Reaction cross sections for proton scattering from stable and unstable nuclei based on a microscopic approach

Microscopic optical model potential results for reaction cross sections of proton elastic scattering are presented. The applications cover the 10-1000 MeV energy range and consider both stable and unstable nuclei. The study is based on in-medium g-matrix full-folding optical model approach with the appropriate relativistic kinematic corrections needed for the higher energy applications. The effective interactions are based on realistic NN potentials supplemented with a separable non-Hermitian term to allow optimum agreement with current NN phase-shift analyzes, particularly the inelasticities above pion production threshold. The target ground-state densities are obtained from Hartree-Fock-Bogoliubov calculations based on the finite range, density dependent Gogny force. The evaluated reaction cross sections for proton scattering are compared with measurements and their systematics is analyzed. A simple function of the total cross sections in terms of the atomic mass number is observed at high energies. At low energies, however, discrepancies with the available data are observed, being more pronounced in the lighter systems.Comment: 11 pages, 4 figures, submitted to Phys. Rev.

Microscopic analysis of K^+-nucleus elastic scattering based on K^+N phase shifts

We investigate $K^{+}$-nucleus elastic scattering at intermediate energies within a microscopic optical model approach. To this effect we use the current $K^{+}$-nucleon {\it (KN)} phase shifts from the Center for Nuclear Studies of the George Washington University as primary input. First, the {\it KN} phase shifts are used to generate Gel'fand-Levitan-Marchenko real and local inversion potentials. Secondly, these potentials are supplemented with a short range complex separable term in such a way that the corresponding unitary and non-unitary {\it KN} $S$ matrices are exactly reproduced. These {\it KN} potentials allow to calculate all needed on- and off-shell contributions of the $t$ matrix,the driving effective interaction in the full-folding $K^{+}$-nucleus optical model potentials reported here. Elastic scattering of positive kaons from $^{6}$Li, $^{12}$C, $^{28}$Si and $^{40}$Ca are studied at beam momenta in the range 400-1000 MeV/{$c$}, leading to a fair description of most differential and total cross section data. To complete the analysis the full-folding model, three kinds of simpler $t\rho$ calculations are considered and results discussed. We conclude that conventional medium effects, in conjunction with a proper representation of the basic {\it KN} interaction are essential for the description of $K^{+}$-nucleus phenomena.Comment: 11 pages, 1 table, 12 figures, submitted to PR

Nuclear halo structure from quasielastic charge-exchange reactions

Neutron and proton densities in the nuclear periphery are investigated within (p,n) charge-exchange isobar transitions. For this purpose we have developed parameter-free optical potentials with a detailed treatment of the in-medium $t_{\tau}$ part of the effective interaction. Non local coupled-channel Lane equations are solved to obtain the scattering observables. The use of conventional proton and neutron densities significantly underestimates Fermi (forward-angle) cross-sections in agreement with findings by various other groups. However, we have found model-independent densities which provide a remarkable improvement in the description of the quasielastic scattering data.The densities obtained are consistent with recent measurements at CERN in studies of the neutron-to-proton halo factor f(r)=Z$\rho_n/N\rho_p$ with antiprotons. These findings provide an alternative way to investigate the nuclear periphery, and may also help to solve the long-standing puzzle of the underestimated Fermi cross section in (p,n) charge-exchange phenomena.Comment: 5 pages and 2 figs. Presented at the Baryons-04 Conference (Palaiseau, France, Oct 2004). To appear in Nucl. Phys.

Sensitivity of nucleon-nucleus scattering to the off-shell behavior of on-shell equivalent NN potentials

The sensitivity of nucleon-nucleus elastic scattering to the off-shell behavior of realistic nucleon-nucleon interactions is investigated when on-shell equivalent nucleon-nucleon potentials are used. The study is based on applications of the full-folding optical model potential for an explicit treatment of the off-shell behavior of the nucleon-nucleon effective interaction. Applications were made at beam energies between 40 and 500 MeV for proton scattering from 40Ca and 208Pb. We use the momentum-dependent Paris potential and its local on-shell equivalent as obtained with the Gelfand-Levitan and Marchenko inversion formalism for the two nucleon Schroedinger equation. Full-folding calculations for nucleon-nucleus scattering show small fluctuations in the corresponding observables. This implies that off-shell features of the NN interaction cannot be unambiguously identified with these processes. Inversion potentials were also constructed directly from NN phase-shift data (SM94) in the 0-1.3 GeV energy range. Their use in proton-nucleus scattering above 200 MeV provide a superior description of the observables relative to those obtained from current realistic NN potentials. Limitations and scope of our findings are presented and discussed.Comment: 17 pages tightened REVTeX, 8 .ps figures, submitted to Phys. Rev.

Hydrophobic RWGS catalysts: Valorization of CO2-rich streams in presence of CO/H2O

Nowadays, the majority of the Reverse Water Gas Shift (RWGS) studies assume somehow model feedstock (diluted CO2/H2) for syngas production. Nonetheless, biogas streams contain certain amounts of CO/H2O which will decrease the obtained CO2 conversion values by promoting the forward WGS reaction. Since the rate limiting step for the WGS reaction concerns the water splitting, this work proposes the use of hydrophobic RWGS catalysts as an effective strategy for the valorization of CO2-rich feedstock in presence of H2O and CO. Over Fe-Mg catalysts, the different hydrophilicities attained over pristine, N- and B-doped carbonaceous supports accounted for the impact on the activity of the catalyst in presence of CO/H2O. Overall, the higher CO productivity (4.12 μmol/(min·m2)) attained by Fe-Mg/CDC in presence of 20 % of H2O relates to hindered water adsorption and unveil the use of hydrophobic surfaces as a suitable approach for avoiding costly pre-conditioning units for the valorization of CO2-rich streams based on RWGS processes in presence of CO/H2O