson models which could be used to describe the effects of decoherence on the quantum dynamics of biomolecules which undergo light-induced conformational change and on biomolecules or quantum dots which are coupled by Forster resonant energy transfer.Comment: More extended version, to appear in Journal of Physics: Condensed Matter. 13 pages, 3 figure