27 research outputs found

    The approach to a superconductor-to-Bose-insulator transition in disordered films

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    Through a detailed study of scaling near the magnetic field-tuned superconductor-to-insulator transition in strongly disordered films, we find that results for a variety of materials can be collapsed onto a single phase diagram. The data display two clear branches, one with weak disorder and an intervening metallic phase, the other with strong disorder. Along the strongly disordered branch, the resistance at the critical point approaches RQ=h/4e2R_Q = h/4e^2 and the scaling of the resistance is consistent with quantum percolation, and therefore with the predictions of the dirty boson model.Comment: 4 pages, 4 figure

    Resonant x-ray scattering reveals possible disappearance of magnetic order under hydrostatic pressure in the Kitaev candidate γ\gamma-Li2_2IrO3_3

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    Honeycomb iridates such as γ\gamma-Li2_2IrO3_3 are argued to realize Kitaev spin-anisotropic magnetic exchange, along with Heisenberg and possibly other couplings. While systems with pure Kitaev interactions are candidates to realize a quantum spin liquid ground state, in γ\gamma-Li2_2IrO3_3 it has been shown that the balance of magnetic interactions leads to the incommensurate spiral spin order at ambient pressure below 38 K. We study the fragility of this state in single crystals of γ\gamma-Li2_2IrO3_3 using resonant x-ray scattering (RXS) under applied hydrostatic pressures of up to 3.0 GPa. RXS is a direct probe of the underlying electronic order, and we observe the abrupt disappearance of the qq=(0.57, 0, 0) spiral order at a critical pressure Pc=1.5 P_c = 1.5\ GPa with no accompanying change in the symmetry of the lattice. This dramatic disappearance is in stark contrast with recent studies of β\beta-Li2_2IrO3_3 that show continuous suppression of the spiral order in magnetic field; under pressure, a new and possibly nonmagnetic ground state emerges

    Weak antilocalization and disorder-enhanced electron interactions in crystalline GeSbTe

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    Phase change materials can be reversibly switched between amorphous and crystalline states and often show strong contrast in the optical and electrical properties of these two phases. They are now in widespread use for optical data storage, and their fast switching and a pronounced change of resistivity upon crystallization are also very attractive for nonvolatile electronic data storage. Nevertheless there are still several open questions regarding the electronic states and charge transport in these compounds. In this work we study electrical transport in thin metallic films of the disordered, crystalline phase change material Ge1_1Sb2_2Te4_4. We observe weak antilocalization and disorder enhanced Coulomb interaction effects at low temperatures, and separate the contributions of these two phenomena to the temperature dependence of the resistivity, Hall effect, and magnetoresistance. Strong spin-orbit scattering causes positive magnetoresistance at all temperatures, and a careful analysis of the low-field magnetoresistance allows us to extract the temperature dependent electron dephasing rate and study other scattering phenomena. We find electron dephasing due to inelastic electron-phonon scattering at higher temperatures, electron-electron scattering dephasing at intermediate temperatures, and a crossover to weak temperature dependence below 1 K

    A new spin-anisotropic harmonic honeycomb iridate

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    The physics of Mott insulators underlies diverse phenomena ranging from high temperature superconductivity to exotic magnetism. Although both the electron spin and the structure of the local orbitals play a key role in this physics, in most systems these are connected only indirectly --- via the Pauli exclusion principle and the Coulomb interaction. Iridium-based oxides (iridates) open a further dimension to this problem by introducing strong spin-orbit interactions, such that the Mott physics has a strong orbital character. In the layered honeycomb iridates this is thought to generate highly spin-anisotropic interactions, coupling the spin orientation to a given spatial direction of exchange and leading to strongly frustrated magnetism. The potential for new physics emerging from such interactions has driven much scientific excitement, most recently in the search for a new quantum spin liquid, first discussed by Kitaev \cite{kitaev_anyons_2006}. Here we report a new iridate structure that has the same local connectivity as the layered honeycomb, but in a three-dimensional framework. The temperature dependence of the magnetic susceptibility exhibits a striking reordering of the magnetic anisotropy, giving evidence for highly spin-anisotropic exchange interactions. Furthermore, the basic structural units of this material suggest the possibility of a new family of structures, the `harmonic honeycomb' iridates. This compound thus provides a unique and exciting glimpse into the physics of a new class of strongly spin-orbit coupled Mott insulators.Comment: 12 pages including bibliography, 5 figure
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