Revealing the Exciton Fine Structure in PbSe Nanocrystal Quantum Dots

We measure the photoluminescence (PL) lifetime, $\tau$, of excitons in colloidal PbSe nanocrystals (NCs) at low temperatures to 270~mK and in high magnetic fields to 15~T. For all NCs (1.3-2.3~nm radii), $\tau$ increases sharply below 10~K but saturates by 500~mK. In contrast to the usual picture of well-separated ``bright" and ``dark" exciton states (found, e.g., in CdSe NCs), these dynamics fit remarkably well to a system having two exciton states with comparable - but small - oscillator strengths that are separated by only 300-900 $\mu$eV. Importantly, magnetic fields reduce $\tau$ below 10~K, consistent with field-induced mixing between the two states. Magnetic circular dichroism studies reveal exciton g-factors from 2-5, and magneto-PL shows $>$10\% circularly polarized emission.Comment: To appear in Physical Review Letter

Cosmic ray results on the A dependence of multiplicity and angular distributions in proton nuclear interactions above 100 GeV

A calorimeter-spark chamber system was used to collect data on several hundred proton-nucleus interactions above 100 GeV using targets of C, Al, Fe, Sn and Pb. The average charged prong multiplicity is found to depend on atomic mass number as nc> = nc>(p-p)Ax where X = 0.129 +/- 0.004, with the dominant increase in multiplicity occuring in the backward (p-p c.m.) hemisphere. The value of x shows no significant energy dependence.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/22150/1/0000579.pd

Subdiffraction, Luminescence-Depletion Imaging of Isolated, Giant, CdSe/CdS Nanocrystal Quantum Dots

Subdiffraction spatial resolution luminescence depletion imaging was performed with giant CdSe/14CdS nanocrystal quantum dots (g-NQDs) dispersed on a glass slide. Luminescence depletion imaging used a Gaussian shaped excitation laser pulse overlapped with a depletion pulse, shaped into a doughnut profile, with zero intensity in the center. Luminescence from a subdiffraction volume is collected from the central portion of the excitation spot, where no depletion takes place. Up to 92% depletion of the luminescence signal was achieved. An average full width at half-maximum of 40 ± 10 nm was measured in the lateral direction for isolated g-NQDs at an air interface using luminescence depletion imaging, whereas the average full width at half-maximum was 450 ± 90 nm using diffraction-limited, confocal luminescence imaging. Time-gating of the luminescence depletion data was required to achieve the stated spatial resolution. No observable photobleaching of the g-NQDs was present in the measurements, which allowed imaging with a dwell time of 250 ms per pixel to obtain images with a high signal-to-noise ratio. The mechanism for luminescence depletion is likely stimulated emission, stimulated absorption, or a combination of the two. The g-NQDs fulfill a need for versatile, photostable tags for subdiffraction imaging schemes where high laser powers or long exposure times are used

Sample-Averaged Biexciton Quantum Yield Measured by Solution-Phase Photon Correlation

The brightness of nanoscale optical materials such as semiconductor nanocrystals is currently limited in high excitation flux applications by inefficient multiexciton fluorescence. We have devised a solution-phase photon correlation measurement that can conveniently and reliably measure the average biexciton-to-exciton quantum yield ratio of an entire sample without user selection bias. This technique can be used to investigate the multiexciton recombination dynamics of a broad scope of synthetically underdeveloped materials, including those with low exciton quantum yields and poor fluorescence stability. Here, we have applied this method to measure weak biexciton fluorescence in samples of visible-emitting InP/ZnS and InAs/ZnS core/shell nanocrystals, and to demonstrate that a rapid CdS shell growth procedure can markedly increase the biexciton fluorescence of CdSe nanocrystals.United States. Dept. of Energy. Office of Basic Energy Sciences (DE-FG02-07ER46454)United States. Dept. of Energy. Office of Basic Energy Sciences (DE-SC0001088)National Institutes of Health (U.S.) (9P41EB015871-26A1

Point-contact spectra of the heavy-fermion superconductors U Be

We have measured the current-voltage characteristics of point contacts between UBe13 or UPt3 and the normal metals W or Pt (metallic point contacts) or GaAs (Schottky-barrier tunneling contact) in the temperature range between 50 mK and 1 K. In the metal-point-contact characteristics (dVdI vs V) there appear zero-bias minima of width 2 below Tc. The ratio 2 kBTc is close to the BCS value. The tunneling spectra of UPt3 exhibit weak additional structure below Tc. A value 2 has been estimated, which is a factor of 2 larger than that for the metal point contacts. © 1987 The American Physical Society

The properties of proton-proton interactions between 100 and 1000 GeV from a cosmic-ray experiment

Proton-proton interactions above 100 GeV have been studied in an experiment using cosmic-ray protons interacting in a liquid hydrogen target. From several hundred hydrogen interactions, it has been learned that: (a) the total inelastic pp cross section is not changing significantly with energy above 30 GeV; (b) the multiplicity distributions of charged prongs agree with a Poisson distribution in charged-particle pairs; (c) the average charged prong multiplicity increases as 1 n s; (d) the angular distribution of charged particles agrees with a c.m. momentum distribution of charged particles that varies as exp exp [-8 pT2-8x2] d3p/E (where X = pL/po) and a nucleon distribution that varies as 10x exp [-3 pT2] d3p/E for 0.05 < x < 0.85. Further properties of the angular distributions, characteristics of the ionization calorimeter, the cross section in iron, and other features of the data are reported.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/34084/1/0000363.pd

Proton-proton interactions above 100GeV : technical report

http://deepblue.lib.umich.edu/bitstream/2027.42/5795/5/bac5749.0001.001.pdfhttp://deepblue.lib.umich.edu/bitstream/2027.42/5795/4/bac5749.0001.001.tx