520 research outputs found

    Systematic Study of Short Range Antiferromagnetic Order and The Spin-Glass State in Lightly Doped La2-xSrxCuO4

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    Systematic measurements of the magnetic susceptibility were performed on single crystals of lightly doped La2-xSrxCuO4 (x=0.03, 0.04 and 0.05). For all samples the temperature dependence of the in-plane magnetic susceptibility shows typical spin-glass features with spin-glass transition temperatures Tg of 6.3K, 5.5K and 5.0K for x=0.03, 0.04 and 0.05, respectively. The canonical spin-glass order parameter extracted from the in-plane susceptibility of all the samples follows a universal scaling curve. On the other hand, the out-of-plane magnetic susceptibility deviates from Curie law below a temperature Tdv, higher than Tg. Comparing with previous neutron scattering results with an instrumental energy resolution of 0.25 meV from Wakimoto et al., the x-dependence of Tdv is qualitatively the same as that of Tel, the temperature below which the elastic magnetic scattering develops around (pi, pi). Thus, a revised magnetic phase diagram in the lightly doped region of La2-xSrxCuO4 is proposed. The Curie constants calculated from the in-plane susceptibility are independent of the Sr concentration. On the basis of the cluster spin-glass model, this fact might reflect an inhomogeneous distribution of doped holes in the CuO2 plane, such as in a stripe structure.Comment: 7 pages, 6 figure

    Field-induced transition between magnetically disordered and ordered phases in underdoped La(2-x)SrxCuO4

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    We report the observation of a magnetic-field-induced transition between magnetically disordered and ordered phases in slightly under-doped La(2-x)SrxCuO4 with x=0.144. Static incommensurate spin-density-wave order is induced above a critical field of about 3 T, as measured by elastic neutron scattering. Our results allow us to constrain the location of a quantum critical point on the phase diagram.Comment: 10 pages, 2 figures; discussion on the location of a quantum critical point is revise

    Free Boson Representation of Uq(sl^3)U_q(\widehat{sl}_3)

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    A representation of the quantum affine algebra Uq(sl^3)U_{q}(\widehat{sl}_3) of an arbitrary level kk is constructed in the Fock module of eight boson fields. This realization reduces the Wakimoto representation in the q1q \rightarrow 1 limit. The analogues of the screening currents are also obtained. They commute with the action of Uq(sl^3)U_{q}(\widehat{sl}_3) modulo total differences of some fields.Comment: 12 pages, LaTeX, RIMS-920, YITP/K-101

    Magnetic field effects and magnetic anisotropy in lightly doped La_{2-x}Sr_xCuO_4

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    The effects of the application of a magnetic field on the diagonal stripe spin-glass phase is studied in lightly doped La_{2-x}Sr_xCuO_4 (x=0.014 and 0.024). With increasing magnetic field, the magnetic elastic intensity at the diagonal incommensurate (DIC) positions (1,\pm\epsilon,0) decreases as opposed to the increase seen in superconducting samples. This diminution in intensity with increasing magnetic field originates from a spin reorientation transition, which is driven by the antisymmetric exchange term in the spin Hamiltonian. On the other hand, the transition temperature, the incommensurability, and the peak width of the diagonal incommensurate correlations are not changed with magnetic field. This result suggests that the magnetic correlations are determined primarily by the charge disproportionation and that the geometry of the diagonal incommensurate magnetism is also determined by effects, that is, stripe formation which are not purely magnetic in origin. The Dzyaloshinskii-Moriya antisymmetric exchange is nevertheless important in determining the local spin structure in the DIC stripe phase.Comment: 7 pages, 5 figures, to appear in Phys. Rev.

