111 research outputs found
Optical mode crossings and the low temperature anomalies of SrTiO3
Optical mode crossing is not a plausible explanation for the new broad
Brillouin doublet nor for the strong acoustic anomalies observed at low
temperatures in SrTiO3. Data presented to support that explanation are also
inconclusive.Comment: This is a comment to a paper from J.F. Scott (same ZFP volume
Hyper-Raman scattering from vitreous boron oxide: coherent enhancement of the boson peak
Hyper-Raman scattering spectra of vitreous BO are reported and
compared to Raman scattering results. The main features are indexed in terms of
vibrations of structural units. Particular attention is given to the low
frequency boson peak which is shown to relate to out-of-plane librations of
BO boroxol rings and BO triangles. Its hyper-Raman strength is
comparable to that of cooperative polar modes. It points to a sizeable coherent
enhancement of the hyper-Raman signal compared to the Raman one. This is
explained by the symmetry of the structural units.Comment: 4 pages, 3 figure
The broad Brillouin doublets and central peak of KTaO_3
The incipient ferroelectric KTaO3 presents low-T Brillouin spectra
anomalies,e.g. a broad central peak (CP), and some additional Brillouin
doublets (BD), whose origin is interpreted in terms of phonon-density
fluctuation processes. A parameterisation from new extensive high-resolution
neutron-scattering measurements is used to show that hydrodynamic second sound
from high damping (compared to BD frequency) TA phonons may exist in the
crystal. Furthermore, low damping thermal phonons may scatter light through
two-phonon difference processes and appear on the Brillouin spectra either as a
sharp or a broader BD, depending on the phonon damping and group velocity . The
comparison between computed anisotropies and experimental measurements favours
the second process.Comment: 3 pages, 1 figure, ECNS99 Proceedings. See http://www.ill.fr
Kinetic glass behavior in a diffusive model
Three properties of the Edwards-Anderson model with mobile bonds are
investigated which are characteristic of kinetic glasses. First is two-time
relaxation in aged systems, where a significant difference is observed between
spin and bond autocorrelation functions. The spin subsystem does not show
two-time behavior, and the relaxation is stretched exponential. The bond
subsystem shows two-time behavior, with the first relaxation nearly exponential
and the second similar to the spin one. Second is the two-temperature behavior,
which can be tuned by bond dilution through the full range reported in the
literature. Third is the rigid-to-floppy transition, identified as a function
of bond dilution. Simple Glauber Monte Carlo evolution without extraneous
constraints reproduces the behavior of classical kinetic simulations, with the
bond (spin) degree of freedom corresponding to configurational (orientational)
disorder.Comment: 4 pages, 3 figures, minimal corrections, to appear in Phys. Rev. B
(RC
Hyper-Raman scattering analysis of the vibrations in vitreous boron oxide
Hyper-Raman scattering has been measured on vitreous boron oxide,
BO. This spectroscopy, complemented with Raman scattering and
infrared absorption, reveals the full set of vibrations that can be observed
with light. A mode analysis is performed based on the local D symmetry
of BO triangles and BO boroxol rings. The results show that in
BO the main spectral components can be succesfully assigned using
this relatively simple model. In particular, it can be shown that the
hyper-Raman boson peak arises from external modes that correspond mainly to
librational motions of rigid boroxol rings.Comment: 13 pages, 11 figures, 2 table
XUV Frequency Combs via Femtosecond Enhancement Cavities
We review the current state of tabletop extreme ultraviolet (XUV) sources
based on high harmonic generation (HHG) in femtosecond enhancement cavities
(fsEC). Recent developments have enabled generation of high photon flux (1014
photons/sec) in the XUV, at high repetition rates (>50 MHz) and spanning the
spectral region from 40 nm - 120 nm. This level of performance has enabled
precision spectroscopy with XUV frequency combs and promises further
applications in XUV spectroscopic and photoemission studies. We discuss the
theory of operation and experimental details of the fsEC and XUV generation
based on HHG, including current technical challenges to increasing the photon
flux and maximum photon energy produced by this type of system. Current and
future applications for these sources are also discussed.Comment: invited review article, 38 page
The crossover from propagating to strongly scattered acoustic modes of glasses observed in densified silica
Spectroscopic results on low frequency excitations of densified silica are
presented and related to characteristic thermal properties of glasses. The end
of the longitudinal acoustic branch is marked by a rapid increase of the
Brillouin linewidth with the scattering vector. This rapid growth saturates at
a crossover frequency Omega_co which nearly coincides with the center of the
boson peak. The latter is clearly due to additional optic-like excitations
related to nearly rigid SiO_4 librations as indicated by hyper-Raman
scattering. Whether the onset of strong scattering is best described by
hybridization of acoustic modes with these librations, by their elastic
scattering (Rayleigh scattering) on the local excitations, or by soft
potentials remains to be settled.Comment: 14 pages, 6 figures, to be published in a special issue of J. Phys.
Condens. Matte
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