877 research outputs found
Si3N4 single-crystal nanowires grown from silicon micro and nanoparticles near the threshold of passive oxidation
A simple and most promising oxide-assisted catalyst-free method is used to
prepare silicon nitride nanowires that give rise to high yield in a short time.
After a brief analysis of the state of the art, we reveal the crucial role
played by the oxygen partial pressure: when oxygen partial pressure is slightly
below the threshold of passive oxidation, a high yield inhibiting the formation
of any silica layer covering the nanowires occurs and thanks to the synthesis
temperature one can control nanowire dimensions
Coherent and incoherent bands in La and Rh doped Sr3Ir2O7
In Sr2IrO4 and Sr3Ir2O7, correlations, magnetism and spin-orbit coupling
compete on similar energy scales, creating a new context to study
metal-insulator transitions (MIT). We use here Angle-Resolved photoemission to
investigate the MIT as a function of hole and electron doping in Sr3Ir2O7,
obtained respectively by Ir/Rh and Sr/La substitutions. We show that there is a
clear reduction as a function of doping of the gap between a lower and upper
band on both sides of the Fermi level, from 0.2eV to 0.05eV. Although these two
bands have a counterpart in band structure calculations, they are characterized
by a very different degree of coherence. The upper band exhibits clear
quasiparticle peaks, while the lower band is very broad and loses weight as a
function of doping. Moreover, their ARPES spectral weights obey different
periodicities, reinforcing the idea of their different nature. We argue that a
very similar situation occurs in Sr2IrO4 and conclude that the physics of the
two families is essentially the same
Angle-resolved photoemission study of the role of nesting and orbital orderings in the antiferromagnetic phase of BaFe2As2
We present a detailed comparison of the electronic structure of BaFe2As2 in
its paramagnetic and antiferromagnetic (AFM) phases, through angle-resolved
photoemission studies. Using different experimental geometries, we resolve the
full elliptic shape of the electron pockets, including parts of dxy symmetry
along its major axis that are usually missing. This allows us to define
precisely how the hole and electron pockets are nested and how the different
orbitals evolve at the transition. We conclude that the imperfect nesting
between hole and electron pockets explains rather well the formation of gaps
and residual metallic droplets in the AFM phase, provided the relative parity
of the different bands is taken into account. Beyond this nesting picture, we
observe shifts and splittings of numerous bands at the transition. We show that
the splittings are surface sensitive and probably not a reliable signature of
the magnetic order. On the other hand, the shifts indicate a significant
redistribution of the orbital occupations at the transition, especially within
the dxz/dyz system, which we discuss
Giant Anisotropy of Spin-Orbit Splitting at the Bismuth Surface
We investigate the bismuth (111) surface by means of time and angle resolved
photoelectron spectroscopy. The parallel detection of the surface states below
and above the Fermi level reveals a giant anisotropy of the Spin-Orbit (SO)
spitting. These strong deviations from the Rashba-like coupling cannot be
treated in perturbation theory. Instead, first
principle calculations could accurately reproduce the experimental dispersion
of the electronic states. Our analysis shows that the giant anisotropy of the
SO splitting is due to a large out-of plane buckling of the spin and orbital
texture.Comment: 5 pages, 4 figure
Transfer of spectral weight across the gap of Sr2IrO4 induced by La doping
We study with Angle Resolved PhotoElectron Spectroscopy (ARPES) the evolution
of the electronic structure of Sr2IrO4, when holes or electrons are introduced,
through Rh or La substitutions. At low dopings, the added carriers occupy the
first available states, at bottom or top of the gap, revealing an anisotropic
gap of 0.7eV in good agreement with STM measurements. At further doping, we
observe a reduction of the gap and a transfer of spectral weight across the
gap, although the quasiparticle weight remains very small. We discuss the
origin of the in-gap spectral weight as a local distribution of gap values
Significant reduction of electronic correlations upon isovalent Ru substitution of BaFe2As2
We present a detailed investigation of Ba(Fe0.65Ru0.35)2As2 by transport
measurements and Angle Resolved photoemission spectroscopy. We observe that Fe
and Ru orbitals hybridize to form a coherent electronic structure and that Ru
does not induce doping. The number of holes and electrons, deduced from the
area of the Fermi Surface pockets, are both about twice larger than in
BaFe2As2. The contribution of both carriers to the transport is evidenced by a
change of sign of the Hall coefficient with decreasing temperature. Fermi
velocities increase significantly with respect to BaFe2As2, suggesting a
significant reduction of correlation effects. This may be a key to understand
the appearance of superconductivity at the expense of magnetism in undoped iron
pnictides
Ultrafast filling of an electronic pseudogap in an incommensurate crystal
We investigate the quasiperiodic crystal (LaS)1.196(VS2) by angle and time
resolved photoemission spectroscopy. The dispersion of electronic states is in
qualitative agreement with band structure calculated for the VS2 slab without
the incommensurate distortion. Nonetheless, the spectra display a temperature
dependent pseudogap instead of quasiparticles crossing. The sudden
photoexcitation at 50 K induces a partial filling of the electronic pseudogap
within less than 80 fs. The electronic energy flows into the lattice modes on a
comparable timescale. We attribute this surprisingly short timescale to a very
strong electron-phonon coupling to the incommensurate distortion. This result
sheds light on the electronic localization arising in aperiodic structures and
quasicrystals
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