Finite size effects and magnetic order in the spin-1/2 honeycomb lattice compound InCu{2/3}V{1/3}O{3}

High field electron spin resonance, nuclear magnetic resonance and magnetization studies addressing the ground state of the quasi two-dimensional spin-1/2 honeycomb lattice compound InCu{2/3}V{1/3}O{3} are reported. Uncorrelated finite size structural domains occurring in the honeycomb planes are expected to inhibit long range magnetic order. Surprisingly, ESR data reveal the development of two collinear antiferromagnetic (AFM) sublattices below ~ 20 K whereas NMR results show the presence of the staggered internal field. Magnetization data evidence a spin reorientation transition at ~ 5.7 T. Quantum Monte-Carlo calculations show that switching on the coupling between the honeycomb spin planes in a finite size cluster yields a Neel-like AFM spin structure with a substantial staggered magnetization at finite temperatures. This may explain the occurrence of a robust AFM state in InCu{2/3}V{1/3}O{3} despite an unfavorable effect of structural disorder.Comment: revised version, accepted as a Rapid Communication in Phys. Rev. B (2010

Magnetic Properties of the low dimensional spin system (VO)2_2P2_2O7_{7}: ESR and susceptibility

Experimental results on magnetic resonance (ESR) and magnetic susceptibility are given for single crystalline (VO)$_2$P$_2$O$_{7}$. The crystal growth procedure is briefly discussed. The susceptibility is interpreted numerically using a model with alternating spin chains. We determine $J$=51 K and $\delta$=0.2. Furthermore we find a spin gap of $\approx 6$meV from our ESR measurements. Using elastic constants no indication of a phase transition forcing the dimerization is seen below 300 K.Comment: 7 pages, REVTEX, 7 figure

Acoustic Faraday effect in Tb3_3Ga5_5O12_{12}

The transverse acoustic wave propagating along the [100] axis of the cubic Tb$_3$Ga$_5$O$_{12}$ (acoustic $c_{44}$ mode) is doubly degenerate. A magnetic field applied in the direction of propagation lifts this degeneracy and leads to the rotation of the polarization vector - the magneto-acoustic Faraday rotation. Here, we report on the observation and analysis of the magneto-acoustic Faraday-effect in Tb$_3$Ga$_5$O$_{12}$ in static and pulsed magnetic fields. We present also a theoretical model based on magnetoelastic coupling of 4$f$ electrons to both, acoustic and optical phonons and an effective coupling between them. This model explains the observed linear frequency dependence of the Faraday rotation angle

Lifetimes of ultralong-range Rydberg molecules in vibrational ground and excited state

Since their first experimental observation, ultralong-range Rydberg molecules consisting of a highly excited Rydberg atom and a ground state atom have attracted the interest in the field of ultracold chemistry. Especially the intriguing properties like size, polarizability and type of binding they inherit from the Rydberg atom are of interest. An open question in the field is the reduced lifetime of the molecules compared to the corresponding atomic Rydberg states. In this letter we present an experimental study on the lifetimes of the ^3\Sigma (5s-35s) molecule in its vibrational ground state and in an excited state. We show that the lifetimes depends on the density of ground state atoms and that this can be described in the frame of a classical scattering between the molecules and ground state atoms. We also find that the excited molecular state has an even more reduced lifetime compared to the ground state which can be attributed to an inward penetration of the bound atomic pair due to imperfect quantum reflection that takes place in the special shape of the molecular potential

GHz Rabi flopping to Rydberg states in hot atomic vapor cells

We report on the observation of Rabi oscillations to a Rydberg state on a timescale below one nanosecond in thermal rubidium vapor. We use a bandwidth-limited pulsed excitation and observe up to 6 full Rabi cycles within a pulse duration of ~ 4 ns. We find good agreement between the experiment and numerical simulations based on a surprisingly simple model. This result shows that fully coherent dynamics with Rydberg states can be achieved even in thermal atomic vapor thus suggesting small vapor cells as a platform for room temperature quantum devices. Furthermore the result implies that previous coherent dynamics in single atom Rydberg gates can be accelerated by three orders of magnitude.Comment: 4 pages, 3 figure

Real space renormalization group approach to the 2d antiferromagnetic Heisenberg model

The low energy behaviour of the 2d antiferromagnetic Heisenberg model is studied in the sector with total spins $S=0,1,2$ by means of a renormalization group procedure, which generates a recursion formula for the interaction matrix $\Delta_S^{(n+1)}$ of 4 neighbouring "$n$ clusters" of size $2^n\times 2^n$, $n=1,2,3,...$ from the corresponding quantities $\Delta_S^{(n)}$. Conservation of total spin $S$ is implemented explicitly and plays an important role. It is shown, how the ground state energies $E_S^{(n+1)}$, $S=0,1,2$ approach each other for increasing $n$, i.e. system size. The most relevant couplings in the interaction matrices are generated by the transitions $$ between the ground states $|S,m;n+1>$ ($m=-S,...,S$) on an $(n+1)$-cluster of size $2^{n+1}\times 2^{n+1}$, mediated by the staggered spin operator $S_q^*$Comment: 18 pages, 8 figures, RevTe

On the absence of ferromagnetism in typical 2D ferromagnets

We consider the Ising systems in $d$ dimensions with nearest-neighbor ferromagnetic interactions and long-range repulsive (antiferromagnetic) interactions which decay with a power, $s$, of the distance. The physical context of such models is discussed; primarily this is $d=2$ and $s=3$ where, at long distances, genuine magnetic interactions between genuine magnetic dipoles are of this form. We prove that when the power of decay lies above $d$ and does not exceed $d+1$, then for all temperatures, the spontaneous magnetization is zero. In contrast, we also show that for powers exceeding $d+1$ (with $d\ge2$) magnetic order can occur.Comment: 15 pages, CMP style fil