1,527 research outputs found
Dynamic Radio-Frequency Transverse Susceptibility in Magnetic Nanoparticle Systems
A novel resonant method based on a tunnel-diode oscillator (TDO) is used to
study the dynamic transverse susceptibility in a Fe nanoparticle system. The
magnetic system consists of an aggregate of nanometer-size core (Au)-shell (Fe)
structure, synthesized by reverse micelle methods. Static and dynamic
magnetization measurements carried out in order to characterize the system
reveal a superparamagnetic behavior at high temperature. The field-dependent
transverse susceptibility at radio-frequencies (RF), for different temperatures
reveals distinct peak structure at characteristics fields (H_k, H_c) which
changes with temperature. It is proposed that relaxation processes could
explain the influence of the temperature on the field dependence of the
transverse susceptibility on the MI.Comment: 3 pages, 2-column, 3 figures, To be published in J. Appl. Phys. 2000
(44th Annual MMM proceedings
Finite-size versus Surface effects in nanoparticles
We study the finite-size and surface effects on the thermal and spatial
behaviors of the magnetisation of a small magnetic particle. We consider two
systems: 1) A box-shaped isotropic particle of simple cubic structure with
either periodic or free boundary conditions. This case is treated analytically
using the isotropic model of D-component spin vectors in the limit , including the magnetic field. 2) A more realistic particle (-FeO) of ellipsoidal (or spherical) shape with open boundaries.
The magnetic state in this particle is described by the anisotropic classical
Dirac-Heisenberg model including exchange and dipolar interactions, and bulk
and surface anisotropy. This case is dealt with by the classical Monte Carlo
technique. It is shown that in both systems finite-size effects yield a
positive contribution to the magnetisation while surface effects render a
larger and negative contribution, leading to a net decrease of the
magnetisation of the small particle with respect to the bulk system. In the
system 2) the difference between the two contributions is enhanced by surface
anisotropy. The latter also leads to non saturation of the magnetisation at low
temperatures, showing that the magnetic order in the core of the particle is
perturbed by the magnetic disorder on the surface. This is confirmed by the
profile of the magnetisation.Comment: 6 pages of RevTex including 4 Figures, invited paper to 3rd
EuroConference on Magnetic Properties of Fine Nanoparticles, Barcelona,
October 9
Scaling relations for magnetic nanoparticles
A detailed investigation of the scaling relations recently proposed by [J.
d'Albuquerque e Castro, D. Altbir, J. C. Retamal, and P. Vargas, Phys. Rev.
Lett. 88, 237202 (2002)] to study the magnetic properties of nanoparticles is
presented. Analytical expressions for the total energy of three characteristic
internal configurations of the particles are obtained, in terms of which the
behavior of the magnetic phase diagram for those particles upon scaling of the
exchange interaction is discussed. The exponent in scaling relations is
shown to be dependent on the geometry of the vortex core, and results for
specific cases are presented.Comment: 6 pages, 4 figure
Integral Relaxation Time of Single-Domain Ferromagnetic Particles
The integral relaxation time \tau_{int} of thermoactivating noninteracting
single-domain ferromagnetic particles is calculated analytically in the
geometry with a magnetic field H applied parallel to the easy axis. It is shown
that the drastic deviation of \tau_{int}^{-1} from the lowest eigenvalue of the
Fokker-Planck equation \Lambda_1 at low temperatures, starting from some
critical value of H, is the consequence of the depletion of the upper potential
well. In these conditions the integral relaxation time consists of two
competing contributions corresponding to the overbarrier and intrawell
relaxation processes.Comment: 8 pages, 3 figure
XAX: a multi-ton, multi-target detection system for dark matter, double beta decay and pp solar neutrinos
A multi-target detection system XAX, comprising concentric 10 ton targets of
136Xe and 129/131Xe, together with a geometrically similar or larger target of
liquid Ar, is described. Each is configured as a two-phase
scintillation/ionization TPC detector, enhanced by a full 4pi array of
ultra-low radioactivity Quartz Photon Intensifying Detectors (QUPIDs) replacing
the conventional photomultipliers for detection of scintillation light. It is
shown that background levels in XAX can be reduced to the level required for
dark matter particle (WIMP) mass measurement at a 10^-10 pb WIMP-nucleon cross
section, with single-event sensitivity below 10^-11 pb. The use of multiple
target elements allows for confirmation of the A^2 dependence of a coherent
cross section, and the different Xe isotopes provide information on the
spin-dependence of the dark matter interaction. The event rates observed by Xe
and Ar would modulate annually with opposite phases from each other for WIMP
mass >~100 GeV/c^2. The large target mass of 136Xe and high degree of
background reduction allow neutrinoless double beta decay to be observed with
lifetimes of 10^27-10^28 years, corresponding to the Majorana neutrino mass
range 0.01-0.1 eV, the most likely range from observed neutrino mass
differences. The use of a 136Xe-depleted 129/131Xe target will also allow
measurement of the pp solar neutrino spectrum to a precision of 1-2%.Comment: 16 pages with 17 figure
The Formation and Coarsening of the Concertina Pattern
The concertina is a magnetization pattern in elongated thin-film elements of
a soft material. It is a ubiquitous domain pattern that occurs in the process
of magnetization reversal in direction of the long axis of the small element.
