2,958 research outputs found

    Coherent photodissociation reactions: Observation by a novel picosecond polarization technique

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    In this communication, we wish to report on a novel picosecond polarization method for measuring the degree of rotational coherence that is preserved in photodissociation reactions. The systems studied here are jet-cooled van der Waals molecules; stilbene [4-6] bound [5] to He or Ne with a 1:1 composition.[7

    Caging phenomena in reactions: Femtosecond observation of coherent, collisional confinement

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    We report striking observations of coherent caging of iodine, above the B state dissociation threshold, by single collisions with rare gas atoms at room-temperature. Despite the random nature of the solute–solvent interaction, the caged population retains coherence of the initially prepared unbound wave packet. We discuss some new concepts regarding dynamical coherent caging and the one-atom cage effect

    Anomalous Negative Magnetoresistance Caused by Non-Markovian Effects

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    A theory of recently discovered anomalous low-field magnetoresistance is developed for the system of two-dimensional electrons scattered by hard disks of radius a,a, randomly distributed with concentration n.n. For small magnetic fields the magentoresistance is found to be parabolic and inversely proportional to the gas parameter, δρxx/ρ(ωcτ)2/na2. \delta \rho_{xx}/\rho \sim - (\omega_c \tau)^2 / n a^2. With increasing field the magnetoresistance becomes linear δρxx/ρωcτ\delta \rho_{xx}/\rho \sim - \omega_c \tau in a good agreement with the experiment and numerical simulations.Comment: 4 pages RevTeX, 5 figure

    Two regimes for effects of surface disorder on the zero-bias conductance peak of tunnel junctions involving d-wave superconductors

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    Impurity-induced quasiparticle bound states on a pair-breaking surface of a d-wave superconductor are theoretically described, taking into account hybridization of impurity- and surface-induced Andreev states. Further a theory for effects of surface disorder (of thin impurity surface layer) on the low-bias conductance of tunnel junctions is developed. We find a threshold ncn_c for surface impurity concentration nSn_S, which separates the two regimes for surface impurity effects on the zero-bias conductance peak (ZBCP). Below the threshold, surface impurities do not broaden the ZBCP, but effectively reduce its weight and generate impurity bands. For low nSn_S impurity bands can be, in principle, resolved experimentally, being centered at energies of bound states induced by an isolated impurity on the surface. For larger nSn_S impurity bands are distorted, move to lower energies and, beginning with the threshold concentration nS=ncn_S=n_c, become centered at zero energy. With increasing nSn_S above the threshold, the ZBCP is quickly destroyed in the case of strong scatterers, while it is gradually suppressed and broaden in the presence of weak impurity potentials. More realistic cases, taking into account additional broadening, not related to the surface disorder, are also considered.Comment: 9 pages, 7 figure

    4D visualization of embryonic, structural crystallization by single-pulse microscopy

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    In many physical and biological systems the transition from an amorphous to ordered native structure involves complex energy landscapes, and understanding such transformations requires not only their thermodynamics but also the structural dynamics during the process. Here, we extend our 4D visualization method with electron imaging to include the study of irreversible processes with a single pulse in the same ultrafast electron microscope (UEM) as used before in the single-electron mode for the study of reversible processes. With this augmentation, we report on the transformation of amorphous to crystalline structure with silicon as an example. A single heating pulse was used to initiate crystallization from the amorphous phase while a single packet of electrons imaged selectively in space the transformation as the structure continuously changes with time. From the evolution of crystallinity in real time and the changes in morphology, for nanosecond and femtosecond pulse heating, we describe two types of processes, one that occurs at early time and involves a nondiffusive motion and another that takes place on a longer time scale. Similar mechanisms of two distinct time scales may perhaps be important in biomolecular folding

    Quasiclassical negative magnetoresistance of a 2D electron gas: interplay of strong scatterers and smooth disorder

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    We study the quasiclassical magnetotransport of non-interacting fermions in two dimensions moving in a random array of strong scatterers (antidots, impurities or defects) on the background of a smooth random potential. We demonstrate that the combination of the two types of disorder induces a novel mechanism leading to a strong negative magnetoresistance, followed by the saturation of the magnetoresistivity ρxx(B)\rho_{xx}(B) at a value determined solely by the smooth disorder. Experimental relevance to the transport in semiconductor heterostructures is discussed.Comment: 4 pages, 2 figure

    Time-Translation Invariance of Scattering Maps and Blue-Shift Instabilities on Kerr Black Hole Spacetimes

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    In this paper, we provide an elementary, unified treatment of two distinct blue-shift instabilities for the scalar wave equation on a fixed Kerr black hole background: the celebrated blue-shift at the Cauchy horizon (familiar from the strong cosmic censorship conjecture) and the time-reversed red-shift at the event horizon (relevant in classical scattering theory). Our first theorem concerns the latter and constructs solutions to the wave equation on Kerr spacetimes such that the radiation field along the future event horizon vanishes and the radiation field along future null infinity decays at an arbitrarily fast polynomial rate, yet, the local energy of the solution is infinite near any point on the future event horizon. Our second theorem constructs solutions to the wave equation on rotating Kerr spacetimes such that the radiation field along the past event horizon (extended into the black hole) vanishes and the radiation field along past null infinity decays at an arbitrarily fast polynomial rate, yet, the local energy of the solution is infinite near any point on the Cauchy horizon. The results make essential use of the scattering theory developed in [M. Dafermos, I. Rodnianski and Y. Shlapentokh-Rothman, A scattering theory for the wave equation on Kerr black hole exteriors, preprint (2014) available at \url{http://arxiv.org/abs/1412.8379}] and exploit directly the time-translation invariance of the scattering map and the non-triviality of the transmission map.Comment: 26 pages, 12 figure
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