Theory of Branching and Annihilating Random Walks

A systematic theory for the diffusion--limited reaction processes $A + A \to 0$ and $A \to (m+1) A$ is developed. Fluctuations are taken into account via the field--theoretic dynamical renormalization group. For $m$ even the mean field rate equation, which predicts only an active phase, remains qualitatively correct near $d_c = 2$ dimensions; but below $d_c' \approx 4/3$ a nontrivial transition to an inactive phase governed by power law behavior appears. For $m$ odd there is a dynamic phase transition for any $d \leq 2$ which is described by the directed percolation universality class.Comment: 4 pages, revtex, no figures; final version with slight changes, now accepted for publication in Phys. Rev. Let

Interacting Monomer-Dimer Model with Infinitely Many Absorbing States

We study a modified version of the interacting monomer-dimer (IMD) model that has infinitely many absorbing (IMA) states. Unlike all other previously studied models with IMA states, the absorbing states can be divided into two equivalent groups which are dynamically separated infinitely far apart. Monte Carlo simulations show that this model belongs to the directed Ising universality class like the ordinary IMD model with two equivalent absorbing states. This model is the first model with IMA states which does not belong to the directed percolation (DP) universality class. The DP universality class can be restored in two ways, i.e., by connecting the two equivalent groups dynamically or by introducing a symmetry-breaking field between the two groups.Comment: 5 pages, 5 figure

Numerical Study of a Field Theory for Directed Percolation

A numerical method is devised for study of stochastic partial differential equations describing directed percolation, the contact process, and other models with a continuous transition to an absorbing state. Owing to the heightened sensitivity to fluctuationsattending multiplicative noise in the vicinity of an absorbing state, a useful method requires discretization of the field variable as well as of space and time. When applied to the field theory for directed percolation in 1+1 dimensions, the method yields critical exponents which compare well against accepted values.Comment: 18 pages, LaTeX, 6 figures available upon request LC-CM-94-00

Nonequilibrium Critical Dynamics of a Three Species Monomer-Monomer Model

We study a three species monomer-monomer catalytic surface reaction model with a reactive steady state bordered by three equivalent unreactive phases where the surface is saturated with one species. The transition from the reactive to a saturated phase shows directed percolation critical behavior. Each pair of these reactive-saturated phase boundaries join at a bicritical point where the universal behavior is in the even branching annihilating random walk class. We find the crossover exponent from bicritical to critical behavior and a new exponent associated with the bicritical interface dynamics.Comment: 4 pages RevTex. 4 eps figures included with psfig.sty. Uses multicol.sty. Accepted for publication in PR

Does hardcore interaction change absorbing type critical phenomena?

It has been generally believed that hardcore interaction is irrelevant to absorbing type critical phenomena because the particle density is so low near an absorbing phase transition. We study the effect of hardcore interaction on the N species branching annihilating random walks with two offspring and report that hardcore interaction drastically changes the absorbing type critical phenomena in a nontrivial way. Through Langevin equation type approach, we predict analytically the values of the scaling exponents, $\nu_{\perp} = 2, z = 2, \alpha = 1/2, \beta = 2$ in one dimension for all N > 1. Direct numerical simulations confirm our prediction. When the diffusion coefficients for different species are not identical, $\nu_{\perp}$ and $\beta$ vary continuously with the ratios between the coefficients.Comment: 4 pages, 1 figur

Criticality of natural absorbing states

We study a recently introduced ladder model which undergoes a transition between an active and an infinitely degenerate absorbing phase. In some cases the critical behaviour of the model is the same as that of the branching annihilating random walk with $N\geq 2$ species both with and without hard-core interaction. We show that certain static characteristics of the so-called natural absorbing states develop power law singularities which signal the approach of the critical point. These results are also explained using random walk arguments. In addition to that we show that when dynamics of our model is considered as a minimum finding procedure, it has the best efficiency very close to the critical point.Comment: 6 page

Damage spreading for one-dimensional, non-equilibrium models with parity conserving phase transitions

