14 research outputs found
Comment on "Short-range magnetic interactions in the spin-ice compound Ho2Ti2O7"
In their recent communication (Phys. Rev. B 64, 060406(R) (2001)) Cornelius
and Gardner have reported the results of magnetization and susceptibility
studies on single crystals of the pyrochlore Ho2Ti2O7. The observed field
dependence of magnetization is totally unexpected, as it seems to suggest that
the magnetic moments in this compound do not obey the 'ice-rule'. We have
re-measured the magnetization curves for Ho2Ti2O7 single crystal for the three
principal directions of an applied magnetic field and found nearly perfect
agreement with the predictions for a nearest-neighbor spin-ice model.Comment: comment on Phys. Rev. B 64, 060406(R) (2001
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The dynamics of diluted Ho spin ice Ho2-xYxTi2O7 studied by neutron spin echo spectroscopy
We have studied the spin relaxation in diluted spin ice Ho{sub 2-x} Y{sub x} Ti{sub 2}O{sub 7} by means of neutron spin echo spectroscopy. Remarkably, the geometrical frustration is not relieved by doping with non-magnetic Y, and the dynamics of the freezing is unaltered in the spin echo time window up to x {approx_equal} 1.6. At higher doping with non-magnetic Y (x {ge} 1.6) a new relaxation process at relatively high temperature (up to at least T {approx_equal} 55 K) appears which is more than 10 times faster than the thermally activated main relaxation process. We find evidence that over the whole range of composition all Ho spins participate in the dynamics. These results are compared to a.c. susceptibility measurements of the diluted Ho and Dy spin ice systems. X-ray absorption fine structure (EXAFS) spectra and x-ray diffraction show that the samples are structurally well ordered
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