    Disorder and relaxation mode in the lattice dynamics of PbMg1/3_{1/3}Nb2/3_{2/3}O3_3 relaxor ferroelectric

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    The low-energy part of vibration spectrum in PbMg1/3_{1/3}Nb2/3_{2/3}O3_3 relaxor ferroelectric was studied by inelastic neutron scattering. We observed the coexistence of a resolution-limited central peak with strong quasielastic scattering. The line-width of the quasielastic component follows a Γ0+Dq2\Gamma_0+Dq^2 dependence. We find that Γ0\Gamma_0 is temperature-dependent. The relaxation time follows the Arrhenius law well. The presence of a relaxation mode associated with quasi-elastic scattering in PMN indicates that order-disorder behaviour plays an important r\^ole in the dynamics of diffuse phase transitions

    Neutron scattering study of soft phonons and diffuse scattering in insulating La1.95_{1.95}Sr0.05_{0.05}CuO4_{4}

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    Soft phonons and diffuse scattering in insulating La2x_{2-x}Srx_{x}CuO4_4 (x=0.05x=0.05) have been studied by the neutron scattering technique. The X-point phonon softens from high temperature towards the structural transition temperature Ts=410T_{s}=410 K, and the Z-point phonon softens again below 200 K. The Z-point phonon softening persists to low temperature, in contrast to the behavior observed in the superconducting x=0.15x=0.15 compound, in which the Z-point phonon hardens below TcT_c. The diffuse scattering associated with the structural phase transition at 410 K appears at commensurate positions. These results highlight interesting differences between superconducting and insulating samples.Comment: 5 pages, 5 figure

    Static and dynamic spin correlations in the spin-glass phase of slightly-doped La_{2-x}Sr_xCuO_4

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    Neutron scattering experiments reveal that a diagonal spin modulation, which is a one-dimensional modulation rotated away by 45^\circ from that in the superconducting phase, occurs universally across the insulating spin-glass phase in La2x_{2-x}Srx_xCuO4_4 (0.02x\le x\le0.055). This establishes an intimate relation between the magnetism and the transport properties in the high-temperature copper oxide superconductors. Furthermore, it is found that the charge density per unit length estimated using a charge stripe model is almost constant throughout the phase diagram, even when the modulation rotates away by 45^\circ at the superconducting boundary. However, at the lowest values for xx the density changes approaching 1 hole/Cu as in La2x_{2-x}Srx_xNiO4_4. Magnetic excitation spectra suggest that magnetic correlations change from incommensurate to commensurate at ω\omega\sim7 meV and TT\sim70 K, indicating a characteristic energy for the incommensurate structure of 6-7 meV.Comment: 7 pages, submitted to Phys. Rev.

    A Neutron Elastic Diffuse Scattering Study of PMN

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    We have performed elastic diffuse neutron scattering studies on the relaxor Pb(Mg1/3_{1/3}Nb2/3_{2/3})O3_3 (PMN). The measured intensity distribution near a (100) Bragg peak in the (hk0) scattering plane assumes the shape of a butterfly with extended intensity in the (110) and (11ˉ\bar{1}0) directions. The temperature dependence of the diffuse scattering shows that both the size of the polar nanoregions (PNR) and the integrated diffuse intensity increase with cooling even for temperatures below the Curie temperature TC213T_C \sim 213 K.Comment: Submitted to PR

    Unusual magnetic susceptibility anisotropy in untwinned La_{2-x}Sr_xCuO_4 single crystals in the lightly-doped region

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    We present a study of the magnetic susceptibility in carefully detwinned La_{2-x}Sr_{x}CuO_4 single crystals in the lightly-doped region (x=0-0.03), which demonstrates a remarkable in-plane anisotropy of the spin system. This anisotropy is found to persist after the long-range antiferromagnetic (AF) order is destroyed by hole doping, suggesting that doped holes break the AF order into domains in which the spin alignment is kept essentially intact. It turns out that the freezing of the spins taking place at low temperatures is also notably anisotropic, implying that the "spin-glass" feature is governed by the domain structure as well.Comment: 4 pages, 3 figures, accepted for publication in Phys.Rev.Let
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