105 research outputs found

    Evolution of the Fermi surface of BaFe_2(As_{1-x}P_x)_2 on entering the superconducting dome

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    Using the de Haas-van Alphen effect we have measured the evolution of the Fermi surface of BaFe_2(As_{1-x}P_x)_2 as function of isoelectric substitution (As/P) for 0.41<x<1 (T_c up to 25 K). We find that the volume of electron and hole Fermi surfaces shrink linearly with decreasing x. This shrinking is accompanied by a strong increase in the quasiparticle effective mass as x is tuned toward the maximum T_c. It is likely that these trends originate from the many-body interaction which give rise to superconductivity, rather than the underlying one-electron bandstructure.Comment: 4 page

    Superconductivity and Pseudogap in Quasi-Two-Dimensional Metals around the Antiferromagnetic Quantum Critical Point

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    Spin fluctuations (SF) and SF-mediated superconductivity (SC) in quasi-two-dimensional metals around the antiferrromagnetic (AF) quantum critical point (QCP) are investigated by using the self-consistent renormalization theory for SF and the strong coupling theory for SC. We introduce a parameter y0 as a measure for the distance from the AFQCP which is approximately proportional to (x-xc), x being the electron (e) or hole (h) doping concentration to the half-filled band and xc being the value at the AFQCP. We present phase diagrams in the T-y0 plane including contour maps of the AF correlation length and AF and SC transition temperatures TN and Tc, respectively. The Tc curve is dome-shaped with a maximum at around the AFQCP. The calculated one-electron spectral density shows a pseudogap in the high-density-of-states region near (pi,0) below around a certain temperature T* and gives a contour map at the Fermi energy reminiscent of the Fermi arc. These results are discussed in comparison with e- and h-doped high-Tc cuprates.Comment: 5 pages, 3 figure

    The fermi arc and fermi pocket in cuprates in a short-range diagonal stripe phase

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    In this paper we studied the fermi arc and the fermi pocket in cuprates in a short-range diagonal stripe phase with wave vectors (7π/8,7π/8)(7\pi/8, 7\pi/8), which reproduce with a high accuracy the positions and sizes of the fermi arc and fermi pocket and the superstructure in cuprates observed by Meng et al\cite{Meng}. The low-energy spectral function indicates that the fermi pocket results from the main band and the shadow band at the fermi energy. Above the fermi energy the shadow band gradually departs away from the main band, leaving a fermi arc. Thus we conclude that the fermi arc and fermi pocket can be fully attributed to the stripe phase but has nothing to do with pairing. Incorporating a d-wave pairing potential in the stripe phase the spectral weight in the antinodal region is removed, leaving a clean fermi pocket in the nodal region.Comment: 5 pages, 6 figure

    Advances in single crystal growth and annealing treatment of electron-doped HTSC

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    High quality electron-doped HTSC single crystals of Pr2−xCexCuO4+ÎŽ\rm Pr_{2-x}Ce_{x}CuO_{4+\delta} and Nd2−xCexCuO4+ÎŽ\rm Nd_{2-x}Ce_{x}CuO_{4+\delta} have been successfully grown by the container-free traveling solvent floating zone technique. The optimally doped Pr2−xCexCuO4+ÎŽ\rm Pr_{2-x}Ce_{x}CuO_{4+\delta} and Nd2−xCexCuO4+ÎŽ\rm Nd_{2-x}Ce_{x}CuO_{4+\delta} crystals have transition temperatures TcT_{\rm c} of 2525\,K and 23.523.5\,K, respectively, with a transition width of less than 11\,K. We found a strong dependence of the optimal growth parameters on the Ce content xx. We discuss the optimization of the post-growth annealing treatment of the samples, the doping extension of the superconducting dome for both compounds as well as the role of excess oxygen. The absolute oxygen content of the as-grown crystals is determined from thermogravimetric experiments and is found to be ≄4.0\ge 4.0. This oxygen surplus is nearly completely removed by a post-growth annealing treatment. The reduction process is reversible as demonstrated by magnetization measurements. In as-grown samples the excess oxygen resides on the apical site O(3). This apical oxygen has nearly no doping effect, but rather influences the evolution of superconductivity by inducing additional disorder in the CuO2_{2} layers. The very high crystal quality of Nd2−xCexCuO4+ÎŽ\rm Nd_{2-x}Ce_{x}CuO_{4+\delta} is particularly manifest in magnetic quantum oscillations observed on several samples at different doping levels. They provide a unique opportunity of studying the Fermi surface and its dependence on the carrier concentration in the bulk of the crystals.Comment: 19 pages, 7 figures, submitted to Eur. Phys. J.

    13C NMR study of superconductivity near charge instability realized in beta"-(BEDT-TTF)4[(H3O)Ga(C2O4)3]C6H5NO2

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    To investigate the superconducting (SC) state near a charge instability, we performed ^{13}C NMR experiments on the molecular superconductor beta"-(BEDT-TTF)_{4}[(H_{3}O)Ga(C_{2}O_{4})_{3}]C_{6}H_{5}NO_{2}, which exhibits a charge anomaly at 100 K. The Knight shift which we measured in the SC state down to 1.5 K demonstrates that Cooper pairs are in spin-singlet state. Measurements of the nuclear spin-lattice relaxation time reveal strong electron-electron correlations in the normal state. The resistivity increase observed below 10 K indicates that the enhanced fluctuation has an electric origin. We discuss the possibility of charge-fluctuation-induced superconductivity.Comment: 5 pages, 4 figure

    From high temperature supercondutivity to quantum spin liquid: progress in strong correlation physics

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    This review gives a rather general discussion of high temperature superconductors as an example of a strongly correlated material. The argument is made that in view of the many examples of unconventional superconductors discovered in the past twenty years, we should no longer be surprised that superconductivity emerges as a highly competitive ground state in systems where Coulomb repulsion plays a dominant role. The physics of the cuprates is discussed, emphasizing the unusual pseudogap phase in the underdoped region. It is argued that the resonating valence bond (RVB) picture, as formulated using gauge theory with fermionic and bosonic matter fields, gives an adequate physical understanding, even though many details are beyond the powers of current calculational tools. The recent discovery of quantum oscillations in a high magnetic field is discussed in this context. Meanwhile, the problem of the quantum spin liquid (a spin system with antiferromagnetic coupling which refuses to order even at zero temperature) is a somewhat simpler version of the high TcT_c problem where significant progress has been made recently. It is understood that the existence of matter fields can lead to de-confinement of the U(1) gauge theory in 2+1 dimensions, and novel new particles (called fractionalized particles), such as fermionic spinons which carry spin 12{1\over 2} and no charge, and gapless gauge bosons can emerge to create a new critical state at low energies. We even have a couple of real materials where such a scenario may be realized experimentally. The article ends with answers to questions such as: what limits TcT_c if pairing is driven by an electronic energy scale? why is the high TcT_c problem hard? why is there no consensus? and why is the high TcT_c problem important?Comment: Submitted as "Key Issue" essay for Report of Progress in Physics; v2: References are added and typos correcte
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