18 research outputs found
Quantum phase transition in a single-molecule quantum dot
Quantum criticality is the intriguing possibility offered by the laws of
quantum mechanics when the wave function of a many-particle physical system is
forced to evolve continuously between two distinct, competing ground states.
This phenomenon, often related to a zero-temperature magnetic phase transition,
can be observed in several strongly correlated materials such as heavy fermion
compounds or possibly high-temperature superconductors, and is believed to
govern many of their fascinating, yet still unexplained properties. In contrast
to these bulk materials with very complex electronic structure, artificial
nanoscale devices could offer a new and simpler vista to the comprehension of
quantum phase transitions. This long-sought possibility is demonstrated by our
work in a fullerene molecular junction, where gate voltage induces a crossing
of singlet and triplet spin states at zero magnetic field. Electronic tunneling
from metallic contacts into the quantum dot provides here the
necessary many-body correlations to observe a true quantum critical behavior.Comment: 8 pages, 5 figure
Kondo physics in carbon nanotubes
The connection of electrical leads to wire-like molecules is a logical step
in the development of molecular electronics, but also allows studies of
fundamental physics. For example, metallic carbon nanotubes are quantum wires
that have been found to act as one-dimensional quantum dots, Luttinger-liquids,
proximity-induced superconductors and ballistic and diffusive one-dimensional
metals. Here we report that electrically-contacted single-wall nanotubes can
serve as powerful probes of Kondo physics, demonstrating the universality of
the Kondo effect. Arising in the prototypical case from the interaction between
a localized impurity magnetic moment and delocalized electrons in a metallic
host, the Kondo effect has been used to explain enhanced low-temperature
scattering from magnetic impurities in metals, and also occurs in transport
through semiconductor quantum dots. The far higher tunability of dots (in our
case, nanotubes) compared with atomic impurities renders new classes of
Kondo-like effects accessible. Our nanotube devices differ from previous
systems in which Kondo effects have been observed, in that they are
one-dimensional quantum dots with three-dimensional metal (gold) reservoirs.
This allows us to observe Kondo resonances for very large electron number (N)
in the dot, and approaching the unitary limit (where the transmission reaches
its maximum possible value). Moreover, we detect a previously unobserved Kondo
effect, occurring for even values of N in a magnetic field.Comment: 7 pages, pdf onl
Spectroscopic analysis of finite size effects around a Kondo quantum dot
We consider a simple setup in which a small quantum dot is strongly connected
to a finite size box. This box can be either a metallic box or a finite size
quantum wire.The formation of the Kondo screening cloud in the box strongly
depends on the ratio between the Kondo temperature and the box level spacing.
By weakly connecting two metallic reservoirs to the quantum dot, a detailed
spectroscopic analysis can be performed. Since the transport channels and the
screening channels are almost decoupled, such a setup allows an easier access
to the measure of finite-size effects associated with the finite extension of
the Kondo cloud.Comment: contribution to Les Houches proceeding, ``Quantum magnetism'' 200
Kondo effect in an integer-spin quantum dot
The Kondo effect is a key many-body phenomenon in condensed matter physics.
It concerns the interaction between a localised spin and free electrons.
Discovered in metals containing small amounts of magnetic impurities, it is now
a fundamental mechanism in a wide class of correlated electron systems. Control
over single, localised spins has become relevant also in fabricated structures
due to the rapid developments in nano-electronics. Experiments have already
demonstrated artificial realisations of isolated magnetic impurities at
metallic surfaces, nanometer-scale magnets, controlled transitions between
two-electron singlet and triplet states, and a tunable Kondo effect in
semiconductor quantum dots. Here, we report an unexpected Kondo effect realised
in a few-electron quantum dot containing singlet and triplet spin states whose
energy difference can be tuned with a magnetic field. This effect occurs for an
even number of electrons at the degeneracy between singlet and triplet states.
The characteristic energy scale is found to be much larger than for the
ordinary spin-1/2 case.Comment: 12 page
Two-channel Kondo effect and renormalization flow with macroscopic quantum charge states
Many-body correlations and macroscopic quantum behaviors are fascinating
condensed matter problems. A powerful test-bed for the many-body concepts and
methods is the Kondo model which entails the coupling of a quantum impurity to
a continuum of states. It is central in highly correlated systems and can be
explored with tunable nanostructures. Although Kondo physics is usually
associated with the hybridization of itinerant electrons with microscopic
magnetic moments, theory predicts that it can arise whenever degenerate quantum
states are coupled to a continuum. Here we demonstrate the previously elusive
`charge' Kondo effect in a hybrid metal-semiconductor implementation of a
single-electron transistor, with a quantum pseudospin-1/2 constituted by two
degenerate macroscopic charge states of a metallic island. In contrast to other
Kondo nanostructures, each conduction channel connecting the island to an
electrode constitutes a distinct and fully tunable Kondo channel, thereby
providing an unprecedented access to the two-channel Kondo effect and a clear
path to multi-channel Kondo physics. Using a weakly coupled probe, we reveal
the renormalization flow, as temperature is reduced, of two Kondo channels
competing to screen the charge pseudospin. This provides a direct view of how
the predicted quantum phase transition develops across the symmetric quantum
critical point. Detuning the pseudospin away from degeneracy, we demonstrate,
on a fully characterized device, quantitative agreement with the predictions
for the finite-temperature crossover from quantum criticality.Comment: Letter (5 pages, 4 figures) and Methods (10 pages, 6 figures