1,644 research outputs found
The effect of Aharanov-Bohm phase on the magnetic-field dependence of two-pulse echos in glasses at low temperatures
The anomalous response of glasses in the echo amplitude experiment is
explained in the presence of a magnetic field. We have considered the low
energy excitations in terms of an effective two level system. The effective
model is constructed on the flip-flop configuration of two interacting two
level systems. The magnetic field affects the tunneling amplitude through the
Aharanov-Bohm effect. The effective model has a lower scale of energy in
addition to the new distribution of tunneling parameters which depend on the
interaction. We are able to explain some features of echo amplitude versus a
magnetic field, namely, the dephasing effect at low magnetic fields, dependence
on the strength of the electric field, pulse separation effect and the
influence of temperature. However this model fails to explain the isotope
effects which essentially can be explained by the nuclear quadrupole moment. We
will finally discuss the features of our results.Comment: 8 pages, 7 figure
Low temperature breakdown of coherent tunneling in amorphous solids induced by the nuclear quadrupole interaction
We consider the effect of the internal nuclear quadrupole interaction on
quantum tunneling in complex multi-atomic two-level systems. Two distinct
regimes of strong and weak interactions are found. The regimes depend on the
relationship between a characteristic energy of the nuclear quadrupole
interaction and a bare tunneling coupling strength
. When , the internal interaction is
negligible and tunneling remains coherent determined by . When
, coherent tunneling breaks down and an effective
tunneling amplitude decreases by an exponentially small overlap factor
between internal ground states of left and right wells of a
tunneling system. This affects thermal and kinetic properties of tunneling
systems at low temperatures . The theory is applied for
interpreting the anomalous behavior of the resonant dielectric susceptibility
in amorphous solids at low temperatures mK where the nuclear
quadrupole interaction breaks down coherent tunneling. We suggest the
experiments with external magnetic fields to test our predictions and to
clarify the internal structure of tunneling systems in amorphous solids.Comment: To appear in the Physical Review
Effect of Nuclear Quadrupole Interaction on the Relaxation in Amorphous Solids
Recently it has been experimentally demonstrated that certain glasses display
an unexpected magnetic field dependence of the dielectric constant. In
particular, the echo technique experiments have shown that the echo amplitude
depends on the magnetic field. The analysis of these experiments results in the
conclusion that the effect seems to be related to the nuclear degrees of
freedom of tunneling systems. The interactions of a nuclear quadrupole
electrical moment with the crystal field and of a nuclear magnetic moment with
magnetic field transform the two-level tunneling systems inherent in amorphous
dielectrics into many-level tunneling systems. The fact that these features
show up at temperatures , where the properties of amorphous materials
are governed by the long-range interaction between tunneling systems,
suggests that this interaction is responsible for the magnetic field dependent
relaxation. We have developed a theory of many-body relaxation in an ensemble
of interacting many-level tunneling systems and show that the relaxation rate
is controlled by the magnetic field. The results obtained correlate with the
available experimental data. Our approach strongly supports the idea that the
nuclear quadrupole interaction is just the key for understanding the unusual
behavior of glasses in a magnetic field.Comment: 18 pages, 9 figure
Tunneling dynamics of side chains and defects in proteins, polymer glasses, and OH-doped network glasses
Simulations on a Lennard-Jones computer glass are performed to study effects
arising from defects in glasses at low temperatures. The numerical analysis
reveals that already a low concentration of defects may dramatically change the
low temperature properties by giving rise to extrinsic double-well potentials
(DWP's). The main characteristics of these extrinsic DWP's are (i) high barrier
heights, (ii) high probability that a defect is indeed connected with an
extrinsic DWP, (iii) highly localized dynamics around this defect, and (iv)
smaller deformation potential coupling to phonons. Designing an extension of
the Standard Tunneling Model (STM) which parametrizes this picture and
comparing with ultrasound experiments on the wet network glass -BO
shows that effects of OH-impurities are accurately accounted for. This model is
then applied to organic polymer glasses and proteins. It is suggested that side
groups may act similarly like doped impurities inasmuch as extrinsic DWP's are
induced, which possess a distribution of barriers peaked around a high barrier
height. This compares with the structurlessly distributed barrier heights of
the intrinsic DWP's, which are associated with the backbone dynamics. It is
shown that this picture is consistent with elastic measurements on polymers,
and can explain anomalous nonlogarithmic line broadening recently observed in
hole burning experiments in PMMA.Comment: 34 pages, Revtex, 9 eps-figures, accepted for publication in J. Chem.
Phy
Damping and decoherence of a nanomechanical resonator due to a few two level systems
We consider a quantum model of a nanomechanical flexing beam resonator
interacting with a bath comprising a few damped tunneling two level systems
(TLS's). In contrast with a resonator interacting bilinearly with an ohmic free
oscillator bath (modeling clamping loss, for example), the mechanical resonator
damping is amplitude dependent, while the decoherence of quantum superpositions
of mechanical position states depends only weakly on their spatial separation
Low temperature dipolar echo in amorphous dielectrics: Significance of relaxation and decoherence free two level systems
The nature of dielectric echoes in amorphous solids at low temperatures is
investigated. It is shown that at long delay times the echo amplitude is
determined by a small subset of two level systems (TLS) having negligible
relaxation and decoherence because of their weak coupling to phonons. The echo
decay can then be described approximately by power law time dependencies with
different powers at times longer and shorter than the typical TLS relaxation
time. The theory is applied to recent measurements of two and three pulse
dipolar echo in borosilicate glass BK7 and provides a perfect data fit in the
broad time and temperature ranges under the assumption that there exist two TLS
relaxation mechanisms due to TLS-phonons and TLS-TLS interaction. This
interpretation is consistent with the previous experimental and theoretical
investigations. Further experiments verifying the theory predictions are
suggested.Comment: 10 pages, 8 figure
Slow relaxation of conductance of amorphous hopping insulators
We discuss memory effects in the conductance of hopping insulators due to
slow rearrangements of structural defects leading to formation of polarons
close to the electron hopping states. An abrupt change in the gate voltage and
corresponding shift of the chemical potential change populations of the hopping
sites, which then slowly relax due to rearrangements of structural defects. As
a result, the density of hopping states becomes time dependent on a scale
relevant to rearrangement of the structural defects leading to the excess time
dependent conductivity.Comment: 6 pages, 1 figur
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