Supplementary document for Dual-coupling effect enables a high-performance self-powered UV Photodetector - 6823938.pdf

Important supplementary material in manuscrip

Understanding Phonon Scattering by Nanoprecipitates in Potassium-Doped Lead Chalcogenides

We present a comprehensive experimental and theoretical study of phonon scattering by nanoprecipitates in potassium-doped PbTe, PbSe, and PbS. We highlight the role of the precipitate size distribution measured by microscopy, whose tuning allows for thermal conductivities lower than the limit achievable with a single size. The correlation between the size distribution and the contributions to thermal conductivity from phonons in different frequency ranges provides a physical basis to the experimentally measured thermal conductivities, and a criterion to estimate the lowest achievable thermal conductivity. The results have clear implications for efficiency enhancements in nanostructured bulk thermoelectrics