23 research outputs found
-Enhanced Imaging of Molecules in an Optical Trap
We report non-destructive imaging of optically trapped calcium monofluoride
(CaF) molecules using in-situ -enhanced gray molasses cooling.
times more fluorescence is obtained compared to destructive on-resonance
imaging, and the trapped molecules remain at a temperature of
. The achieved number of scattered photons makes possible
non-destructive single-shot detection of single molecules with high fidelity.Comment: 6 pages, 4 figure
One dimensional magneto-optical compression of a cold CaF molecular beam
We demonstrate with a RF-MOT the one dimensional, transverse magneto-optical
compression of a cold beam of calcium monofluoride (CaF). By continually
alternating the magnetic field direction and laser polarizations of the
magneto-optical trap, a photon scattering rate of 0.4 MHz is
achieved. A 3D model for this RF-MOT, validated by agreement with data,
predicts a 3D RF-MOT capture velocity for CaF of 5 m/s
Branching Ratios, Radiative Lifetimes and Transition Dipole Moments for YbOH
Medium resolution (Δν~ 3 GHz) laser-induced fluorescence (LIF) excitation spectra of a rotationally cold sample of YbOH in the 17300-17950 cm⁻¹ range have been recorded using two-dimensional (excitation and dispersed fluorescence) spectroscopy. High resolution (Δλ~ 0.65 nm) dispersed laser induced fluorescence (DLIF) spectra and radiative decay curves of numerous bands detected in the medium resolution LIF excitation spectra were recorded. The vibronic energy levels of the X²Σ state were predicted using a discrete variable representation approach and compared with observations. The radiative decay curves were analyzed to produce fluorescence lifetimes. DLIF spectra resulting from high resolution (Δν < 10 MHz) LIF excitation of individual low-rotational lines in the A²Π_(1/2)(000)-X²Σ((000), A²Π_(1/2)(100)-X²Σ((000), and [17.73]Ω=0.5-X²Σ((000) bands were also recorded. The DLIF spectra were analyzed to determine branching ratios which were combined with radiative lifetimes to obtain transition dipole moments. The implications for laser cooling and trapping of YbOH are discussed