A New Model for the Hard Time Lags in Black Hole X-Ray Binaries

The time-dependent Comptonized output of a cool soft X-ray source drifting inward through an inhomogeneous hot inner disk or corona is numerically simulated. We propose that this scenario can explain from first principles the observed trends in the hard time lags and power spectra of the rapid aperiodic variability of the X-ray emission of Galactic black-hole candidates.Comment: 10 pages, including 2 figures; uses epsf.sty, rotate.sty; accepted for ApJ Letter

Conversion of relativistic pair energy into radiation in the jets of active galactic nuclei

It is generally accepted that relativistic jet outflows power the nonthermal emission from active galactic nuclei (AGN). The composition of these jets -- leptonic versus hadronic -- is still under debate. We investigate the microphysical details of the conversion process of the kinetic energy in collimated relativistic pair outflows into radiation through interactions with the ambient interstellar medium. Viewed from the coordinate system comoving with the pair outflow, the interstellar protons and electrons represent a proton-electron beam propagating with relativistic speed in the pair plasma. We demonstrate that the beam excites both electrostatic and low-frequency magnetohydrodynamic Alfven-type waves via a two-stream instability in the pair background plasma, and we calculate the time evolution of the distribution functions of the beam particles and the generated plasma wave turbulence power spectra. For standard AGN jet outflow and environment parameters we show that the initial beam distributions of interstellar protons and electrons quickly relax to plateau-distributions in parallel momentum, transferring thereby one-half of the initial energy density of the beam particles to electric field fluctuations of the generated electrostatic turbulence. On considerably longer time scales, the plateaued interstellar electrons and protons will isotropise by their self-generated transverse turbulence and thus be picked-up in the outflow pair plasma. These longer time scales are also characteristic for the development of transverse hydromagnetic turbulence from the plateaued electrons and protons. This hydromagnetic turbulence upstream and downstream is crucial for diffusive shock acceleration to operate at external or internal shocks associated with pair outflows.Comment: A&A in pres

Metastable precursors during the oxidation of the Ru(0001) surface

Using density-functional theory, we predict that the oxidation of the Ru(0001) surface proceeds via the accumulation of sub-surface oxygen in two-dimensional islands between the first and second substrate layer. This leads locally to a decoupling of an O-Ru-O trilayer from the underlying metal. Continued oxidation results in the formation and stacking of more of these trilayers, which unfold into the RuO_2(110) rutile structure once a critical film thickness is exceeded. Along this oxidation pathway, we identify various metastable configurations. These are found to be rather close in energy, indicating a likely lively dynamics between them at elevated temperatures, which will affect the surface chemical and mechanical properties of the material.Comment: 11 pages including 9 figures. Submitted to Phys. Rev. B. Related publications can be found at http://www.fhi-berlin.mpg.de/th/paper.htm

Equation of Motion for the Solvent Polarization Apparent Charges in the Polarizable Continuum Model: Application to Time-Dependent CI

The dynamics of the electrons for a molecule in solution is coupled to the dynamics of its polarizable environment, i.e., the solvent. To theoretically investigate such electronic dynamics, we have recently developed equations of motion (EOM) for the apparent solvent polarization charges that generate the reaction field in the Polarizable Continuum Model (PCM) for solvation and we have coupled them to a real-time time-dependent density functional theory (RT TDDFT) description of the solute [Corni et al. J. Phys. Chem. A 119, 5405 (2014)]. Here we present an extension of the EOM-PCM approach to a Time-Dependent Configuration Interaction (TD CI) description of the solute dynamics, which is free from the qualitative artifacts of RT TDDFT in the adiabatic approximation. As tests of the developed approach, we investigate the solvent Debye relaxation after an electronic excitation of the solute obtained either by a $\pi$ pulse of light or by assuming the idealized sudden promotion to the excited state. Moreover, we present EOM for the Onsager solvation model and we compare the results with PCM. The developed approach provides qualitatively correct real-time evolutions and is promising as a general tool to investigate the electron dynamics elicited by external electromagnetic fields for molecules in solution.Comment: This is the final peer-reviewed manuscript accepted for publication in The Journal of Chemical Physics. Copyright by AIP, the final published version can be found at http://scitation.aip.org/content/aip/journal/jcp/146/6/10.1063/1.497562