The damage spreading (DS) transitions of two one-dimensional stochastic cellular automata suggested by Grassberger (A and B) and the kinetic Ising model of Menyh\'ard (NEKIM) have been investigated on the level of kinks and spins. On the level of spins the parity conservation is not satisfied and therefore studying these models provides a convenient tool to understand the dependence of DS properties on symmetries. For the model B the critical point and the DS transition point is well separated and directed percolation damage spreading transition universality was found for spin damage as well as for kink damage in spite of the conservation of damage variables modulo 2 in the latter case. For the A stochastic cellular automaton, and the NEKIM model the two transition points coincide with drastic effects on the damage of spin and kink variables showing different time dependent behaviours. While the kink DS transition is continuous and shows regular PC class universality, the spin damage exhibits a discontinuous phase transition with compact clusters and PC like dynamical scaling ($\eta^,$), ($\delta_s$) and ($z_s$) exponents whereas the static exponents determined by FSS are consistent with that of the spins of the NEKIM model at the PC transition point. The generalised hyper-scaling law is satisfied.Comment: 11 pages, 20 figures embedded in the text, minor changes in the text, a new table and new references are adde

One-dimensional Nonequilibrium Kinetic Ising Models with local spin-symmetry breaking: N-component branching annihilation transition at zero branching rate

The effects of locally broken spin symmetry are investigated in one dimensional nonequilibrium kinetic Ising systems via computer simulations and cluster mean field calculations. Besides a line of directed percolation transitions, a line of transitions belonging to N-component, two-offspring branching annihilating random-walk class (N-BARW2) is revealed in the phase diagram at zero branching rate. In this way a spin model for N-BARW2 transitions is proposed for the first time.Comment: 6 pages, 5 figures included, 2 new tables added, to appear in PR

Cation distribution in manganese cobaltite spinels Co3−xMnxO4 (0 ≤ x ≤ 1) determined by thermal analysis

Thermogravimetric analysis was used in order to study the reduction in air of submicronic powders of Co3−x Mn x O4 spinels, with 0 ≤ x ≤ 1. For x = 0 (i.e. Co3O4), cation reduction occurred in a single step. It involved the CoIII ions at the octahedral sites, which were reduced to Co2+ on producing CoO. For 0 < x ≤ 1, the reduction occurred in two stages at increasing temperature with increasing amounts of manganese. The first step corresponded to the reduction of octahedral CoIII ions and the second was attributed to the reduction of octahedral Mn4+ ions to Mn3+. From the individual weight losses and the electrical neutrality of the lattice, the CoIII and Mn4+ ion concentrations were calculated. The distribution of cobalt and manganese ions present on each crystallographic site of the spinel was determined. In contrast to most previous studies that took into account either CoIII and Mn3+ or Co2+, CoIII and Mn4+ only, our thermal analysis study showed that Co2+/CoIII and Mn3+/Mn4+ pairs occupy the octahedral sites. These results were used to explain the resistivity measurements carried out on dense ceramics prepared from our powders sintered at low temperature (700–750 °C) in a Spark Plasma Sintering apparatus

The three species monomer-monomer model: A mean-field analysis and Monte Carlo study

We study the phase diagram and critical behavior of a one dimensional three species monomer-monomer surface reaction model. Static Monte Carlo simulations show a phase diagram consisting of a reactive steady state bordered by three equivalent unreactive phases where the surface is saturated with one monomer species. The transitions from the reactive to saturated phases are all continuous, while the transitions between poisoned phases are first-order, with bicritical points where the reactive phase meets two poisoned phases. A mean-field cluster analysis predicts all of the qualitative features of the phase diagram only when correlations up to triplets of adjacent sites are included. Dynamic Monte Carlo simulations show that the transition from the reactive to a saturated phase show critical behavior in the directed percolation universality class, while the bicritical point shows critical behavior in the even branching annihilating random walk class. The crossover from bicritical to critical behavior is also studied.Comment: 16 pages using RevTeX, plus 10 figures. Uses psfig.st