Magnetic critical properties and basal-plane anisotropy of Sr2_2IrO4_4

The anisotropic magnetic properties of Sr$_2$IrO$_4$ are investigated, using longitudinal and torque magnetometry. The critical scaling across $T_c$ of the longitudinal magnetization is the one expected for the 2D XY universality class. Modeling the torque for a magnetic field in the basal-plane, and taking into account all in-plane and out-of-plane magnetic couplings, we derive the effective 4-fold anisotropy $K_4 \approx$ 1 10$^5$ erg mole$^{-1}$. Although larger than for the cuprates, it is found too small to account for a significant departure from the isotropic 2D XY model. The in-plane torque also allows us to put an upper bound for the anisotropy of a field-induced shift of the antiferromagnetic ordering temperature

Gaps and excitations in fullerides with partially filled bands : NMR study of Na2C60 and K4C60

We present an NMR study of Na2C60 and K4C60, two compounds that are related by electron-hole symmetry in the C60 triply degenerate conduction band. In both systems, it is known that NMR spin-lattice relaxation rate (1/T1) measurements detect a gap in the electronic structure, most likely related to singlet-triplet excitations of the Jahn-Teller distorted (JTD) C60^{2-} or C60^{4-}. However, the extended temperature range of the measurements presented here (10 K to 700 K) allows to reveal deviations with respect to this general trend, both at high and low temperatures. Above room temperature, 1/T1 deviates from the activated law that one would expect from the presence of the gap and saturates. In the same temperature range, a lowering of symmetry is detected in Na2C60 by the appearance of quadrupole effects on the 23Na spectra. In K4C60, modifications of the 13C spectra lineshapes also indicate a structural modification. We discuss this high temperature deviation in terms of a coupling between JTD and local symmetry. At low temperatures, 1/T$_1$T tends to a constant value for Na2C60, both for 13C and 23Na NMR. This indicates a residual metallic character, which emphasizes the proximity of metallic and insulting behaviors in alkali fullerides.Comment: 12 pages, 13 figure

Oriented gap opening in the magnetically ordered state of Iron-pnicitides: an impact of intrinsic unit cell doubling on the FeFe square lattice by AsAs atoms

We show that the complicated band reconstruction near Fermi surfaces in the magnetically ordered state of iron-pnictides observed by angle-resolved photoemission spectroscopies (ARPES) can be understood in a meanfield level if the \emph{intrinsic unit cell doubling} due to As atoms is properly considered as shown in the recently constructed S$_{4}$ microscopic effective model. The (0,$\pi$) or ($\pi$,0) col-linear antiferromagnetic (C-AFM) order does not open gaps between two points at Fermi surfaces linked by the ordered wave vector but forces a band reconstruction involving four points in unfolded Brillouin zone (BZ) and gives rise to small pockets or hot spots. The S$_4$ symmetry naturally chooses a staggered orbital order over a ferro-orbital order to coexist with the C-AFM order. These results strongly suggest that the kinematics based on the S$_{4}$ symmetry captures the essential low energy physics of iron-based superconductors.Comment: 5 figures, 5 page

Sr 2 IrO 4 magnetic phase diagram, from resistivity

International audienceWe show that the transition to the antiferromagnetic state in zero magnetic field does show up in the transverse resistivity, for which we point out the possibility for a direct spin orientation effect. In an applied field, we propose that the transition is split into two lines, corresponding to in-plane and out-of-plane magnetic ordering. This picture is corroborated by transverse magnetization measurements. The magnetic phase diagram for Sr2IrO4 was investigated, using the angular dependence of the resistivity transverse to the IrO2 planes