Absence of structural correlations of magnetic defects in heavy fermion LiV2O4

Magnetic defects have pronounced effects on the magnetic properties of the face-centered cubic compound LiV2O4. The magnetic defects arise from crystal defects present within the normal spinel structure. High-energy x-ray diffraction studies were performed on LiV2O4 single crystals to search for superstructure peaks or any other evidence of periodicity in the arrangement of the crystal defects present in the lattice. Entire reciprocal lattice planes are mapped out with help of synchrotron radiation. No noticeable differences in the x-ray diffraction data between a crystal with high magnetic defect concentration and a crystal with low magnetic defect concentration have been found. This indicates the absence of any long-range periodicity or short-range correlations in the arrangements of the crystal/magnetic defects.Comment: 6 pages, 4 figure

Nature of the Magnetic Order in BaMn2As2

Neutron diffraction measurements have been performed on a powder sample of BaMn2As2 over the temperature T range from 10 K to 675 K. These measurements demonstrate that this compound exhibits collinear antiferromagnetic ordering below the Neel temperature T_N = 625(1) K. The ordered moment mu = 3.88(4) mu_B/Mn at T = 10 K is oriented along the c axis and the magnetic structure is G-type, with all nearest-neighbor Mn moments antiferromagnetically aligned. The value of the ordered moment indicates that the oxidation state of Mn is Mn^{2+} with a high spin S = 5/2. The T dependence of mu suggests that the magnetic transition is second-order in nature. In contrast to the closely related AFe2As2 (A = Ca, Sr, Ba, Eu) compounds, no structural distortion is observed in the magnetically ordered state of BaMn2As2.Comment: 4 pages, 3 figures, 1 table; v2: additional discussion of Mn-Mn interactions; accepted for publication as a Rapid Communication in Phys. Rev.

Intrinsic pinning on structural domains in underdoped single crystals of Ba(Fe1−x_{1-x}Cox_x)2_2As2_2

Critical current density was studied in single crystals of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ for the values of $x$ spanning the entire doping phase diagram. A noticeable enhancement was found for slightly underdoped crystals with the peak at $x = 0.058$. Using a combination of polarized-light imaging, x-ray diffraction and magnetic measurements we associate this behavior with the intrinsic pinning on structural domains in the orthorhombic phase. Domain walls extend throughout the sample thickness in the direction of vortices and act as extended pinning centers. With the increasing $x$ domain structure becomes more intertwined and fine due to a decrease of the orthorhombic distortion. This results in the energy landscape with maze-like spatial modulations favorable for pinning. This finding shows that iron-based pnictide superconductors, characterized by high values of the transition temperature, high upper critical fields, and low anisotropy may intrinsically have relatively high critical current densities.Comment: estimation of Jc correcte

Magnetic ordering in EuRh2As2 studied by x-ray resonant magnetic scattering

Element-specific x-ray resonant magnetic scattering investigations were performed to determine the magnetic structure of Eu in EuRh2As2. In the temperature range from 46 K down to 6 K, an incommensurate antiferromagnetic (ICM)structure with a temperature dependent propagation vector (0 0 0.9) coexists with a commensurate antiferromagnetic (CM) structure. Angular-dependent measurements of the magnetic intensity indicate that the magnetic moments lie in the tetragonal basal plane and are ferromagnetically aligned within the a-b plane for both magnetic structures. The ICM structure is a spiral-like magnetic structure with a turn angle of 162 deg between adjacent Eu planes. In the CM structure, this angle is 180 deg. These results are consistent with band-structure calculations which indicate a strong sensitivity of the magnetic configuration on the Eu valence.Comment: 5 pages, 5 figures (technical problem with abstract corrected, no other changes