3,492 research outputs found
Amorphous ferromagnetism and re-entrant magnetic glassiness in SmMoO: new insights into the electronic phase diagram of pyrochlore molybdates
We discuss the magnetic properties of a SmMoO single
crystal as investigated by means of different experimental techniques. In the
literature, a conventional itinerant ferromagnetic state is reported for the
Mo sublattice below K. However, our results of dc
magnetometry, muon spin spectroscopy (SR) and high-harmonics magnetic
ac susceptibility unambiguously evidence highly disordered conditions in this
phase, in spite of the crystalline and chemical order. This disordered magnetic
state shares several common features with amorphous ferromagnetic alloys. This
scenario for SmMoO is supported by the anomalously high
values of the critical exponents, as mainly deduced by a scaling analysis of
our dc magnetization data and confirmed by the other techniques. Moreover,
SR detects a significant static magnetic disorder at the microscopic
scale. At the same time, the critical divergence of the third-harmonic
component of the ac magnetic susceptibility around K leads to
additional evidence towards the glassy nature of this magnetic phase. Finally,
the longitudinal relaxation of spin polarization (also supported by
results of ac susceptibility) evidences re-entrant glassy features similar to
amorphous ferromagnets.Comment: 15 pages, 13 figure
Fishtail effect and vortex dynamics in LiFeAs single crystals
We investigate the fishtail effect, critical current density () and
vortex dynamics in LiFeAs single crystals. The sample exhibits a second peak
(SP) in the magnetization loop only with the field c-axis. We calculate a
reasonably high , however, values are lower than in 'Ba-122' and
'1111'-type FeAs-compounds. Magnetic relaxation data imply a strong pinning
which appears not to be due to conventional defects. Instead, its behavior is
similar to that of the triplet superconductor SrRuO. Our data suggest
that the origin of the SP may be related to a vortex lattice phase transition.
We have constructed the vortex phase diagram for LiFeAs on the
field-temperature plane.Comment: 5 pages, 5 figure
The superconducting gaps in LiFeAs: Joint study of specific heat and ARPES
We present specific heat, c_P, and ARPES data on single crystals of the
stoichiometric superconductor LiFeAs. A pronounced anomaly is found in c_P at
the superconducting transition. The electronic contribution can be described by
two s-type energy gaps with magnitudes of approximately Delta1 = 1.2 meV and
Delta2 = 2.6 meV and a normal-state gamma coefficient of 10 mJ/mol K^2. All
these values are in remarkable agreement with ARPES results.Comment: 4 pages, 3 figure
Nature of the spin dynamics and 1/3 magnetization plateau in azurite
We present a specific heat and inelastic neutron scattering study in magnetic
fields up into the 1/3 magnetization plateau phase of the diamond chain
compound azurite Cu(CO)(OH). We establish that the
magnetization plateau is a dimer-monomer state, {\it i.e.}, consisting of a
chain of monomers, which are separated by dimers on the
diamond chain backbone. The effective spin couplings K
and K are derived from the monomer and dimer
dispersions. They are associated to microscopic couplings K,
K and a ferromagnetic K, possibly as
result of orbitals in the Cu-O bonds providing the superexchange
pathways.Comment: 5 pages, 4 figure
Giant spin canting in the S = 1/2 antiferromagnetic chain [CuPM(NO3)2(H2O)2]n observed by 13C-NMR
We present a combined experimental and theoretical study on copper pyrimidine
dinitrate [CuPM(NO3)2(H2O)2]n, a one-dimensional S = 1/2 antiferromagnet with
alternating local symmetry. From the local susceptibility measured by NMR at
the three inequivalent carbon sites in the pyrimidine molecule we deduce a
giant spin canting, i.e., an additional staggered magnetization perpendicular
to the applied external field at low temperatures. The magnitude of the
transverse magnetization, the spin canting of 52 degrees at 10 K and 9.3 T and
its temperature dependence are in excellent agreement with exact
diagonalization calculations.Comment: 5 pages, 6 Postscript figure
Electronic structure of the molecule based magnet Cu PM(NO3)2 (H2O)2
We present density functional calculations on the molecule based S=1/2
antiferromagnetic chain compound Cu PM(NO3)2 (H2O)2; PM = pyrimidine. The
properties of the ferro- and antiferromagnetic state are investigated at the
level of the local density approximation and with the hybrid functional B3LYP.
Spin density maps illustrate the exchange path via the pyrimidine molecule
which mediates the magnetism in the one-dimensional chain. The computed
exchange coupling is antiferromagnetic and in reasonable agreement with the
experiment. It is suggested that the antiferromagnetic coupling is due to the
possibility of stronger delocalization of the charges on the nitrogen atoms,
compared to the ferromagnetic case. In addition, computed isotropic and
anisotropic hyperfine interaction parameters are compared with recent NMR
experiments
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