254 research outputs found

    Transfer of spectral weight across the gap of Sr2IrO4 induced by La doping

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    We study with Angle Resolved PhotoElectron Spectroscopy (ARPES) the evolution of the electronic structure of Sr2IrO4, when holes or electrons are introduced, through Rh or La substitutions. At low dopings, the added carriers occupy the first available states, at bottom or top of the gap, revealing an anisotropic gap of 0.7eV in good agreement with STM measurements. At further doping, we observe a reduction of the gap and a transfer of spectral weight across the gap, although the quasiparticle weight remains very small. We discuss the origin of the in-gap spectral weight as a local distribution of gap values

    Role of dynamic Jahn-Teller distortions in Na2C60 and Na2CsC60 studied by NMR

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    Through 13C NMR spin lattice relaxation (T1) measurements in cubic Na2C60, we detect a gap in its electronic excitations, similar to that observed in tetragonal A4C60. This establishes that Jahn-Teller distortions (JTD) and strong electronic correlations must be considered to understand the behaviour of even electron systems, regardless of the structure. Furthermore, in metallic Na2CsC60, a similar contribution to T1 is also detected for 13C and 133Cs NMR, implying the occurence of excitations typical of JT distorted C60^{2-} (or equivalently C60^{4-}). This supports the idea that dynamic JTD can induce attractive electronic interactions in odd electron systems.Comment: 3 figure

    Mn local moments prevent superconductivity in iron-pnictides Ba(Fe 1-x Mn x)2As2

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    75As nuclear magnetic resonance (NMR) experiments were performed on Ba(Fe1-xMnx)2As2 (xMn = 2.5%, 5% and 12%) single crystals. The Fe layer magnetic susceptibility far from Mn atoms is probed by the75As NMR line shift and is found similar to that of BaFe2As2, implying that Mn does not induce charge doping. A satellite line associated with the Mn nearest neighbours (n.n.) of 75As displays a Curie-Weiss shift which demonstrates that Mn carries a local magnetic moment. This is confirmed by the main line broadening typical of a RKKY-like Mn-induced staggered spin polarization. The Mn moment is due to the localization of the additional Mn hole. These findings explain why Mn does not induce superconductivity in the pnictides contrary to other dopants such as Co, Ni, Ru or K.Comment: 6 pages, 7 figure

    Evidence for distinct polymer chain orientations in KC60 and RbC60

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    The KC60 and RbC60 polymer phases exhibit contrasting electronic properties while powder diffraction studies have revealed no definite structural difference. We have performed single crystal X-ray diffraction and diffuse scattering studies of these compounds. It is found that KC60 and RbC60 possess different chain orientations about their axes, which are described by distinct space groups Pmnn and I2/m, respectively. Such a structural difference will be of great importance to a complete understanding of the physical properties.Comment: To be published in Phys. Rev. Let

    Nouveau décodeur à complexité réduite pour codes convolutifs de rendement 1/2

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    Les codes convolutifs peuvent être décodés de façon optimale à l'aide l'algorithme de Viterbi (VA). Nous proposons un décodeur à entrée souple dans lequel l'algorithme de Viterbi est employé pour identifier le vecteur d'erreur plutôt que le message d'information avec une métrique appropriée. Ce type de décodage permet d'éviter la mise en oeuvre d'un nombre important d'opérations ACS (Add Compare Select). Nous montrons que les performances atteintes sont proches de l'optimum tout en bénéficiant d'une réduction de la complexité qui est d'autant plus importante que le rapport signal à bruit (SNR) est favorable. Par exemple, pour des SNR supérieurs à 3 dB et dans le cas d'une transmission avec la modulation BPSK sur canal gaussien, au moins 88% des ACS peuvent être évités

    Interplay of Superconductivity and Fermi-Liquid Transport in Rh-Doped CaFe2As2 with Lattice-Collapse Transition

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    Ca(Fe1−x_{1-x}Rhx_x)2_2As2_2 undergoes successive phase transitions with increasing Rh doping in the TT == 0 limit. The antiferromagnetic-metal phase with orthorhombic structure at 0.00 ≤\le xx ≤\le 0.020 is driven to a superconducting phase with uncollapsed-tetragonal (ucT) structure at 0.020 ≤\le xx ≤\le 0.024; a non-superconducting collapsed-tetragonal (cT) phase takes over at xx ≥\geq 0.024. The breakdown of Fermi-liquid transport is observed in the ucT phase above TcT_{\rm c}. In the adjacent cT phase, Fermi-liquid transport is restored along with a disappearance of superconductivity. This interplay of superconductivity and Fermi-liquid transport suggests the essential role of magnetic fluctuations in the emergence of superconductivity in doped CaFe2_2As2_2.Comment: 11 pages, 4 figure

    Coexistence of Superconductivity and Charge Density Wave in SrPt2As2

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    SrPt2As2 is a novel arsenide superconductor, which crystallizes in the CaBe2Ge2-type structure as a different polymorphic form of the ThCr2Si2-type structure. SrPt2As2 exhibits a charge-density-wave (CDW) ordering at about 470 K and enters into a superconducting state at Tc = 5.2 K. The coexistence of superconductivity and CDW refers to Peierls instability with a moderately strong electron-phonon interaction. Thus SrPt2As2 can be viewed as a nonmagnetic analog of iron-based superconductors, such as doped BaFe2As2, in which superconductivity emerges in close proximity to spin-density-wave ordering.Comment: 4 pages, 5 figure

    Evidence for Insulating Behavior in the Electric Conduction of (NH3_3)K3_3C60_{60} Systems

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    Microwave study using cavity perturbation technique revealed that the conductivity of antiferromagnet (NH3_3)K3−x_{3-x}Rbx_xC60_{60} at 200K is already 3-4 orders of magnitude smaller than those of superconductors, K3_3C60_{60} and (NH3_3)x_xNaRb2_2C60_{60}, and that the antiferromagnetic compounds are {\it insulators} below 250K without metal-insulator transitions. The striking difference in the magnitude of the conductivity between these materials strongly suggests that the Mott-Hubbard transition in the ammoniated alkali fullerides is driven by a reduction of lattice symmetry from face-centered-cubic to face-centered-orthorhombic, rather than by the magnetic ordering.Comment: accepted for publication in PR

    (pi,pi)-electronic order in iron arsenide superconductors

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    The distribution of valence electrons in metals usually follows the symmetry of an ionic lattice. Modulations of this distribution often occur when those electrons are not stable with respect to a new electronic order, such as spin or charge density waves. Electron density waves have been observed in many families of superconductors[1-3], and are often considered to be essential for superconductivity to exist[4]. Recent measurements[5-9] seem to show that the properties of the iron pnictides[10, 11] are in good agreement with band structure calculations that do not include additional ordering, implying no relation between density waves and superconductivity in those materials[12-15]. Here we report that the electronic structure of Ba1-xKxFe2As2 is in sharp disagreement with those band structure calculations[12-15], instead revealing a reconstruction characterized by a (pi,pi) wave vector. This electronic order coexists with superconductivity and persists up to room temperature
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