Induced order and reentrant melting in classical two-dimensional binary clusters

A binary system of classical charged particles interacting through a dipole repulsive potential and confined in a two-dimensional hardwall trap is studied by Brownian dynamics simulations. We found that the presence of small particles \emph{stabilizes} the angular order of the system as a consequence of radial fluctuations of the small particles. There is an optimum in the increased rigidity of the cluster as function of the number of small particles. The small (i.e. defect) particles melt at a lower temperature compared to the big particles and exhibit a \emph{reentrant} behavior in its radial order that is induced by the intershell rotation of the big particles.Comment: 7 pages, 3 figure

Adsorption and desorption in confined geometries: a discrete hopping model

We study the adsorption and desorption kinetics of interacting particles moving on a one-dimensional lattice. Confinement is introduced by limiting the number of particles on a lattice site. Adsorption and desorption are found to proceed at different rates, and are strongly influenced by the concentration-dependent transport diffusion. Analytical solutions for the transport and self-diffusion are given for systems of length 1 and 2 and for a zero-range process. In the last situation the self- and transport diffusion can be calculated analytically for any length.Comment: Published in EPJ ST volume "Brownian Motion in Confined Geometries

Comment on "Generalized exclusion processes: Transport coefficients"

In a recent paper Arita et al. [Phys. Rev. E 90, 052108 (2014)] consider the transport properties of a class of generalized exclusion processes. Analytical expressions for the transport-diffusion coefficient are derived by ignoring correlations. It is claimed that these expressions become exact in the hydrodynamic limit. In this Comment, we point out that (i) the influence of correlations upon the diffusion does not vanish in the hydrodynamic limit, and (ii) the expressions for the self- and transport diffusion derived by Arita et al. are special cases of results derived in [Phys. Rev. Lett. 111, 110601 (2013)].Comment: (citation added, published version

Diffusion of interacting particles in discrete geometries

We evaluate the self-diffusion and transport diffusion of interacting particles in a discrete geometry consisting of a linear chain of cavities, with interactions within a cavity described by a free-energy function. Exact analytical expressions are obtained in the absence of correlations, showing that the self-diffusion can exceed the transport diffusion if the free-energy function is concave. The effect of correlations is elucidated by comparison with numerical results. Quantitative agreement is obtained with recent experimental data for diffusion in a nanoporous zeolitic imidazolate framework material, ZIF-8.Comment: 5 pages main text (3 figures); 9 pages supplemental material (2 figures). (minor changes, published version

A Response-Time Analysis for Non-Preemptive Job Sets under Global Scheduling

An effective way to increase the timing predictability of multicore platforms is to use non-preemptive scheduling. It reduces preemption and job migration overheads, avoids intra-core cache interference, and improves the accuracy of worst-case execution time (WCET) estimates. However, existing schedulability tests for global non-preemptive multiprocessor scheduling are pessimistic, especially when applied to periodic workloads. This paper reduces this pessimism by introducing a new type of sufficient schedulability analysis that is based on an exploration of the space of possible schedules using concise abstractions and state-pruning techniques. Specifically, we analyze the schedulability of non-preemptive job sets (with bounded release jitter and execution time variation) scheduled by a global job-level fixed-priority (JLFP) scheduling algorithm upon an identical multicore platform. The analysis yields a lower bound on the best-case response-time (BCRT) and an upper bound on the worst-case response time (WCRT) of the jobs. In an empirical evaluation with randomly generated workloads, we show that the method scales to 30 tasks, a hundred thousand jobs (per hyperperiod), and up to 9 cores.info:eu-repo/semantics/publishedVersio

On Strong and Weak Sustainability, with an Application to Self-Susp ending Real-Time Tasks

Motivated by an apparent contradiction regarding whether certain scheduling policies are sustainable, we revisit the topic of sustainability in real-time scheduling and argue that the existing definitions of sustainability should be further clarified and generalized. After proposing a formal, generic sustainability theory, we relax the existing notion of (strongly) sustainable scheduling policy to provide a new classification called weak sustainability. Proving weak sustainability properties allows reducing the number of variables that must be considered in the search of a worst-case schedule, and hence enables more efficient schedulability analyses and testing regimes even for policies that are not (strongly) sustainable. As a proof of concept, and to better understand a model for which many mistakes were found in the literature, we study weak sustainability in the context of dynamic self-suspending tasks, where we formalize a generic suspension model using the Coq proof assistant and provide a machine-checked proof that any JLFP scheduling policy is weakly sustainable with respect to job costs and variable suspension times.info:eu-repo/semantics/publishedVersio

Response-Time Analysis for Non-Preemptive Global Scheduling with {FIFO} Spin Locks

Motivated by the lack of response-time analyses for non-preemptive global scheduling that consider shared resources, this paper provides such an analysis for global job-level fixed-priority (JLFP) scheduling policies and FIFO-ordered spin locks. The proposed analysis computes response-time bounds for a set of resource-sharing jobs subject to release jitter and execution-time uncertainties by implicitly exploring all possible execution scenarios using state-abstraction and state-pruning techniques. A large-scale empirical evaluation of the proposed analysis shows it to be substantially less pessimistic than simple execution-time inflation methods, thanks to the explicit modeling of contention for shared resources and scenario-aware blocking analysis

Diffusion of interacting particles in discrete geometries: equilibrium and dynamical properties

We expand on a recent study of a lattice model of interacting particles [Phys. Rev. Lett. 111, 110601 (2013)]. The adsorption isotherm and equilibrium fluctuations in particle number are discussed as a function of the interaction. Their behavior is similar to that of interacting particles in porous materials. Different expressions for the particle jump rates are derived from transition state theory. Which expression should be used depends on the strength of the inter-particle interactions. Analytical expressions for the self- and transport diffusion are derived when correlations, caused by memory effects in the environment, are neglected. The diffusive behavior is studied numerically with kinetic Monte Carlo (kMC) simulations, which reproduces the diffusion including correlations. The effect of correlations is studied by comparing the analytical expressions with the kMC simulations. It is found that the Maxwell-Stefan diffusion can exceed the self-diffusion. To our knowledge, this is the first time this is observed. The diffusive behavior in one-dimensional and higher dimensional systems is qualitatively the same, with the effect of correlations decreasing for increasing dimension. The length dependence of both the self- and transport diffusion is studied for one-dimensional systems. For long lengths the self-diffusion shows a one over length dependence. Finally, we discuss when agreement with experiments and simulations can be expected. The assumption that particles in different cavities do not interact is expected to hold quantitatively at low and medium particle concentrations, if the particles are not strongly interacting.Comment: (18 pages, 16 figures, published version