Van den Berg argued that this pattern grows out of the flux closure domains as
the external field is reduced. Based on experimental observations and theory,
we argue that in sufficiently elongated thin-film elements, the concertina
pattern rather bifurcates from an oscillatory buckling mode. Using a reduced
model derived by asymptotic analysis and investigated by numerical simulation,
we quantitatively predict the average period of the concertina pattern and
qualitatively predict its hysteresis. In particular, we argue that the
experimentally observed coarsening of the concertina pattern is due to
secondary bifurcations related to an Eckhaus instability. We also link the
concertina pattern to the magnetization ripple and discuss the effect of a weak
(crystalline or induced) anisotropy
Magnetic irreversibility and Verwey transition in nano-crystalline bacterial magnetite
The magnetic properties of biologically-produced magnetite nanocrystals
biomineralized by four different magnetotactic bacteria were compared to those
of synthetic magnetite nanocrystals and large, high quality single crystals.
The magnetic feature at the Verwey temperature, , was clearly seen in
all nanocrystals, although its sharpness depended on the shape of individual
nanoparticles and whether or not the particles were arranged in magnetosome
chains. The transition was broader in the individual superparamagnetic
nanoparticles for which , where is the superparamagnetic
blocking temperature. For the nanocrystals organized in chains, the effective
blocking temperature and the Verwey transition is sharply
defined. No correlation between the particle size and was found.
Furthermore, measurements of suggest that magnetosome chains
behave as long magnetic dipoles where the local magnetic field is directed
along the chain and this result confirms that time-logarithmic magnetic
relaxation is due to the collective (dipolar) nature of the barrier for
magnetic moment reorientation
Thermal fluctuations and longitudinal relaxation of single-domain magnetic particles at elevated temperatures
We present numerical and analytical results for the swiching times of
magnetic nanoparticles with uniaxial anisotropy at elevated temperatures,
including the vicinity of T_c. The consideration is based in the
Landau-Lifshitz-Bloch equation that includes the relaxation of the
magnetization magnitude M. The resulting switching times are shorter than those
following from the naive Landau-Lifshitz equation due to (i) additional barrier
lowering because of the reduction of M at the barrier and (ii) critical
divergence of the damping parameters.Comment: 4 PR pages, 1 figur
Increased Expression of Tissue Factor and Receptor for Advanced Glycation End Products in Peripheral Blood Mononuclear Cells of Patients With Type 2 Diabetes Mellitus with Vascular Complications
The aim of the study was to determine the correlation between
the expression of tissue factor (TF) and the receptor
for advanced glycation end products (RAGEs) and vascular
complications in patients with longstanding uncontrolled
type 2 diabetes (T2D). TF and RAGE mRNAs as well as
TF antigen and activity were investigated in 21 T2D patients
with and without vascular complications. mRNA expression
was assessed by reverse transcriptaseâpolymerase
chain reaction (RT-PCR) in nonstimulated and advanced
glycation end product (AGE) albuminâstimulated peripheral
blood mononuclear cells (PBMCs). TF antigen expression
was determined by enzyme-linked immunosorbent assay
(ELISA) and TF activity by a modified prothrombin
time assay. Basal RAGE mRNA expression was 0.2 ± 0.06
in patients with complications and 0.05 ± 0.06 patients without
complications (P = .004). Stimulation did not cause any
further increase in either group. TF mRNA was 0.58 ± 0.29
in patients with complications and 0.21 ± 0.18 in patients
without complications (P = .003). Stimulation resulted in
a nonsignificant increase in both groups. Basal TF activity
(U/106 PBMCs) was 18.4 ± 13.2 in patients with complications
and 6.96 ± 5.2 in patients without complications (P =
.003). It increased 3-fold in both groups after stimulation
(P = .001). TF antigen (pg/106 PBMCs) was 33.7 ± 28.6 in
patients with complications, 10.4 ± 7.8 in patients without complications (P = .02). Stimulation tripled TF antigen in
both groups of patients (P = .001). The RAGE/TF axis is
up-regulated inT2Dpatients with vascular complications as
compared to patients without complications. This suggests
a role for this axis in the pathogenesis of vascular complications
in T2D
Nanostratification of optical excitation in self-interacting 1D arrays
The major assumption of the Lorentz-Lorenz theory about uniformity of local
fields and atomic polarization in dense material does not hold in finite groups
of atoms, as we reported earlier [A. E. Kaplan and S. N. Volkov, Phys. Rev.
Lett., v. 101, 133902 (2008)]. The uniformity is broken at sub-wavelength
scale, where the system may exhibit strong stratification of local field and
dipole polarization, with the strata period being much shorter than the
incident wavelength. In this paper, we further develop and advance that theory
for the most fundamental case of one-dimensional arrays, and study nanoscale
excitation of so called "locsitons" and their standing waves (strata) that
result in size-related resonances and related large field enhancement in finite
arrays of atoms. The locsitons may have a whole spectrum of spatial
frequencies, ranging from long waves, to an extent reminiscent of ferromagnetic
domains, -- to super-short waves, with neighboring atoms alternating their
polarizations, which are reminiscent of antiferromagnetic spin patterns. Of
great interest is the new kind of "hybrid" modes of excitation, greatly
departing from any magnetic analogies. We also study differences between
Ising-like near-neighbor approximation and the case where each atom interacts
with all other atoms in the array. We find an infinite number of "exponential
eigenmodes" in the lossless system in the latter case. At certain "magic"
numbers of atoms in the array, the system may exhibit self-induced (but linear
in the field) cancellation of resonant local-field suppression. We also studied
nonlinear modes of locsitons and found optical bistability and hysteresis in an
infinite array for the simplest modes.Comment: 39 pages, 5 figures; v2: Added the Conclusions section, corrected a
typo in Eq. (5.3), corrected minor stylistic and grammatical imperfection
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