The long-term optical spectral variability of BL Lacertae

We present the results from a study of the long-term optical spectral variations of BL Lacertae, using the long and well-sampled B and R-band light curves of the Whole Earth Blazar Telescope (WEBT) collaboration, binned on time intervals of 1 day. The relation between spectral slope and flux (the spectrum gets bluer as the source flux increases) is well described by a power-law model, although there is significant scatter around the best-fitting model line. To some extent, this is due to the spectral evolution of the source (along well-defined loop-like structures) during low-amplitude events, which are superimposed on the major optical flares, and evolve on time scales of a few days. The "bluer-when-brighter" mild chromatism of the long-term variations of the source can be explained if the flux increases/decreases faster in the B than in the R band. The B and R-band variations are well correlated, with no significant, measurable delays larger than a few days. On the other hand, we find that the spectral variations lead those in the flux light curves by ~ 4 days. Our results can be explained in terms of Doppler factor variations due to changes in the viewing angle of a curved and inhomogeneous emitting jet.Comment: 7 pages, 5 figures, accepted for publication in A&

Investigation of the shear-mechanical and dielectric relaxation processes in two mono-alcohols close to the glass transition

Shear-mechanical and dielectric measurements on the two monohydroxy (mono-alcohol) molecular glass formers 2-ethyl-1-hexanol and 2-butanol close to the glass transition temperature are presented. The shear-mechanical data are obtained using the piezoelectric shear-modulus gauge method covering frequencies from 1mHz to 10kHz. The shear-mechanical relaxation spectra show two processes, which follow the typical scenario of a structural (alpha) relaxation and an additional (Johari-Goldstein) beta relaxation. The dielectric relaxation spectra are dominated by a Debye-type peak with an additional non-Debye peak visible. This Debye-type relaxation is a common feature peculiar to mono-alcohols. The time scale of the non-Debye dielectric relaxation process is shown to correspond to the mechanical structural (alpha) relaxation. Glass-transition temperatures and fragilities are reported based on the mechanical alpha relaxation and the dielectric Debye-type process, showing that the two glass-transition temperatures differ by approximately 10K and that the fragility based on the Debye-type process is a factor of two smaller than the structural fragility. If a mechanical signature of the Debye-type relaxation exists in these liquids, its relaxation strength is at most 1% and 3% of the full relaxation strength of 2-butanol and 2-ethyl-1-hexanol respectively. These findings support the notion that it is the non-Debye dielectric relaxation process that corresponds to the structural alpha relaxation in the liquid.Comment: 8 pages, 6 figures. Minor corrections, updated figures, more dielectric data show

H.E.S.S. discovery of very-high-energy gamma-ray emission of PKS 1440-389

Blazars are the most abundant class of known extragalactic very-high-energy (VHE, E>100 GeV) gamma-ray sources. However, one of the biggest difficulties in investigating their VHE emission resides in their limited number, since less than 60 of them are known by now. In this contribution we report on H.E.S.S. observations of the BL Lac object PKS 1440-389. This source has been selected as target for H.E.S.S. based on its high-energy gamma-ray properties measured by Fermi-LAT. The extrapolation of this bright, hard-spectrum gamma-ray blazar into the VHE regime made a detection on a relatively short time scale very likely, despite its uncertain redshift. H.E.S.S. observations were carried out with the 4-telescope array from February to May 2012 and resulted in a clear detection of the source. Contemporaneous multi-wavelength data are used to construct the spectral energy distribution of PKS 1440-389 which can be described by a simple one-zone synchrotron-self Compton model.Comment: In Proceedings of the 34th International Cosmic Ray Conference (ICRC2015), The Hague, The Netherland