875 research outputs found
Microspectroscopy and Imaging in the THz Range Using Coherent CW Radiation
A novel THz near-field spectrometer is presented which allows to perform
biological and medical studies with high spectral resolution combined with a
spatial resolution down to l/100. In the setup an aperture much smaller than
the used wavelength is placed in the beam very close to the sample. The sample
is probed by the evanescent wave behind the aperture. The distance is measured
extremely accurate by a confocal microscope. We use monochromatic sources which
provide powerful coherent cw radiation tuneable from 50 GHz up to 1.5 THz.
Transmission and reflection experiments can be performed which enable us to
study solids and molecules in aqueous solution. Examples for spectroscopic
investigations on biological tissues are presented.Comment: 4 pages, 5 figures, email: [email protected]
Mobility gap in intermediate valent TmSe
The infrared optical conductivity of intermediate valence compound TmSe
reveals clear signatures for hybridization of light - and heavy f-electronic
states with m* ~ 1.6 m_0 and m* ~ 16 m_0, respectively. At moderate and high
temperatures, the metal-like character of the heavy carriers dominate the
low-frequency response while at low temperatures (T_N < T < 100 K) a gap-like
feature is observed in the conductivity spectra below 10 meV which is assigned
to be a mobility gap due to localization of electrons on local Kondo singlets,
rather than a hybridization gap in the density of states
Analysis of broadband microwave conductivity and permittivity measurements of semiconducting materials
We perform broadband phase sensitive measurements of the reflection
coefficient from 45 MHz up to 20 GHz employing a vector network analyzer with a
2.4 mm coaxial sensor which is terminated by the sample under test. While the
material parameters (conductivity and permittivity) can be easily extracted
from the obtained impedance data if the sample is metallic, no direct solution
is possible if the material under investigation is an insulator. Focusing on
doped semiconductors with largely varying conductivity, here we present a
closed calibration and evaluation procedure for frequencies up to 5 GHz, based
on the rigorous solution for the electromagnetic field distribution inside the
sample combined with the variational principle; basically no limiting
assumptions are necessary. A simple static model based on the electric current
distribution proves to yield the same frequency dependence of the complex
conductivity up to 1 GHz. After a critical discussion we apply the developed
method to the hopping transport in Si:P at temperature down to 1 K.Comment: 9 pages, 10 figures, accepted for publication in the Journal of
Applied Physic
Evidence for a Bulk Complex Order-Parameter in Y0.9Ca0.1Ba2Cu3O7-delta Thin Films
We have measured the penetration depth of overdoped Y0.9Ca0.1Ba2Cu3O7-delta
(Ca-YBCO) thin films using two different methods. The change of the penetration
depth as a function of temperature has been measured using the parallel plate
resonator (PPR), while its absolute value was obtained from a quasi-optical
transmission measurements. Both sets of measurements are compatible with an
order parameter of the form: Delta*dx2-y2+i*delta*dxy, with Delta=14.5 +- 1.5
meV and delta=1.8 meV, indicating a finite gap at low temperature. Below 15 K
the drop of the scattering rate of uncondensed carriers becomes steeper in
contrast to a flattening observed for optimally doped YBCO films. This decrease
supports our results on the penetration depth temperature dependence. The
findings are in agreement with tunneling measurements on similar Ca-YBCO thin
films.Comment: 11 pages, 4 figure
Spin excitations of the correlated semiconductor FeSi probed by THz radiation
By direct measurements of the complex optical conductivity of
FeSi we have discovered a broad absorption peak centered at frequency
that develops at temperatures below 20 K.
This feature is caused by spin-polaronic states formed in the middle of the gap
in the electronic density of states. We observe the spin excitations between
the electronic levels split by the exchange field of . Spin
fluctuations are identified as the main factor determining the formation of the
spin polarons and the rich magnetic phase diagram of FeSi.Comment: 5 pages, 4 figure
Linear-in-frequency optical conductivity in GdPtBi due to transitions near the triple points
The complex optical conductivity of the half-Heusler compound GdPtBi is
measured in a frequency range from 20 to 22 000 cm (2.5 meV - 2.73 eV)
at temperatures down to 10 K in zero magnetic field. We find the real part of
the conductivity, , to be almost perfectly linear in
frequency over a broad range from 50 to 800 cm ( 6 - 100 meV) for
K. This linearity strongly suggests the presence of
three-dimensional linear electronic bands with band crossings (nodes) near the
chemical potential. Band-structure calculations show the presence of triple
points, where one doubly degenerate and one nondegenerate band cross each other
in close vicinity of the chemical potential. From a comparison of our data with
the optical conductivity computed from the band structure, we conclude that the
observed nearly linear originates as a cumulative effect
from all the transitions near the triple points.Comment: 5+ pages, 5 figures, band-structure and optical-conductivity
calculations adde
Origin of Low-Energy Excitations in Charge-Ordered Manganites
The low-energy excitations in the charge-ordered phase of polycrystalline
La0.25Ca0.75MnO3 are explored by frequency-domain terahertz spectroscopy. In
the frequency range from 4 cm^-1 to 700 cm^-1 (energies 0.4 meV to 90 meV) and
at temperatures down to 5 K, we do not detect any feature that can be
associated with the collective response of the spatially modulated charge
continuum. In the antiferromagnetically ordered phase, broad absorption bands
appear in the conductivity and permittivity spectra around 30 cm^-1 and 100
cm^-1 which are assigned to former acoustic phonons optically activated due to
a fourfold superstructure in the crystal lattice. Our results indicate that
characteristic energies of collective excitations of the charge-ordered phase
in La0:25Ca0:75MnO3, if any, lie below 1 meV. At our lowest frequencies of only
few wavenumbers a strong relaxation is observed above 100 K connected to the
formation of the charge-ordered state.Comment: 5 pages, 3 figure
Two-channel conduction in YbPtBi
We investigated transport, magnetotransport, and broadband optical properties
of the half-Heusler compound YbPtBi. Hall measurements evidence two types of
charge carriers: highly mobile electrons with a temperature-dependent
concentration and low-mobile holes; their concentration stays almost constant
within the investigated temperature range from 2.5 to 300 K. The optical
spectra (10 meV - 2.7 eV) can be naturally decomposed into contributions from
intra- and interband absorption processes, the former manifesting themselves as
two Drude bands with very different scattering rates, corresponding to the
charges with different mobilities. These results of the optical measurements
allow us to separate the contributions from electrons and holes to the total
conductivity and to implement a two-channel-conduction model for description of
the magnetotransport data. In this approach, the electron and hole mobilities
are found to be around 50000 and 10 cm/Vs at the lowest temperatures (2.5
K), respectively.Comment: 6 page
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